Article(id=1319222685213770386, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222668956643677, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220823, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1664467200000, receivedDateStr=2022-09-30, revisedDate=1665331200000, revisedDateStr=2022-10-10, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456798127, onlineDateStr=2026-10-20, pubDate=1684512000000, pubDateStr=2023-05-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456798127, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456798127, creator=13701087609, updateTime=1792456798127, updator=13701087609, issue=Issue{id=1319222668956643677, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='5', pageStart='1091', pageEnd='1372', issueExtLink='null', onlineDate='null', pubDate='1684512000000', pubDateStr='2023-05-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456794251, creator='13701087609', updateTime=1792456976356, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319223432827490920, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222668956643677, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319223432827490921, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222668956643677, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1146, endPage=1153, ext={EN=ArticleExt(id=1319222685461234323, articleId=1319222685213770386, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Modification of Cellulose Nanocrystals on Microstructure of Calcium Silicate Hydrate, columnId=1321891041012200067, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Progress on Cement-Based Materials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

Calcium silicate hydrate (C-S-H) gel is a gene of cement-based cementitious materials, and its structural changes are crucial to the development of concrete macroscopic properties. To clarify the modification mechanism of cellulose nanocrystals (CNCs) in cement, C-S-H gels were prepared by a co-precipitation method, and the morphological and nucleation effects of CNCs on the microstructure of C-S-H gels were investigated by X-ray diffraction (XRD), transmission electron microscopy, nanoindentation, and nuclear magnetic resonance. The results show that the hydroxyl groups (—OH) on the surface of CNCs can complex Ca²⁺ ions, and then react with SiO₄^2- ions in solution to form C-S-H gels that wraps around the CNCs. The CNCs can provide additional nucleation sites for the precipitation and growth of C-S-H gels, promote the reduction of the polymerization degree and the shortening of the chain length of the C-S-H gel, and increase the content of high-density C-S-H gel.

, authors=Dapeng ZHENG, Yuan FANG, Hongzhi CUI, authorsList=Dapeng ZHENG, Yuan FANG, Hongzhi CUI, authorCompany=null, correspAuthors=Hongzhi CUI, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222685691921044, articleId=1319222685213770386, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=纤维素纳米晶对水化硅酸钙微观结构的改性机理, columnId=1321891041192555140, journalTitle=硅酸盐学报, columnName=水泥基材料研究新进展—研究论文, runingTitle=null, highlight=null, articleAbstract=

水化硅酸钙（C-S-H）作为水泥基胶凝材料的基因，其结构变化对混凝土宏观性能发展至关重要。为了明确纤维素纳米晶（CNCs）在水泥中的改性机理，采用共沉淀法制备C-S-H凝胶，探讨了CNCs的形态效应及成核效应对C-S-H凝胶结构的影响。基于X射线衍射、透射电子显微镜、纳米压痕以及核磁共振等测试，结果显示CNCs表面携带的羟基（—OH）可络合Ca²⁺，随后与溶液中的SiO₄^2-反应形成C-S-H凝胶，包裹在CNCs周围形成致密的网络结构。CNCs为C-S-H凝胶的沉淀和生长提供了额外的成核位点，促进了C-S-H凝胶聚合度的降低以及链长的缩短，并且显著提升了高密度C-S-H凝胶的含量。

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ZHENG Dapeng (1991-), male, Ph.D. E-mail: dapengzheng@szu.edu.cn

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郑大鹏（1991—），男，博士。

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