Article(id=1318974543616660354, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318974513019207979, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20221040, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1669824000000, receivedDateStr=2022-12-01, revisedDate=1671897600000, revisedDateStr=2022-12-25, acceptedDate=null, acceptedDateStr=null, onlineDate=1792397636560, onlineDateStr=2026-10-19, pubDate=1685289600000, pubDateStr=2023-05-29, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792397636560, onlineIssueDateStr=2026-10-19, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792397636560, creator=13701087609, updateTime=1792397636560, updator=13701087609, issue=Issue{id=1318974513019207979, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='7', pageStart='1649', pageEnd='1882', issueExtLink='null', onlineDate='null', pubDate='1689782400000', pubDateStr='2023-07-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792397629265, creator='13701087609', updateTime=1792399256269, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1318981337223119779, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318974513019207979, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1318981337223119780, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1318974513019207979, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1792, endPage=1799, ext={EN=ArticleExt(id=1318974543822181251, articleId=1318974543616660354, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=SO₂ Removal Performance of Porous High-Content Iron Fly Ash Modified by NaClO, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

It is of great significance for the improvement and utilization of fly ash to reduce the accumulation pollution of coal based solid waste. In this work, a porous high-content iron fly ash sorbent named KIFA was obtained via CaO hydration, addition of pore-making agent and binder, and oxidation modification by NaClO. This sorbent KIFA with an optimized pore structure can promote the formation of K₂FeO₄. The fixed-bed evaluation results show that the KIFA has the maximum SO₂ removal ability at 700 ℃, 5% O₂ and 500 mg/m³ SO₂, and the breakthrough time and sulfur capacity of the removal efficiency of > 93% are 111.8 min and 93.58 mg/g, respectively, having the ultra-low emission standard of 35 mg/m³. According to the characterization results of fresh and used KIFA, K₂FeO₄ is a main active component in removing SO₂ by KIFA, and Fe(VI) provides the oxidation site, which oxidizes SO₂ to SO₄^2-. NO can promote the forward desulfurization reaction. NO, SO₂ and CaO can form an intermediate product of NO₃SO₃Ca, which can be converted into SO₄^2-, thus improving the removal efficiency of SO₂.

, authors=Yongjia LI, Xianrong ZHENG, Guangyuan TIAN, Xiaofeng HAO, Yuying WANG, authorsList=Yongjia LI, Xianrong ZHENG, Guangyuan TIAN, Xiaofeng HAO, Yuying WANG, authorCompany=null, correspAuthors=Xianrong ZHENG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1318974544048673668, articleId=1318974543616660354, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=NaClO改性多孔高铁粉煤灰脱除SO₂性能, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

燃煤固体废弃物粉煤灰的提质利用对缓解煤基固废堆积污染有重大意义。对高铁粉煤灰进行CaO水合、添加造孔剂和粘结剂、NaClO氧化改性，获得多孔高铁粉煤灰吸附剂KIFA，既优化了孔隙结构，又促进了K₂FeO₄的生成。固定床评价结果显示：KIFA在700 ℃、5% O₂、500 mg/m³ SO₂的条件下具有最强的脱除SO₂性能，脱除效率维持在93%以上的穿透时间和硫容分别为111.8 min和93.58 mg/g，达到了超低排放标准35 mg/m³；KIFA脱硫前后表征结果揭示：K₂FeO₄是KIFA脱除SO₂的主要活性组分，Fe（VI）提供氧化位点，将SO₂氧化为SO₄^2-；NO会促进脱硫反应正向进行，NO可与SO₂、CaO生成中间产物NO₃SO₃Ca，进而转化为SO₄^2-，提升SO₂的脱除效率。

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LI Yongjia (1997-), male, Master candidate. E-mail: liyongjia987@163.com

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李泳佳（1997—），男，硕士研究生。

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李泳佳（1997—），男，硕士研究生。

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