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Article(id=1319236719862468763, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236705027207343, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220209, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1647964800000, receivedDateStr=2022-03-23, revisedDate=1649865600000, revisedDateStr=2022-04-14, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460144247, onlineDateStr=2026-10-20, pubDate=1666195200000, pubDateStr=2022-10-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460144247, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460144247, creator=13701087609, updateTime=1792460144247, updator=13701087609, issue=Issue{id=1319236705027207343, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='10', pageStart='2579', pageEnd='2808', issueExtLink='null', onlineDate='null', pubDate='1666195200000', pubDateStr='2022-10-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460140711, creator='13701087609', updateTime=1792460672919, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319238937323884737, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236705027207343, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319238937323884738, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236705027207343, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2722, endPage=2733, ext={EN=ArticleExt(id=1319236720114127004, articleId=1319236719862468763, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Development on Recycling Rare Metal Lithium from Waste Lithium-Ion Batteries, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

The demand for lithium-ion batteries (LIBs) is increasing with a rapid development of new energy vehicles. Massive waste LIBs pollute the environment and have a risk of insufficient supply of lithium resources. Recycling metal lithium from waste LIBs thus becomes a recent research hotspot. Effective battery recycling can alleviate the shortage of resources and realize resource utilization, as well as reduce environmental pollution and promote the sustainable development of the industry. Also, research work on recovering lithium by preferential extraction and step-by-step separation has attracted much attentions to realize the efficient recovery of lithium metal in waste LIBs. This review represented the existing situation and methods of recycling waste LIBs, described recent research work on pyrometallurgy, hydrometallurgy, bio metallurgy and electrochemical methods in the process of selective lithium recovery, and analyzed the technical features of electrode electric field drive and membrane electrodialysis in the field of selective lithium recovery. Also, the advantages and disadvantages of each recovery process were summarized, and the problems faced by lithium recovery were analyzed in combination with economic benefits and environmental impact. In addition, the challenges and limitations of LIBs recycling were given, and the future development on LIBs recycling was prospected. This review thus provides a reference for the research and development of more energy-saving, environment-friendly and efficient recycling process of lithium metal in waste LIBs.

, authors=Jilong HAN1, Kuihu WANG1, Lilong ZHOU1, Zhengjie LI1, Hanya ZHANG1, Qingfen MENG2, Jimmy YUN3, authorsList=Jilong HAN, Kuihu WANG, Lilong ZHOU, Zhengjie LI, Hanya ZHANG, Qingfen MENG, Jimmy YUN, authorCompany=null, correspAuthors=Zhengjie LI, Qingfen MENG, authorNote=

HAN Jilong (1982-), male, Ph.D., Lecturer. E-mail:

, correspAuthorsNote=
MENG Qingfen (1980-), female, Ph.D., Professor; E-mail:
LI Zhengjie (1988-), male, Ph.D., Lecturer.
, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319236720374173853, articleId=1319236719862468763, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=废旧锂离子电池回收稀有金属锂的研究进展和展望, columnId=1263922774356181565, journalTitle=硅酸盐学报, columnName=综合评述, runingTitle=null, highlight=null, articleAbstract=

随着新能源汽车的迅速发展，锂离子电池（LiBs）需求不断增加，大量废旧LiBs对环境造成污染，同时面临着锂资源供给不足的风险，回收废LiBs中稀有金属锂成为目前研究的热点。有效的电池回收不仅可以缓解资源短缺、实现资源利用，更重要的是可以减少环境污染，推动行业可持续发展。为实现废旧LiBs中锂金属的高效回收，通过优先提取及分步分离的方式回收锂工艺受到研究者的广泛关注。本文对废旧LiBs回收现状及方法进行了阐述，讨论了火法冶金、湿法冶金、生物冶金及电化学法在选择性回收锂工艺上的最新研究进展，详细分析了电极-电场驱动与膜-电渗析技术在选择性回收锂领域的技术优势，同时归纳了各回收工艺的优缺点，并结合经济效益和环境影响对锂回收所面临的问题进行了总结分析。最后，对LiBs回收利用面临的挑战和局限性进行总结，并对未来LiBs回收的发展趋势进行了展望，为研发更加节能环保高效的回收工艺提供参考。

, authors=韩继龙1, 王奎虎1, 周理龙1, 李正杰1, 张含雅1, 孟庆芬2, Jimmy Yun3, authorsList=韩继龙, 王奎虎, 周理龙, 李正杰, 张含雅, 孟庆芬, Jimmy Yun, authorCompany=null, correspAuthors=李正杰, 孟庆芬, authorNote=

韩继龙（1982—），男，博士，讲师。

, correspAuthorsNote=
孟庆芬（1980—），女，博士，研究员；
李正杰（1988—），男，博士，讲师。
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HAN Jilong (1982-), male, Ph.D., Lecturer. E-mail:

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HAN Jilong (1982-), male, Ph.D., Lecturer. E-mail:

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韩继龙（1982—），男，博士，讲师。

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韩继龙（1982—），男，博士，讲师。

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废旧锂离子电池回收稀有金属锂的研究进展和展望
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韩继龙 1 , 王奎虎 1 , 周理龙 1 , 李正杰 1 , 张含雅 1 , 孟庆芬 2 , Jimmy Yun 3
硅酸盐学报 | 综合评述 2022,50(10): 2722-2733
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硅酸盐学报 |综合评述 2022 , 50 (10) : 2722 -2733
废旧锂离子电池回收稀有金属锂的研究进展和展望
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韩继龙（1982—），男，博士，讲师。

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韩继龙1 , 王奎虎1, 周理龙1, 李正杰1 , 张含雅1, 孟庆芬2 , Jimmy Yun3
作者信息
  • 1．河北科技大学，石家庄 050018
  • 2．金昆仑锂业有限公司，青海 格尔木 817000
  • 3．天俱时工程科技集团有限公司，石家庄 050000
通讯作者:
孟庆芬（1980—），女，博士，研究员；
李正杰（1988—），男，博士，讲师。
作者简介:

韩继龙（1982—），男，博士，讲师。

Development on Recycling Rare Metal Lithium from Waste Lithium-Ion Batteries
Jilong HAN1 , Kuihu WANG1, Lilong ZHOU1, Zhengjie LI1 , Hanya ZHANG1, Qingfen MENG2 , Jimmy YUN3
Affiliations
  • 1.Hebei University of Science and Technology, Shijiazhuang 050018, China
  • 2.Jin Kunlun Lithium Industry Co., Ltd., Golmud 817000, Qinghai, China
  • 3.Tianjushi Engineering Technology Group Co., Ltd., Shijiazhuang 050000, China
    • Corresponding Author:
    MENG Qingfen (1980-), female, Ph.D., Professor; E-mail:
    LI Zhengjie (1988-), male, Ph.D., Lecturer.

    HAN Jilong (1982-), male, Ph.D., Lecturer. E-mail:

出版时间: 2022-10-20 doi: 10.14062/j.issn.0454-5648.20220209
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随着新能源汽车的迅速发展，锂离子电池（LiBs）需求不断增加，大量废旧LiBs对环境造成污染，同时面临着锂资源供给不足的风险，回收废LiBs中稀有金属锂成为目前研究的热点。有效的电池回收不仅可以缓解资源短缺、实现资源利用，更重要的是可以减少环境污染，推动行业可持续发展。为实现废旧LiBs中锂金属的高效回收，通过优先提取及分步分离的方式回收锂工艺受到研究者的广泛关注。本文对废旧LiBs回收现状及方法进行了阐述，讨论了火法冶金、湿法冶金、生物冶金及电化学法在选择性回收锂工艺上的最新研究进展，详细分析了电极-电场驱动与膜-电渗析技术在选择性回收锂领域的技术优势，同时归纳了各回收工艺的优缺点，并结合经济效益和环境影响对锂回收所面临的问题进行了总结分析。最后，对LiBs回收利用面临的挑战和局限性进行总结，并对未来LiBs回收的发展趋势进行了展望，为研发更加节能环保高效的回收工艺提供参考。

锂离子电池  /  资源利用  /  锂金属  /  回收工艺  /  电化学

The demand for lithium-ion batteries (LIBs) is increasing with a rapid development of new energy vehicles. Massive waste LIBs pollute the environment and have a risk of insufficient supply of lithium resources. Recycling metal lithium from waste LIBs thus becomes a recent research hotspot. Effective battery recycling can alleviate the shortage of resources and realize resource utilization, as well as reduce environmental pollution and promote the sustainable development of the industry. Also, research work on recovering lithium by preferential extraction and step-by-step separation has attracted much attentions to realize the efficient recovery of lithium metal in waste LIBs. This review represented the existing situation and methods of recycling waste LIBs, described recent research work on pyrometallurgy, hydrometallurgy, bio metallurgy and electrochemical methods in the process of selective lithium recovery, and analyzed the technical features of electrode electric field drive and membrane electrodialysis in the field of selective lithium recovery. Also, the advantages and disadvantages of each recovery process were summarized, and the problems faced by lithium recovery were analyzed in combination with economic benefits and environmental impact. In addition, the challenges and limitations of LIBs recycling were given, and the future development on LIBs recycling was prospected. This review thus provides a reference for the research and development of more energy-saving, environment-friendly and efficient recycling process of lithium metal in waste LIBs.

lithium ion battery  /  resource utilization  /  lithium metal  /  recovery process  /  electrochemistry
韩继龙, 王奎虎, 周理龙, 李正杰, 张含雅, 孟庆芬, Jimmy Yun. 废旧锂离子电池回收稀有金属锂的研究进展和展望. 硅酸盐学报, 2022 , 50 (10) : 2722 -2733 . DOI: 10.14062/j.issn.0454-5648.20220209
Jilong HAN, Kuihu WANG, Lilong ZHOU, Zhengjie LI, Hanya ZHANG, Qingfen MENG, Jimmy YUN. Development on Recycling Rare Metal Lithium from Waste Lithium-Ion Batteries[J]. Journal of the Chinese Ceramic Society, 2022 , 50 (10) : 2722 -2733 . DOI: 10.14062/j.issn.0454-5648.20220209
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  • 青海省海西州科技局企业创新资金计划项目(2019-104)
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doi: 10.14062/j.issn.0454-5648.20220209
  • 接收时间：2022-03-23
  • 首发时间：2026-10-20
  • 出版时间：2022-10-20
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  • 收稿日期：2022-03-23
  • 修回日期：2022-04-14
基金
青海省海西州科技局企业创新资金计划项目(2019-104)
作者信息
    1．河北科技大学，石家庄 050018
    2．金昆仑锂业有限公司，青海 格尔木 817000
    3．天俱时工程科技集团有限公司，石家庄 050000

通讯作者:

孟庆芬（1980—），女，博士，研究员；
李正杰（1988—），男，博士，讲师。
参考文献
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20220209
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2种不同金属材料的力学参数
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Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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