Article(id=1319232615727612076, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319232566922695375, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20211056, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1638720000000, receivedDateStr=2021-12-06, revisedDate=1641225600000, revisedDateStr=2022-01-04, acceptedDate=null, acceptedDateStr=null, onlineDate=1792459165745, onlineDateStr=2026-10-20, pubDate=1658246400000, pubDateStr=2022-07-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792459165745, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792459165745, creator=13701087609, updateTime=1792459165745, updator=13701087609, issue=Issue{id=1319232566922695375, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='7', pageStart='1775', pageEnd='2066', issueExtLink='null', onlineDate='null', pubDate='1658246400000', pubDateStr='2022-07-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792459154109, creator='13701087609', updateTime=1792460038980, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319236278420357264, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319232566922695375, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319236278420357265, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319232566922695375, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1978, endPage=1987, ext={EN=ArticleExt(id=1319232615996047533, articleId=1319232615727612076, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Preparation and Pervaporation Performance of SiO₂@ZIF-8 Composite Membrane, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

Silicon dioxide (SiO₂) membrane has attracted much attention in the field of separation and purification due to its high-temperature resistance and adjustable pore size. However, the amorphous structure on the surface leads to the mutual restriction of permeability and selectivity, which affects the results of separation. A SiO₂@ZIF-8 composite membrane was prepared with SiO₂ membrane as abase membrane and modified with metal organic framework material (ZIF-8). The effects of synthesis condition of ZIF-8, addition amount of ZIF-8 and temperature of raw material solution on the dehydration inaqueous ethanol solution mixture under pervaporation conditions were investigated. The results show that the regular channel structure in ZIF-8 can provide additional channels for water molecule transport, the water content on the permeate side of the composite membrane is 99.5 %, the permeate flux increasesto 9.6 kg/(m²·h) and the separation factor is 1 973. A relationship between membrane permeation flux and temperature follows the Arrhenius equation. The apparent activation energy of water molecules in the composite membrane is higher, and the water flux increases faster with the increase of temperature, indicating a better separation effect. SiO₂@ZIF-8 composite membrane can effectively improve the defects of amorphous network structure of silica film, which has a broad application prospect in the dehydration of organic solvent by pervaporation.

, authors=Hongdan WU, Zhaoying SUN, Zhihui ZHOU, Xiaodi LIU, authorsList=Hongdan WU, Zhaoying SUN, Zhihui ZHOU, Xiaodi LIU, authorCompany=null, correspAuthors=Zhihui ZHOU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319232616377729198, articleId=1319232615727612076, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=SiO₂@ZIF-8复合膜的制备及渗透汽化性能, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

二氧化硅（SiO₂）膜因其耐高温且孔径可调在分离纯化领域得到了广泛关注，但其表面的无定型结构导致渗透性与选择性相互制约，影响分离效果。以二氧化硅膜为基膜，金属有机框架材料（ZIF-8）对其进行修饰改性，制得SiO₂@ZIF-8复合膜，探究了ZIF-8合成条件、ZIF-8添加量及原料液温度对复合膜乙醇渗透汽化脱水性能的影响。结果表明：ZIF-8规则的孔道结构提供了额外的水分子传输通道，复合膜的渗透侧含水率可达99.5%，渗透通量提高至9.6 kg/（m²·h），分离因子为1973。采用Arrhenius方程对改性前后膜的渗透通量与温度的关系进行拟合，发现复合膜在渗透汽化过程中水分子的表观活化能更高，随着温度升高水通量增加的更快，分离效果更好。SiO₂@ZIF-8复合膜有效改善了无定型网状结构的缺陷，在渗透汽化有机溶剂脱水方面具有广阔的应用前景。

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WU Hongdan (1982-), female, Lecturer. E-mail: wu_dan725@wust.edu.cn

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WU Hongdan (1982-), female, Lecturer. E-mail: wu_dan725@wust.edu.cn

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吴红丹（1982—），女，讲师。

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吴红丹（1982—），女，讲师。

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