Article(id=1319222740398224077, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220860, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1665417600000, receivedDateStr=2022-10-11, revisedDate=1667404800000, revisedDateStr=2022-11-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456811284, onlineDateStr=2026-10-20, pubDate=1687190400000, pubDateStr=2023-06-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456811284, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456811284, creator=13701087609, updateTime=1792456811284, updator=13701087609, issue=Issue{id=1319222716851405704, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='6', pageStart='1373', pageEnd='1648', issueExtLink='null', onlineDate='null', pubDate='1687190400000', pubDateStr='2023-06-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456805669, creator='13701087609', updateTime=1792456995739, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319223514108903801, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319223514108903802, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1555, endPage=1564, ext={EN=ArticleExt(id=1319222740599550670, articleId=1319222740398224077, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Design and Preparation of Y
3Al
5O
12-Al
4SiC
4 Composite Refractory, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=
Y3Al5O12-Al4SiC4 composite refractory was prepared via pressureless sintering with Al4SiC4 as a raw material and Y2O3 as an additive. The effect of Y2O3 addition (i.e., 0-5% in mass fraction) on the phase composition, microstructure and mechanical properties of the composite was investigated, and the effect of Y3+ ions on the surface energy of Al4SiC4 different crystal faces was calculated via the DFT simulation. The results show that the addition of Y2O3 can form an eutectic liquid phase with anintrinsic oxide layer on the surface of Al4SiC4 at a high temperature, Y3Al5O12 and a small amount of Y2SiO5 appear at the grain boundary of the composite.The addition of Y2O3 promotes the growth of Al4SiC4 grains along the two-dimensional plane and the transformation from irregular to hexagonal flakes due to the reduction of surface energy of different crystal faces of Al4SiC4 by Y3+ in the additive, according to the DFT results. The flexural strength of the composite first increases and then decreases with the increase of Y2O3 addition. At theY2O3 addition of 3%, the hexagonal lamellar Al4SiC4 grains with a uniform size form a staggered skeleton structure, and Y3Al5O12 dispersesat the grain boundary of Al4SiC4, which is conducive to the improvement of the mechanical properties of Y3Al5O12-Al4SiC4 composite. The bulk density, apparent porosity and flexural strength of the composite are 2.44 g·cm-3, 20.15% and 52.7 MPa, respectively.
, authors=Xiaobing DENG
1, Chengji DENG
1, Guangchao XING
1, Jun DING
1, Zhoufu WANG
1, Beiyue MA
2, Hongxi ZHU
1, Chao YU
1, authorsList=Xiaobing DENG, Chengji DENG, Guangchao XING, Jun DING, Zhoufu WANG, Beiyue MA, Hongxi ZHU, Chao YU, authorCompany=null, correspAuthors=Chao YU, authorNote=
, correspAuthorsNote=
, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222740956066511, articleId=1319222740398224077, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=Y
3Al
5O
12-Al
4SiC
4复合耐火材料的设计与制备, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=
以Al4SiC4为原料、Y2O3为添加剂,采用无压烧结制备Y3Al5O12-Al4SiC4复合耐火材料,研究Y2O3添加量[0~5%(质量分数)]对复合材料物相组成、微观形貌与力学性能的影响,并通过DFT模拟计算Y3+对Al4SiC4不同晶面表面能的影响。结果表明:高温下Y2O3与Al4SiC4表面固有氧化层形成共晶液相,在复合材料晶界处生成Y3Al5O12和少量Y2SiO5。Y2O3的添加促使Al4SiC4晶粒沿二维平面生长,由不规则状向六方片状转变,这是由于添加剂中Y3+降低了晶面的表面能。复合材料的抗折强度随Y2O3添加量增加呈现先增大后降低趋势,当Y2O3添加量为3%时,尺寸均一的六方片状Al4SiC4晶粒交错生长构筑成骨架结构,Y3Al5O12弥散分布于Al4SiC4晶界处,Y3Al5O12-Al4SiC4复合材料力学性能得到提升,复合材料体积密度、显气孔率和抗折强度分别为2.44 g·cm-3、20.15%和52.7 MPa。
, authors=邓孝兵
1, 邓承继
1, 邢广超
1, 丁军
1, 王周福
1, 马北越
2, 祝洪喜
1, 余超
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, correspAuthorsNote=
余超(1986—),男,博士,副教授。
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DENG Xiaobing (1997-), male, Master candidate. E-mail: 1564847843@qq.com
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邓孝兵(1997—),男,硕士研究生。
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