Article(id=1319237172817936404, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319237171312177253, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220469, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1654790400000, receivedDateStr=2022-06-10, revisedDate=1661443200000, revisedDateStr=2022-08-26, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460252241, onlineDateStr=2026-10-20, pubDate=1671465600000, pubDateStr=2022-12-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460252241, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460252241, creator=13701087609, updateTime=1792460252241, updator=13701087609, issue=Issue{id=1319237171312177253, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='12', pageStart='3091', pageEnd='3336', issueExtLink='null', onlineDate='null', pubDate='1671465600000', pubDateStr='2022-12-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460251882, creator='13701087609', updateTime=1792460721974, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319239143067071226, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319237171312177253, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319239143067071227, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319237171312177253, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=3116, endPage=3125, ext={EN=ArticleExt(id=1319237172985708565, articleId=1319237172817936404, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Thermally Enhanced High-sensitivity Temperature Probe ScF₃: Nd³⁺/Yb³⁺/Er³⁺ Based on Negative Thermal Expansion, columnId=1321891473390415997, journalTitle=Journal of the Chinese Ceramic Society, columnName=Advanced Rare Earth Luminescence Materials for Sensing and Detection—Research Articles, runingTitle=null, highlight=null, articleAbstract=

Rapid and non-invasive temperature detection inside biological tissues can be realized through a fluorescence intensity ratio thermometry technology, but it is still restricted due to the thermal quenching of fluorescence and the large absorption and scattering coefficients of tissues in practical applications. In this paper, cubic phase ScF₃:Yb³⁺/Er³⁺ nanocrystals with negative thermal expansion characteristics were synthesized by a one-step hydrothermal method, in which the thermal enhancement of up-conversion (UC) luminescence was achieved due to the thermally improved energy transfer efficiency from a shortened distance between the activator and sensitizer. For further realizing its application in biology, Nd³⁺ was introduced in ScF₃:Yb³⁺/Er³⁺ to construct a high-sensitivity temperature probe with near-infrared (NIR) excitation and NIR emission. Furthermore, calibrating the temperature measurement curve and designing the ex vivo experiment rationally can give a potential temperature detection of the present sample inside the tissue. The results indicate a strategy for solving the UC luminescence thermal quenching and developing NIR emission temperature probes for organisms.

, authors=Minkun JIN, Jinmeng XIANG, Changheng CHEN, Yuexin LI, Jingjing TANG, Chongfeng GUO, authorsList=Minkun JIN, Jinmeng XIANG, Changheng CHEN, Yuexin LI, Jingjing TANG, Chongfeng GUO, authorCompany=null, correspAuthors=Chongfeng GUO, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319237173359001622, articleId=1319237172817936404, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=基于负热膨胀的热增强型ScF₃：Nd³⁺/Yb³⁺/Er³⁺高灵敏度温度探针, columnId=1321891473621102718, journalTitle=硅酸盐学报, columnName=稀土发光传感与探测新材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

荧光强度比测温技术在生物组织内部实现了快速和无创的温度探测，但在实际应用中仍受荧光热猝灭及生物组织较大的吸收与散射的影响。本工作采用一步水热法制备了长方体ScF₃：Yb³⁺/Er³⁺纳米晶，利用ScF₃特有的负热膨胀属性，提高了激活剂与敏化剂之间的能量传递效率，实现了上转换发光整体34倍的热增强。同时，引入Nd³⁺构建了近红外-近红外高灵敏度的温度探针（S_a = 0.112 0 K^-1在400 K），并通过对测温曲线的矫正和离体实验，证明了样品在组织内部的测温性能，为解决上转换发光热猝灭和开发生物近红外发射温度探针提供了新的设计思路。

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金旻坤（1997—），男，博士研究生。

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