Article(id=1319222250872615814, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220354, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1658160000000, receivedDateStr=2022-07-19, revisedDate=1659628800000, revisedDateStr=2022-08-05, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456694572, onlineDateStr=2026-10-20, pubDate=1674144000000, pubDateStr=2023-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456694572, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456694572, creator=13701087609, updateTime=1792456694572, updator=13701087609, issue=Issue{id=1319222240177144549, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='1', pageStart='1', pageEnd='282', issueExtLink='null', onlineDate='null', pubDate='1674144000000', pubDateStr='2023-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456692021, creator='13701087609', updateTime=1792456863865, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319222960989262349, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319222960989262350, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=49, endPage=57, ext={EN=ArticleExt(id=1319222251069748103, articleId=1319222250872615814, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=In-situ Preparation of Flexible Fern-Like Bi₂O₃/Carbon Paper Composite with Enhanced Photocatalytic Activity, columnId=1321891568328487649, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Photocatalytic Materials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

Bismuth oxide (Bi₂O₃) is an important visible-light-driven photocatalyst, which possesses an application potential in photocatalytic degradation of organic pollutants and treatment of wastewater. However, low specific surface area and rapid recombination of carriers lead to a poor photocatalytic performance of Bi₂O₃, seriously restricting its application. Besides, the particle morphology of Bi₂O₃ is also not conducive to recycling and application. In this work, a flexible Bi₂O₃/carbon paper composite photocatalyst was prepared via electrochemical deposition and subsequent in-situ oxidation to improve its photocatalytic performance and operation convenience. In the as-prepared composite photocatalysts, fern-like β-Bi₂O₃ with a hierarchical structure is grown on the carbon paper substrate. In the visible-light-driven photocatalytic degradation of phenol in water, the photocatalytic performance of Bi₂O₃/carbon paper composite can surpasses α-Bi₂O₃ powder without a hierarchical structure and precedes the β-Bi₂O₃ with a hierarchical structure. Based on the analysis of N₂ adsorption, diffuse reflection spectra, photoluminescence and reactive radical, the improved activity of Bi₂O₃/carbon paper composite is ascribed to the fern-like hierarchical structure of Bi₂O₃ and the electron capturing role of conductive carbon paper. The hierarchical structure favors the light absorption of Bi₂O₃ and its contact with reactants, while the electron capturing role of carbon paper can effectively separate the photogenerated electrons and holes in Bi₂O₃, thus promoting the utilization of carriers. In addition, the macro-size, flexibility and two-dimensional morphology of the composite also make the operation and recycling more convenient. This study provides an effective strategy for the design of flexible photocatalysts with a hierarchical structure.

, authors=Rong'an HE, Miyan HUANG, Luyao XU, Shutong SI, Jintao HE, Difa XU, authorsList=Rong'an HE, Miyan HUANG, Luyao XU, Shutong SI, Jintao HE, Difa XU, authorCompany=null, correspAuthors=null, authorNote=, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222251283657608, articleId=1319222250872615814, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=蕨草状氧化铋/碳纸柔性复合物的原位制备及其增强的光催化活性, columnId=1321891568521425634, journalTitle=硅酸盐学报, columnName=光催化材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

氧化铋（Bi₂O₃）是一种重要的可见光光催化剂，在光催化降解有机污染物、污水处理方面有较大的应用潜力。然而，Bi₂O₃比表面积较低、其光生电子与空穴复合快等缺点都导致其光催化性能较差，严重制约了其应用。同时，Bi₂O₃的粉末形态不利于回收利用，也使其应用受到较大的限制。为此，以柔性导电碳纸作基底，采用电化学沉积和后续原位氧化的方法，制备了柔性Bi₂O₃/碳纸复合光催化剂，以提高其光催化性能和操作便利性。制备的复合物中，具有蕨草状分级结构的β-Bi₂O₃牢固地长在碳纸基底上。在可见光光催化分解水中苯酚的反应中，Bi₂O₃/碳纸复合物的光催化性能不仅明显优于无分级结构的α-Bi₂O₃粉体，还优于有一定分级结构的β-Bi₂O₃。结合N₂吸附、紫外可见漫反射光谱、荧光和自由基测试等测试分析，发现Bi₂O₃/碳纸复合光催化剂的性能提升源于Bi₂O₃的分级结构和导电碳纸的电子捕获作用。分级结构有利于Bi₂O₃的光吸收和与反应物的接触，而碳纸的电荷捕获作用能有效分离Bi₂O₃的光生电子和空穴，从而共同促进光生载流子的有效利用。此外，复合光催化剂所具有的宏观尺度、柔性和二维形貌等特征也使其使用和回收变得更为方便。本研究为柔性分级结构光催化剂的设计提供了一个新的思路。

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HE Rong'an (1973-), male, Ph.D., Professor. E-mail: hslra@sina.com

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赫荣安（1973—），男，博士，教授。

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赫荣安（1973—），男，博士，教授。

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