Article(id=1319222295466455241, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220643, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1659801600000, receivedDateStr=2022-08-07, revisedDate=1663776000000, revisedDateStr=2022-09-22, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456705204, onlineDateStr=2026-10-20, pubDate=1674144000000, pubDateStr=2023-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456705204, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456705204, creator=13701087609, updateTime=1792456705204, updator=13701087609, issue=Issue{id=1319222240177144549, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='1', pageStart='1', pageEnd='282', issueExtLink='null', onlineDate='null', pubDate='1674144000000', pubDateStr='2023-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456692021, creator='13701087609', updateTime=1792456863865, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319222960989262349, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319222960989262350, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=260, endPage=269, ext={EN=ArticleExt(id=1319222295680364746, articleId=1319222295466455241, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Progress on Negative/Zero Thermal Expansion Properties of Mn-Based Antiperovskite Compounds, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

Nearly zero thermal expansion (NZTE) materials have a high dimensional stability with a less possibility producing thermal stress under variable-temperature environment. Therefore, they can be used in aerospace, microelectronics, optics, precision devices and other fields. Mn-based antiperovskite compounds Mn₃AX (A=metal or semiconductor element, X=N or C) have attracted recent attention due to their negative or nearly zero thermal expansion (NTE/NZTE) properties within a wide temperature range, isotropy and easy regulation. Mn₃AX compounds exhibit rich magnetic structures, and their NTE/NZTE properties are closely related to the magnetic phase transitions and intense lattice-spin correlation. The magnetic structure and magnetic phase transition can be changed via optimizing the composition, thus effectively regulating the thermal expansion behavior and obtaining other functional properties. The existing methods to obtain the wide temperature range NTE/NZTE properties mainly include the broadening of the NTE behavior in the magnetic phase transition temperature range, regulation of specific magnetic phases that critically affect negative/zero thermal expansion properties, and multi-phase composition of the materials with different thermal expansion coefficients. This review represented the experimental and theoretical studies on the regulation of abnormal thermal expansion behavior of Mn₃AX antiperovskite compounds in recent years. The effective regulation and in-depth analysis of the abnormal NTE/ZTE properties of Mn-based antiperovskite compounds can reveal the physical origin of the anomaly in thermal expansion, which can greatly promote the application of these materials. This review also summarized recent research progress on the regulation strategy and mechanism of the NTE/ZTE properties of Mn-based antiperovskite, and prospected the future direction in this field.

, authors=Zhijie MA¹, Ying SUN¹, Xiuliang YUAN¹, Kewen SHI², Cong WANG^{1, 2}, authorsList=Zhijie MA, Ying SUN, Xiuliang YUAN, Kewen SHI, Cong WANG, authorCompany=null, correspAuthors=Cong WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222295906857163, articleId=1319222295466455241, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=锰基反钙钛矿化合物负/零热膨胀性质的研究进展, columnId=1263922774356181565, journalTitle=硅酸盐学报, columnName=综合评述, runingTitle=null, highlight=null, articleAbstract=

近零热膨胀材料在变温环境下具有高的尺寸稳定性，不易产生热应力，可保证相关器件或构件具有高的精密性和稳定的使用寿命，因此其在航空航天、微电子、光学、精密仪器仪表等领域具有重要应用价值。锰基反钙钛矿化合物Mn₃AX（A=金属或半导体元素，X=N或C）由于具有宽温区、各向同性、易调控的负或近零热膨胀性质，近年来引起广泛关注。Mn₃AX化合物具有丰富的磁结构，此类化合物负或近零热膨胀性质与其磁相变和晶格-自旋强关联特性密切相关。因此，通过优化组分可改变其磁结构及磁相变过程，进而有效调控其热膨胀行为并获得其它功能物性。综述并评价了国内外研究者在Mn₃AX反常热膨胀行为调控方面所做的实验和理论工作。对锰基反钙钛矿化合物反常负/零热膨胀性质实验上的有效调控和机制上的深入分析，对揭示反常热膨胀的物理起源具有重要意义，能够积极推动这类材料走向应用。旨在总结目前本领域的研究进展，着重介绍了锰基反钙钛矿化合物负/零热膨胀性质的调控策略与机理研究，也对本领域未来的研究趋势进行了展望。

, authors=马之杰¹, 孙莹¹, 袁秀良¹, 史可文², 王聪^{1, 2}, authorsList=马之杰, 孙莹, 袁秀良, 史可文, 王聪, authorCompany=null, correspAuthors=王聪, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=IJeV2806VgRUt0wUT1I1eg==, magXml=WYwXWbzYKdGicvGUibH2Sg==, pdfUrl=null, pdf=sj0fTsyrbOrMt+dyiiIoTw==, pdfFileSize=719321, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=Q3/LFY1qBVuWbP5C0Z3QGw==, mapNumber=null, fund=null)}, authors=[Author(id=1322521477597999192, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319222295466455241, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=mazhijie@buaa.edu.cn, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1322521477677690970, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319222295466455241, authorId=1322521477597999192, language=EN, stringName=Zhijie MA, firstName=Zhijie, middleName=null, lastName=MA, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.School of Physics, Beihang University, Beijing 100191, China, bio={"content":"

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MA Zhijie (1996-), male, Doctoral candidate. E-mail: mazhijie@buaa.edu.cn

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马之杰（1996—），男，博士研究生。

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