Article(id=1318976904854618128, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230286, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1682784000000, receivedDateStr=2023-04-30, revisedDate=1684512000000, revisedDateStr=2023-05-20, acceptedDate=null, acceptedDateStr=null, onlineDate=1792398199523, onlineDateStr=2026-10-19, pubDate=1695139200000, pubDateStr=2023-09-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792398199523, onlineIssueDateStr=2026-10-19, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792398199523, creator=13701087609, updateTime=1792398199523, updator=13701087609, issue=Issue{id=1318976874252980746, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='9', pageStart='2119', pageEnd='2516', issueExtLink='null', onlineDate='null', pubDate='1695139200000', pubDateStr='2023-09-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792398192226, creator='13701087609', updateTime=1792399292764, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1318981490315210817, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1318981490315210818, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2138, endPage=2152, ext={EN=ArticleExt(id=1318976908365250577, articleId=1318976904854618128, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Effect of CLDH on Microstructure and Properties of Slag-Based Geopolymer, columnId=1321890837848511157, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Innovation of Inorganic Non-Metallic Materials and Technologies to Support "Dual-Carbon" Goal—Research Articles, runingTitle=null, highlight=null, articleAbstract=

Geopolymer has attracted attention for the process features of energy saving, reduced carbon emissions and excellent properties. In this paper, we proposed a concept of phase engineering for geopolymer, and demonstrated the utilization of calcined layered double hydroxides (CLDHs). The effects of microstructure and property in slag-based geopolymer were analyzed. The rehydration reaction and nucleation mechanism of CLDH were revealed by high-energy X-ray synchrotron radiation, pair distribution function calculation, transmission electron microscopy and other characterization techniques, thus improving the short-distance order of the gel and the crystal-to-binder ratio. For the macroscopic properties, the mechanical strength and water retention of geopolymer with CLDH are improved, and the chemical shrinkage and dry shrinkage of geopolymer are decreased. Incorporation of CLDH as a technical approach to improve the microstructure of geopolymer can remedy the performance defects of geopolymer, and is thus an effective approach for manufacturing high-performance geopolymer products.

, authors=Zhengning ZHOU¹, Zuhua ZHANG^{1, 2}, Yulin DENG¹, Jie HU³, Qijun YU³, Caijun SHI¹, authorsList=Zhengning ZHOU, Zuhua ZHANG, Yulin DENG, Jie HU, Qijun YU, Caijun SHI, authorCompany=null, correspAuthors=Zuhua ZHANG, Caijun SHI, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1318976908746932242, articleId=1318976904854618128, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=CLDH对矿渣基地聚合物微观结构和性能的影响, columnId=1321890840360899254, journalTitle=硅酸盐学报, columnName=无机非金属材料及技术创新助力实现双碳目标专刊—研究论文, runingTitle=null, highlight=null, articleAbstract=

地聚合物因其节能减排、性能优异而广受关注。本工作提出了地聚合物相调控的概念，并在矿渣基地聚合物体系中，使用煅烧层状双氢氧化物（CLDHs），研究其对微观结构和性能的影响。同步辐射高能XRD及PDF计算、TEM等表征结果揭示了CLDH的再水化反应，在微观结构上提高了晶胶比和凝胶的短程有序性。在宏观性能上，掺入CLDH的地聚合物力学性能和保水性得到提高，自收缩和干燥收缩显著降低。掺用CLDH作为改善地聚合物微观结构的一种技术方法，有助于解决地聚合物的性能缺陷问题，为制备高性能地聚合物提供了一个新思路。

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