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Article(id=1318977218160742902, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318977205884014990, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230476, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1688572800000, receivedDateStr=2023-07-06, revisedDate=1690473600000, revisedDateStr=2023-07-28, acceptedDate=null, acceptedDateStr=null, onlineDate=1792398274221, onlineDateStr=2026-10-19, pubDate=1694534400000, pubDateStr=2023-09-13, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792398274221, onlineIssueDateStr=2026-10-19, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792398274221, creator=13701087609, updateTime=1792398274221, updator=13701087609, issue=Issue{id=1318977205884014990, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='12', pageStart='3039', pageEnd='3250', issueExtLink='null', onlineDate='null', pubDate='1703001600000', pubDateStr='2023-12-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792398271294, creator='13701087609', updateTime=1792399409679, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1318981980671295626, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318977205884014990, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1318981980671295627, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318977205884014990, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=3133, endPage=3143, ext={EN=ArticleExt(id=1318977218349486583, articleId=1318977218160742902, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Thermal, Mechanical and Molten Silicate Environmental Deposits Corrosion Resistance Properties of High-Entropy (Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4 Ceramic Materials, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

Novel high-temperature thermal barrier materials become the key materials for the development of new generation aeroengines. In this paper, a monoclinic high-entropy rare-earth tantalate material (Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4[(5RE0.2)TaO4] was synthesized via solid-state reaction. The thermal, the mechanical and the molten silicate environmental deposits (CMAS) corrosion resistance were investigated. The results indicate that (5RE0.2)TaO4 exhibits a low thermal conductivity (i.e., 1.22 W·m-1·K-1, 600 ℃) and a high thermal expansion coefficient (i.e., 10.3×10-6 K-1, 1 200 ℃), Compared with YSZ material (i.e., 2.1-2.7 W·m-1·K-1, 100-900 ℃), the thermal conductivity is decreased by 42%. The fracture toughness reaches 2.8 MPa·m1/2, which is superior to most thermal barrier coating materials because of its unique ferroelastic toughening effect. The thickness and penetration depth of the (5RE0.2)TaO4 reaction layer are smaller than those of the YSZ material after being corroded by CMAS at 1 350 ℃ for different durations. This material is a developed thermal barrier coating material with a great application potential.

, authors=Ruida WANG1, 2, Shixian ZHAO2, Lei LI3, Liugang CHEN1, Yaochen SI2, Lingfeng LI2, Hongxia LI2, 3, Jing FENG4, authorsList=Ruida WANG, Shixian ZHAO, Lei LI, Liugang CHEN, Yaochen SI, Lingfeng LI, Hongxia LI, Jing FENG, authorCompany=null, correspAuthors=Shixian ZHAO, Liugang CHEN, authorNote=

WANG Ruida (1998-), male, Master candidate. E-mail:

, correspAuthorsNote=
ZHAO Shixian (1981-), male, Ph.D., Senior Engineer; E-mail:
CHEN Liugang (1988-), male, Ph.D., Associate Professor.
, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1318977219012186616, articleId=1318977218160742902, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=高熵(Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4陶瓷材料的热学、力学及抗熔融硅酸盐环境沉积物侵蚀性能, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

新型高温热障涂层材料已成为新一代航空发动机发展的关键材料。本工作通过固相反应法合成了一种单斜结构的高熵稀土钽酸盐材料（Y0.2Gd0.2Dy0.2Ce0.2La0.2）TaO4[（5RE0.2）TaO4]，研究了其热、力学性能及抗熔融硅酸盐环境沉积物（CMAS）侵蚀性能。结果表明：（5RE0.2）TaO4具有极低的热导率（1.22 W·m-1·K-1, 600 ℃）和较高的热膨胀系数（10.3×10-6 K-1，1 200 ℃），与YSZ材料相比（2.1~2.7 W·m-1·K-1, 100~900 ℃）热导率下降了近42%。由于独特的铁弹增韧效应，其断裂韧性达2.8 MPa·m1/2，优于多数新型热障涂层材料。1 350 ℃不同时间及CMAS侵蚀后，（5RE0.2）TaO4反应层厚度和渗透深度均显著小于YSZ材料，是一种极具应用潜力的新型热障涂层材料。

, authors=王瑞达1, 2, 赵世贤2, 李磊3, 陈留刚1, 司瑶晨2, 李凌锋2, 李红霞2, 3, 冯晶4, authorsList=王瑞达, 赵世贤, 李磊, 陈留刚, 司瑶晨, 李凌锋, 李红霞, 冯晶, authorCompany=null, correspAuthors=赵世贤, 陈留刚, authorNote=

王瑞达（1998—），男，硕士研究生。

, correspAuthorsNote=
赵世贤（1981—），男，博士，高级工程师；
陈留刚（1988—），男，博士，副教授。
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WANG Ruida (1998-), male, Master candidate. E-mail:

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WANG Ruida (1998-), male, Master candidate. E-mail:

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王瑞达（1998—），男，硕士研究生。

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高熵(Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4陶瓷材料的热学、力学及抗熔融硅酸盐环境沉积物侵蚀性能
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王瑞达 1, 2 , 赵世贤 2 , 李磊 3 , 陈留刚 1 , 司瑶晨 2 , 李凌锋 2 , 李红霞 2, 3 , 冯晶 4
硅酸盐学报 | 研究论文 2023,51(12): 3133-3143
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硅酸盐学报 |研究论文 2023 , 51 (12) : 3133 -3143
高熵(Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4陶瓷材料的热学、力学及抗熔融硅酸盐环境沉积物侵蚀性能
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王瑞达1, 2 , 赵世贤2 , 李磊3, 陈留刚1 , 司瑶晨2, 李凌锋2, 李红霞2, 3, 冯晶4
作者信息
  • 1．郑州大学材料科学与工程学院河南省高温功能材料重点实验室，郑州 10459
  • 2．中钢集团洛阳耐火材料研究院有限公司先进耐火材料国家重点实验室，河南 洛阳 471039
  • 3．中国中钢集团有限公司，北京 100080
  • 4．昆明理工大学材料科学与工程学院，昆明 650000
通讯作者:
赵世贤（1981—），男，博士，高级工程师；
陈留刚（1988—），男，博士，副教授。
作者简介:

王瑞达（1998—），男，硕士研究生。

Thermal, Mechanical and Molten Silicate Environmental Deposits Corrosion Resistance Properties of High-Entropy (Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4 Ceramic Materials
Ruida WANG1, 2 , Shixian ZHAO2 , Lei LI3, Liugang CHEN1 , Yaochen SI2, Lingfeng LI2, Hongxia LI2, 3, Jing FENG4
Affiliations
  • 1.Henan Key Laboratory of High Temperature Functional Materials, School of Zhengzhou University Materials Science and Engineering, Zhengzhou University, Zhengzhou 10459, China
  • 2.State Key Laboratory of Advanced Refractories, Sinosteel Luoyang Institute of Refractories Research Co., Ltd., Luoyang 471039, Henan, China
  • 3.China Sinosteel Group Co., Ltd., Beijing 100080, China
  • 4.School of Materials Science and Engineering, Kunming University of Science and Technology, Kunming 650000, China
    • Corresponding Author:
    ZHAO Shixian (1981-), male, Ph.D., Senior Engineer; E-mail:
    CHEN Liugang (1988-), male, Ph.D., Associate Professor.

    WANG Ruida (1998-), male, Master candidate. E-mail:

出版时间: 2023-09-13 doi: 10.14062/j.issn.0454-5648.20230476
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新型高温热障涂层材料已成为新一代航空发动机发展的关键材料。本工作通过固相反应法合成了一种单斜结构的高熵稀土钽酸盐材料（Y0.2Gd0.2Dy0.2Ce0.2La0.2）TaO4[（5RE0.2）TaO4]，研究了其热、力学性能及抗熔融硅酸盐环境沉积物（CMAS）侵蚀性能。结果表明：（5RE0.2）TaO4具有极低的热导率（1.22 W·m-1·K-1, 600 ℃）和较高的热膨胀系数（10.3×10-6 K-1，1 200 ℃），与YSZ材料相比（2.1~2.7 W·m-1·K-1, 100~900 ℃）热导率下降了近42%。由于独特的铁弹增韧效应，其断裂韧性达2.8 MPa·m1/2，优于多数新型热障涂层材料。1 350 ℃不同时间及CMAS侵蚀后，（5RE0.2）TaO4反应层厚度和渗透深度均显著小于YSZ材料，是一种极具应用潜力的新型热障涂层材料。

稀土钽酸盐  /  高熵陶瓷  /  熔融硅酸盐环境沉积物侵蚀  /  热障涂层

Novel high-temperature thermal barrier materials become the key materials for the development of new generation aeroengines. In this paper, a monoclinic high-entropy rare-earth tantalate material (Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4[(5RE0.2)TaO4] was synthesized via solid-state reaction. The thermal, the mechanical and the molten silicate environmental deposits (CMAS) corrosion resistance were investigated. The results indicate that (5RE0.2)TaO4 exhibits a low thermal conductivity (i.e., 1.22 W·m-1·K-1, 600 ℃) and a high thermal expansion coefficient (i.e., 10.3×10-6 K-1, 1 200 ℃), Compared with YSZ material (i.e., 2.1-2.7 W·m-1·K-1, 100-900 ℃), the thermal conductivity is decreased by 42%. The fracture toughness reaches 2.8 MPa·m1/2, which is superior to most thermal barrier coating materials because of its unique ferroelastic toughening effect. The thickness and penetration depth of the (5RE0.2)TaO4 reaction layer are smaller than those of the YSZ material after being corroded by CMAS at 1 350 ℃ for different durations. This material is a developed thermal barrier coating material with a great application potential.

rare earth tantalate  /  high entropy ceramics  /  molten silicate environmental deposits corrosion resistance properties  /  thermal barrier coating
王瑞达, 赵世贤, 李磊, 陈留刚, 司瑶晨, 李凌锋, 李红霞, 冯晶. 高熵(Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4陶瓷材料的热学、力学及抗熔融硅酸盐环境沉积物侵蚀性能. 硅酸盐学报, 2023 , 51 (12) : 3133 -3143 . DOI: 10.14062/j.issn.0454-5648.20230476
Ruida WANG, Shixian ZHAO, Lei LI, Liugang CHEN, Yaochen SI, Lingfeng LI, Hongxia LI, Jing FENG. Thermal, Mechanical and Molten Silicate Environmental Deposits Corrosion Resistance Properties of High-Entropy (Y0.2Gd0.2Dy0.2Ce0.2La0.2)TaO4 Ceramic Materials[J]. Journal of the Chinese Ceramic Society, 2023 , 51 (12) : 3133 -3143 . DOI: 10.14062/j.issn.0454-5648.20230476
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  • 河南省中央引导地方科技发展资金项目(Z20221343008)
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doi: 10.14062/j.issn.0454-5648.20230476
  • 接收时间：2023-07-06
  • 首发时间：2026-10-19
  • 出版时间：2023-09-13
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  • 收稿日期：2023-07-06
  • 修回日期：2023-07-28
基金
河南省中央引导地方科技发展资金项目(Z20221343008)
作者信息
    1．郑州大学材料科学与工程学院河南省高温功能材料重点实验室，郑州 10459
    2．中钢集团洛阳耐火材料研究院有限公司先进耐火材料国家重点实验室，河南 洛阳 471039
    3．中国中钢集团有限公司，北京 100080
    4．昆明理工大学材料科学与工程学院，昆明 650000

通讯作者:

赵世贤（1981—），男，博士，高级工程师；
陈留刚（1988—），男，博士，副教授。
参考文献
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2种不同金属材料的力学参数
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Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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