Article(id=1319222571392942623, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222570398888648, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220874, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1665676800000, receivedDateStr=2022-10-14, revisedDate=1667318400000, revisedDateStr=2022-11-02, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456770989, onlineDateStr=2026-10-20, pubDate=1679241600000, pubDateStr=2023-03-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456770989, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456770989, creator=13701087609, updateTime=1792456770989, updator=13701087609, issue=Issue{id=1319222570398888648, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='3', pageStart='561', pageEnd='830', issueExtLink='null', onlineDate='null', pubDate='1679241600000', pubDateStr='2023-03-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456770752, creator='13701087609', updateTime=1792456924637, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319223215889699377, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222570398888648, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319223215889699378, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222570398888648, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=562, endPage=570, ext={EN=ArticleExt(id=1319222571581686304, articleId=1319222571392942623, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Infrared Emission Properties of Ni²⁺ Ions Doped MgCr₂O₄ Materials, columnId=1321891096775472081, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Advances in Basic Research on Refractories Related—Research Articles, runingTitle=null, highlight=null, articleAbstract=

It is important to develop high emissivity infrared radiation materials for energy saving in high-temperature furnaces. In this work, Ni²⁺-doped MgCr₂O₄ materials were prepared by a high-temperature solid-phase reaction process. The effect of Ni²⁺ doping content on the infrared radiation properties of MgCr₂O₄ materials was investigated, and the mechanism of emissivity enhancement of MgCr₂O₄ materials was explored. The results show that Ni²⁺ ions can be doped into the lattice of MgCr₂O₄ materials, and the prepared Mg_1-xNi_xCr₂O₄ (0.1≤x≤0.5) materials produce the lattice distortion and a small amount of Ni²⁺ valence state transformation. Also, the concentration of oxygen vacancies increases, the forbidden band width decreases with the increase of Ni²+doping, thus improving the emissivity of the prepared materials in the near-mid-infrared band. The material with x of 0.5 (Mg_0.5Ni_0.5Cr₂O₄) has an average emissivity of 0.88 in the near infrared ref bands (i.e., 0.8-2.5 μm), which is 167% greater than that of the undoped specimens. Ni²⁺ ions doping enhances the lattice vibration absorption, free carrier absorption and impurity energy level absorption, and improves the infrared emissivity of MgCr₂O₄ materials in the near-mid-infrared band.

, authors=Guangyang WANG, Shaobai SANG, Qinghu WANG, Qi WU, Yiran SUN, authorsList=Guangyang WANG, Shaobai SANG, Qinghu WANG, Qi WU, Yiran SUN, authorCompany=null, correspAuthors=Shaobai SANG, Qinghu WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222571829150241, articleId=1319222571392942623, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=Ni²⁺掺杂对MgCr₂O₄材料红外辐射性能的影响, columnId=1321891096976798674, journalTitle=硅酸盐学报, columnName=耐火材料相关基础研究进展专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

开发高发射率红外辐射材料是高温窑炉节能的重要方向。本工作采用高温固相反应工艺制备Ni²⁺掺杂MgCr₂O₄材料，研究了Ni²⁺掺杂量摩尔分数对MgCr₂O₄材料红外辐射性能的影响，探讨了影响MgCr₂O₄材料红外发射率的机理。结果表明，Ni²⁺能掺杂进入MgCr₂O₄材料晶格，所制备的Mg_1-xNi_xCr₂O₄（0.1≤x≤0.5）材料产生了晶格畸变，少量Ni²⁺价态发生转变；同时，随着Ni²⁺掺杂量增加，氧空位浓度的增大，禁带宽度减小，所制备材料在近中红外波段的发射率均有提高。x=0.5的材料（Mg_0.5Ni_0.5Cr₂O₄）在近红外波段（0.8~2.5 μm）的平均发射率达到0.88，较未掺杂样品提升了167%。Ni²⁺掺杂强化了晶格振动吸收、自由载流子吸收和杂质能级吸收，提升了MgCr₂O₄材料在近中红外波段的红外发射率。

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WANG Guangyang (1996-), male, Doctorial candidate. E-mail: 1134179751@qq.com

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WANG Guangyang (1996-), male, Doctorial candidate. E-mail: 1134179751@qq.com

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王光阳（1996—），男，博士研究生。

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王光阳（1996—），男，博士研究生。

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