Article(id=1318976919153005350, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230102, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1675612800000, receivedDateStr=2023-02-06, revisedDate=1680451200000, revisedDateStr=2023-04-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1792398202931, onlineDateStr=2026-10-19, pubDate=1695139200000, pubDateStr=2023-09-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792398202931, onlineIssueDateStr=2026-10-19, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792398202931, creator=13701087609, updateTime=1792398202931, updator=13701087609, issue=Issue{id=1318976874252980746, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='9', pageStart='2119', pageEnd='2516', issueExtLink='null', onlineDate='null', pubDate='1695139200000', pubDateStr='2023-09-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792398192226, creator='13701087609', updateTime=1792399292764, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1318981490315210817, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1318981490315210818, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2206, endPage=2213, ext={EN=ArticleExt(id=1318976919421440807, articleId=1318976919153005350, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Interference Mechanism of H₂S on CO₂ Adsorption of Aluminum-Based Solid Amine Adsorbent, columnId=1321890837848511157, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Innovation of Inorganic Non-Metallic Materials and Technologies to Support "Dual-Carbon" Goal—Research Articles, runingTitle=null, highlight=null, articleAbstract=

The interference mechanism of H₂S impurity on the CO₂ adsorption performance of solid amine adsorbents is still lack of comprehensive research. An aluminum-based solid amine adsorbent (PEI@Al₂O₃) was prepared with Al₂O₃ as a support to load polyethyleneimine (PEI), and the influence of H₂S on the CO₂ adsorption capacity, adsorption rate and cyclic adsorption performance of the adsorbent was investigated. The results show that the competitive adsorption occurs when H₂S and CO₂ coexist due to H₂S and CO₂ simultaneously grabbed the active sites of amine groups on the adsorbent. However, the adsorption competitiveness of CO₂ is larger than that of H₂S under the simulated biogas condition (i.e., 40% CO₂+59.5% CH₄+0.5% H₂S), thus inhibiting H₂S adsorption. Furthermore, the optimal adsorption temperature of CO₂ and H₂S is inconsistent, and the CO₂ adsorption capacity and cyclic stability of PEI@Al₂O₃ are not disturbed by H₂S at the optimal adsorption temperature of CO₂.

, authors=Xuehua SHEN^{1, 2}, Feng YAN^{1, 2}, Pengju WANG¹, Feng XIE¹, Xin SUN¹, Heijin CHEN¹, Zuotai ZHANG^{1, 2}, authorsList=Xuehua SHEN, Feng YAN, Pengju WANG, Feng XIE, Xin SUN, Heijin CHEN, Zuotai ZHANG, authorCompany=null, correspAuthors=Zuotai ZHANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1318976919740207912, articleId=1318976919153005350, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=H₂S对铝基固态胺吸附剂吸附CO₂性能的干扰机制, columnId=1321890840360899254, journalTitle=硅酸盐学报, columnName=无机非金属材料及技术创新助力实现双碳目标专刊—研究论文, runingTitle=null, highlight=null, articleAbstract=

H₂S杂质对固态胺吸附剂吸附CO₂性能的干扰机制还缺少全面研究。以Al₂O₃为载体负载聚乙烯亚胺（PEI）制备铝基固态胺吸附剂（PEI@Al₂O₃），系统探究了H₂S对其CO₂吸附容量、吸附速率和循环吸附性能的影响规律。结果表明：H₂S与CO₂共存时，会相互抢占吸附剂上的胺基活性位点，从而发生竞争性吸附，但在模拟沼气条件（40% CO₂+59.5% CH₄+0.5% H₂S）下，H₂S的吸附竞争力远小于CO₂，H₂S吸附被抑制，且二者的最佳吸附温度不一致，在CO₂最佳吸附温度下，PEI@Al₂O₃的CO₂吸附容量和循环稳定性均不受H₂S干扰。

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SHEN Xuehua (1992-), male, Ph.D., Associate Researcher. E-mail: shenxh@sustech.edu.cn

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