Article(id=1318978561361425335, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318978537852359595, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230281, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1682524800000, receivedDateStr=2023-04-27, revisedDate=1685721600000, revisedDateStr=2023-06-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1792398594465, onlineDateStr=2026-10-19, pubDate=1697731200000, pubDateStr=2023-10-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792398594465, onlineIssueDateStr=2026-10-19, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792398594465, creator=13701087609, updateTime=1792398594465, updator=13701087609, issue=Issue{id=1318978537852359595, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='10', pageStart='2517', pageEnd='2738', issueExtLink='null', onlineDate='null', pubDate='1697731200000', pubDateStr='2023-10-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792398588860, creator='13701087609', updateTime=1792399337892, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1318981679578993157, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318978537852359595, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1318981679578993158, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318978537852359595, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2727, endPage=2738, ext={EN=ArticleExt(id=1318978563370496954, articleId=1318978561361425335, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Research Process on Determination of Oxygen Surface Exchange Coefficient for Oxygen Electrode Materials of Reversible Solid Oxide Cells, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

Energy storage and fuel cell power generation are the most important development directions for realizing the carbon neutrality goal in China. Reversible solid oxide cells (i.e., RSOCs) are promising electrochemical energy conversion devices with a high efficiency and a low emission. The polarization resistance of oxygen electrode is large, and oxygen reduction/evolution reaction (ORR/OER) is sluggish. A lower oxygen exchange rate is considered as a main rate limiting step in reactions of RSOCs, restricting the efficiency and performance. This review summarized various techniques for characterizing the oxygen surface exchange coefficient (k), and introduced the working principle, merits and research progress of optical transmission relaxation approach. Also, this review discussed the factors like defect chemistry, surface chemistry, orientation, grain boundary/grain size and the crystallinity on the oxygen exchange kinetics and catalytic activity of oxygen electrode, and gave some advices for the future research.

, authors=Ting CHEN¹, Kui LIU¹, Guozhu ZHENG¹, Guangjun ZHANG¹, Zichen ZHUANG¹, Yihang LIN², Shaorong WANG¹, authorsList=Ting CHEN, Kui LIU, Guozhu ZHENG, Guangjun ZHANG, Zichen ZHUANG, Yihang LIN, Shaorong WANG, authorCompany=null, correspAuthors=Shaorong WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1318978563643126715, articleId=1318978561361425335, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=可逆固体氧化物电池氧电极材料氧表面交换系数测定及研究进展, columnId=1263922774356181565, journalTitle=硅酸盐学报, columnName=综合评述, runingTitle=null, highlight=null, articleAbstract=

可再生能源储能与燃料电池发电是目前中国双碳背景下最重要的发展方向。可逆固体氧化物电池（RSOCs）是极具前景的能源存储与转化装置，具有能量转化效率高、排放低等优点。通常氧电极（正极）材料的极化阻抗大、氧还原/氧析出反应慢，影响了RSOCs的性能，而氧表面交换系数（k）被认为是限制氧还原/析出反应的最关键因素之一。本文总结了目前国内外k值测定方法的种类、原理及其优缺点，并重点介绍了利用光透射弛豫方法测量k值的原理、优势及应用进展。同时分析总结了缺陷化学、表面化学、晶向、晶粒尺寸和晶界、结晶度等因素对k值以及氧电极催化活性的影响。最后对未来的研究方向提出了若干建议。

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CHEN Ting (1989-), female, Ph.D., Lecturer. E-mail: chenting@cumt.edu.cn

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CHEN Ting (1989-), female, Ph.D., Lecturer. E-mail: chenting@cumt.edu.cn

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陈婷（1989—），女，博士，讲师。

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陈婷（1989—），女，博士，讲师。

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