Article(id=1318979397378495063, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318979383570837667, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230546, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1690387200000, receivedDateStr=2023-07-27, revisedDate=1691251200000, revisedDateStr=2023-08-06, acceptedDate=null, acceptedDateStr=null, onlineDate=1792398793786, onlineDateStr=2026-10-19, pubDate=1700409600000, pubDateStr=2023-11-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792398793786, onlineIssueDateStr=2026-10-19, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792398793786, creator=13701087609, updateTime=1792398793786, updator=13701087609, issue=Issue{id=1318979383570837667, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='11', pageStart='2739', pageEnd='3038', issueExtLink='null', onlineDate='null', pubDate='1700409600000', pubDateStr='2023-11-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792398790495, creator='13701087609', updateTime=1792399377667, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1318981846411629158, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318979383570837667, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1318981846411629159, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318979383570837667, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2763, endPage=2779, ext={EN=ArticleExt(id=1318979397571433048, articleId=1318979397378495063, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Influence of NaAlO₂ on Hydration and Property of Mussel Shell-Based Carbonaluminate Cementitious Materials, columnId=1321891504432460086, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Advanced Marine Materials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

Ocean is a largest carbon reservoir in the Earth, and the total production of marine shellfish in China is huge. Most of shellfish only utilizes their edible value, and shells are randomly stacked or buried as a solid waste. To improve the utilization rate of shellfish waste, the effect of NaAlO₂ on the hydration process, solid-liquid phase composition, pore structure and mechanical property of the shell powder-calcium aluminate cementitious system was investigated. The results show that NaAlO₂ enables accelerating the hydration process, shortening the setting time, and slightly improving the compactness and mechanical properties of the hardened matrix. NaAlO₂ affects the solid-liquid phase composition. Adding NaAlO₂ increases the alkalinity of the pore solution and improves the reactivity of CaCO₃, leading such a cementitious system to the formation of a stable phase (i.e., monocarboaluminate (C₄AcH₁₁)) with a reduced amount of the unstable phase (i.e., calcium aluminate hydrate (CAH₁₀)). The samples with 3.75‰ and 5.00‰ of NaAlO₂ produce 13.0% and 13.6% of C₄AcH₁₁, respectively, and no CAH₁₀ phase occurs after cured for 28 d. The crystallite size of the microcrystalline AH₃ phase grows, which compromises the cementitious property because NaAlO₂ increases the alkalinity. The excessive NaAlO₂ leads to a decreased mechanical property. Mussel shell-based carbonaluminate cementitions materials hold promise in marine civil engineering construction.

, authors=Yuantao LIU, Biqin DONG, Feng XING, Yanshuai WANG, authorsList=Yuantao LIU, Biqin DONG, Feng XING, Yanshuai WANG, authorCompany=null, correspAuthors=Yanshuai WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1318979398250910297, articleId=1318979397378495063, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=NaAlO₂对贻贝质碳铝酸盐胶凝材料水化和性能的影响, columnId=1321891504612815159, journalTitle=硅酸盐学报, columnName=先进海洋材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

海洋是地球系统中最大的碳库，我国海水贝类总产量大。大部分贝类仅利用其食用价值，贝壳作为固体废弃物随意堆放或掩埋。为提升贝类废弃物利用率，本论文研究了NaAlO₂对贝壳粉-铝酸钙胶凝体系水化进程、固液相组成、孔隙结构及力学性能的影响机理。结果表明：NaAlO₂加速水化进程，缩短凝结时间，略微提高硬化基体的密实度与力学性能。NaAlO₂显著影响固液相组成。NaAlO₂的加入提升了孔溶液的碱度，增强了CaCO₃的反应性，使胶凝体系更倾向生成稳定相单碳型水化碳铝酸钙（C₄AcH₁₁），并降低不稳定相水化铝酸一钙（CAH₁₀）的含量。养护28 d时，3.75‰、5.00‰NaAlO₂组样品分别生成13.0%与13.6%的C₄AcH₁₁，且不含CAH₁₀。但由于NaAlO₂提升了碱度，微晶AH₃相的晶粒尺寸增大、胶凝特性降低。因此，过量的NaAlO₂会导致力学性能下降。贻贝质碳铝酸盐胶凝材料在海洋土木工程建设领域具有应用前景。

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LIU Yuantao (1996-), male, Doctoral candidate. E-mail: liuyuantao2021@email.szu.edu.cn

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LIU Yuantao (1996-), male, Doctoral candidate. E-mail: liuyuantao2021@email.szu.edu.cn

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刘源涛（1996—），男，博士研究生。

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刘源涛（1996—），男，博士研究生。

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