Article(id=1319236616779055139, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236561179366013, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220331, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1650902400000, receivedDateStr=2022-04-26, revisedDate=1654617600000, revisedDateStr=2022-06-08, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460119670, onlineDateStr=2026-10-20, pubDate=1663603200000, pubDateStr=2022-09-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460119670, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460119670, creator=13701087609, updateTime=1792460119670, updator=13701087609, issue=Issue{id=1319236561179366013, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='9', pageStart='2351', pageEnd='2578', issueExtLink='null', onlineDate='null', pubDate='1663603200000', pubDateStr='2022-09-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460106415, creator='13701087609', updateTime=1792460650608, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319238843744764843, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236561179366013, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319238843744764844, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236561179366013, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2501, endPage=2509, ext={EN=ArticleExt(id=1319236617034907684, articleId=1319236616779055139, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Fluorescence Properties and Thermal Stability of Sr₂Gd_1-xNbO6: xEu³⁺ with Dual-Wavelength Wxcitation Response, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

A series of Sr₂GdNbO₆:xEu³⁺ (x=0.04-0.12) red phosphors were prepared by a high-temperature solid-phase method, and the target products were characterized by X-ray diffraction, UV-Vis spectrophotometry and fluorescence spectroscopy. The results show that the synthesized phosphor has a monoclinic crystal structure with the space group P2₁/c. The structural analysis indicates that doped europium replaces Gd³⁺ ion in the matrix Sr₂GdNbO₆ with the chemical state of Eu³⁺ ion, thus forming a single crystal structure phosphor. Sr₂GdNbO₆:Eu³⁺ phosphor exhibits a red-orange emission under dual-wavelength excitation of blue light λ_ex of 468 nm and near-ultraviolet light λ_ex of 395 nm, and the main emission peaks are centered at wavelengths of 622 nm and 593 nm, which belong to the ⁵D₀→⁷F₂ and ⁵D₀→⁷F₁ energy level transitions of Eu³⁺, respectively. When the doping amount (x) of Eu³⁺ is 8%, its luminescence quantum efficiency for blue light excitation reaches the maximum value of 16%. Based on the analysis and comparison of the temperature (295-568 K) effect on the emission intensity and quantum efficiency under dual-wavelength excitation, the phosphor has a high luminescence quantum efficiency under the excitation of blue light λ_ex of 468 nm and a higher thermal stability. Under the excitation of blue light, the average fluorescence decay lifetime of the sample Sr₂GdNbO₆: 0.08Eu³⁺ is 0.841 ms, the color coordinates are (0.648, 0.368), and the luminescence purity reaches 93%. This phosphor is a kind of red fluorescent material with the dual-wavelength response for a promising potential application.

, authors=Ying LI¹, Guodong FAN¹, Fangyi RUAN¹, Jianfeng ZHOU¹, Qianqian CHEN¹, Tuo WANG², authorsList=Ying LI, Guodong FAN, Fangyi RUAN, Jianfeng ZHOU, Qianqian CHEN, Tuo WANG, authorCompany=null, correspAuthors=Guodong FAN, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319236617299148837, articleId=1319236616779055139, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=双激发波长响应的Sr₂Gd_1-xNbO₆：xEu³⁺的荧光性能与热稳定性, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

针对目前钙钛矿型红色荧光粉热稳定性较差的问题，以带隙和结构可调变的双钙钛矿型Sr₂GdNbO₆为基质、Eu³⁺为激活离子，采用高温固相法成功制备双钙钛矿型Sr₂Gd_1-xNbO₆：xEu³⁺（x=0.04~0.12）红色荧光粉，通过X射线衍射、紫外-可见分光光度和荧光光谱分析对目标产物进行表征。结果表明：合成的荧光粉具有单斜晶体结构，其空间群为P2₁/c。结构分析表明：掺杂的铕以Eu³⁺的化合态取代了基质Sr₂GdNbO₆中的Gd³⁺，形成了单一晶体结构的荧光粉。Sr₂Gd_1-xNbO₆：xEu³⁺荧光粉在蓝光λ_ex=468 nm和近紫外λ_ex=395 nm双波长激发下均呈现红橙色发射光，主发射峰中心波长位于622 nm和593 nm处，分别归属于Eu³⁺的⁵D₀→⁷F₂和⁵D₀→⁷F₁能级跃迁。当Eu³⁺的掺杂量为x=8%（摩尔分数），其蓝光激发的发光量子效率达到最高值16%。对比分析了双波长激发下温度（295~568 K）对其荧光强度和发光量子效率的影响。结果表明：蓝光λ_ex=468 nm激发下该荧光粉不仅发光量子效率高，而且其耐热稳定性也更高。在蓝光激发下样品Sr₂GdNbO₆：0.08Eu³⁺的荧光衰减平均寿命为0.841 ms，色坐标为（0.648、0.368），发光色纯度达到93%，是一种具有应用潜在前景的双波长响应的新型红色荧光材料。

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LI Ying (1995-), female, Master candidate. E-mail: 982195550@qq.com

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LI Ying (1995-), female, Master candidate. E-mail: 982195550@qq.com

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李瑛（1995—），女，硕士研究生。

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李瑛（1995—），女，硕士研究生。

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