Article(id=1318976881081307704, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230232, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1681056000000, receivedDateStr=2023-04-10, revisedDate=1682956800000, revisedDateStr=2023-05-02, acceptedDate=null, acceptedDateStr=null, onlineDate=1792398193854, onlineDateStr=2026-10-19, pubDate=1695139200000, pubDateStr=2023-09-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792398193854, onlineIssueDateStr=2026-10-19, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792398193854, creator=13701087609, updateTime=1792398193854, updator=13701087609, issue=Issue{id=1318976874252980746, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='9', pageStart='2119', pageEnd='2516', issueExtLink='null', onlineDate='null', pubDate='1695139200000', pubDateStr='2023-09-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792398192226, creator='13701087609', updateTime=1792399292764, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1318981490315210817, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1318981490315210818, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318976874252980746, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2128, endPage=2137, ext={EN=ArticleExt(id=1318976881282634297, articleId=1318976881081307704, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Design and Preparation of Ultra-High Strength CO₂ Solidified Carbonate Materials, columnId=1321890837848511157, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Innovation of Inorganic Non-Metallic Materials and Technologies to Support "Dual-Carbon" Goal—Research Articles, runingTitle=null, highlight=null, articleAbstract=

CO₂ solidified carbonate material is defined as a calcium carbonate-based composite material with a rapid strength obtained via the carbonation reaction of carbonatable binders with CO₂ under normal conditions. In this paper, the mechanical properties and product composition of the CO₂ solidified carbonate materials with Fe doping, chitosan inducing and curing regime designing were investigated as γ-C₂S was used as a carbonatable binder. The results show that the enhancing strategies have a conflicting connection with one another. The Fe-γ-C₂S group with chitosan inducing (i.e., 200 MPa after 24 h curing) and the chitosan induced γ-C₂S group with long curing time (i.e., 230 MPa after 7 d curing) have a high strength. The crystalline form of calcium carbonate in γ-C₂S group is mainly aragonite, while the calcium carbonate in Fe-γ-C₂S group is calcite. The product composition of the CO₂ solidified carbonate material is another crucial factor influencing the strength. The CO₂ solidified carbonate material with an ultra-high strength has a structural feature, i.e., chitosan connects two phases (silica gel and calcium carbonate), and calcite exists inside in the calcium carbonate layer and aragonite outside. The presence of calcite can provide the strength at early curing stage, while aragonite occupies the main pore space on the outside, providing a diffusion channel for CO₂ at the later curing stage.

, authors=Sixue ZHAO^{1, 2}, Zhichao LIU^{1, 2}, Fazhou WANG¹, authorsList=Sixue ZHAO, Zhichao LIU, Fazhou WANG, authorCompany=null, correspAuthors=Fazhou WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1318976881509126714, articleId=1318976881081307704, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=超高强碳矿化材料的设计与制备, columnId=1321890840360899254, journalTitle=硅酸盐学报, columnName=无机非金属材料及技术创新助力实现双碳目标专刊—研究论文, runingTitle=null, highlight=null, articleAbstract=

碳矿化材料是由固碳胶凝材料通过与CO₂在常规环境下的碳化反应快速形成以碳酸钙为主要基体组成的复合材料，是实现工业烟气CO₂建材化利用的重要技术途径。本工作以γ-C₂S为固碳胶凝材料，研究了Fe掺杂、壳聚糖引入、养护制度设计3种复合增强措施对碳矿化材料力学性能与产物组成的影响规律。结果表明，不同的增强措施并非简单的叠加效应，也存在矛盾关系，其中，可以获得超高强度的组别有：Fe-γ-C₂S+壳聚糖引入的碳矿化材料在养护24 h后抗压强度达到200 MPa以上，壳聚糖引入组可以在延长养护时间后获得更高的强度上限，养护7 d后抗压强度可达约230 MPa。Fe-γ-C₂S组的碳酸钙晶型以方解石为主，而长期CO₂养护下的γ-C₂S组则为文石相组成。不同的产物组成也是影响强度增长的重要因素，由此提出超高强碳矿化材料的理想结构模型：壳聚糖存在于硅凝胶与碳酸钙之间，连接两相，方解石生长于内部，文石包裹于外部。方解石为碳矿化体养护早期提供强度，文石则在外侧占据了主要的孔隙空间，为后期养护过程中CO₂提供扩散通道。

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ZHAO Sixue (1993-), female, Ph.D. E-mail: zhaosixue@whut.edu.cn

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