Article(id=1320107556542993046, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1320107530261479891, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20260118, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1772467200000, receivedDateStr=2026-03-03, revisedDate=1776614400000, revisedDateStr=2026-04-20, acceptedDate=null, acceptedDateStr=null, onlineDate=1792667767892, onlineDateStr=2026-10-22, pubDate=1780588800000, pubDateStr=2026-06-05, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792667767892, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792667767892, creator=13701087609, updateTime=1792667767892, updator=13701087609, issue=Issue{id=1320107530261479891, tenantId=1146029695717560320, journalId=1263187385517883426, year='2026', volume='54', issue='7', pageStart='2171', pageEnd='2576', issueExtLink='null', onlineDate='null', pubDate='1784476800000', pubDateStr='2026-07-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792667761625, creator='13701087609', updateTime=1792720444956, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1320328500238725499, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1320107530261479891, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1320328500238725500, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1320107530261479891, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2309, endPage=2324, ext={EN=ArticleExt(id=1320107556798845591, articleId=1320107556542993046, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Organic Functional Crystal Structure Design and Spin Effects, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=
Organic materials have attracted recent attention in spintronics due to their weak spin-orbit coupling (SOC), long spin relaxation times, and highly designable molecular/crystal structures. Compared with inorganic systems, spin behaviors in organic materials are more sensitive to microstructures and chemical environments, making it feasible to regulate spin effects through structural design.
This review represents the rules and strategies by which structural design in organic functional crystals tunes spin effects. From the perspective of spin dynamics, SOC, exchange interaction, and hyperfine interaction (HFI) jointly determine the characteristics of spin relaxation in organic systems, while their relative importance varies with structural order, carrier density, and transport pathways. In this context, experimental phenomena such as organic magnetic-field effects, spin transport, and organic magnetism can be regarded as collective manifestations of multiple microscopic interactions under specific structural and device conditions rather than direct reflections of a single mechanism. Tailoring interaction strengths and their modes of action via structural design thus constitutes an effective route for regulating spin effects.
Regarding crystal-structure regulation, this review summarizes the effects of crystallinity and crystal parameters on the spin behaviors. Improving crystal order can enhance carrier transport, reduce disorder-induced scattering and local random fields, thereby providing more stable channels for spin transmission. Meanwhile, molecular packing motifs, intermolecular interactions, and molecular curvature are also key factors affecting spin relaxation. Structural isomers, by introducing well-defined conformational differences, offer clean comparative platforms for clarifying how subtle structural variations alter spin-related interactions, and they also inspire further molecular-level approaches for tuning spin effects.
Regarding chemical-composition regulation, this review discusses the impacts of isotope effects, atom substitution, and multicomponent systems on the spin behaviors. Isotopic substitution can modulate HFI via altering nuclear spins, serving as an important means to regulate spin decoherence. Atom substitution changes the molecular electronic structure and local environment, providing flexible pathways to tune SOC and energy-level distributions. Multicomponent systems introduce new localized states, energy-level gradients, and phase interfaces, enabling cooperative interactions that lead to more complex yet tunable spin responses. In addition, the coupling between spin and charge at magnetoelectric heterostructure interfaces can also realize electric-field modulation of spin polarization and spin transport, as well as magnetic-field and optical-field modulation of polarization, further expanding the design space for spin regulation in organic systems.
Moreover, this review represents recent progress on spin-selective effects in chiral material systems and points out that chiral structures provide a solution for controlling spin polarization that differs from conventional magnetic routes. Spin-related responses can be achieved without relying on strong SOC via constructing molecules and crystal structures with stable chiral features, offering some opportunities for developing novel spin-functional devices.
Summary and Prospects Centered on structural design of organic functional crystals and starting from the fundamentals of spin dynamics, this review represents key spin-relaxation mechanisms in organic materials, including SOC, exchange interaction, and HFI, and summarizes representative spin-related phenomena such as organic magnetic-field effects, spin transport, and organic magnetism. On this basis, this review highlights how crystal order, polymorphism, molecular packing, and conformational differences regulate spin behavior, and summarizes how isotope effects, atom substitution, and cooperative interactions in multicomponent systems affect spin effects. Meanwhile, this review introduces spin behaviors at heterojunction interfaces and the physical mechanisms of chirality-induced spin selectivity in chiral materials, together with commonly used strategies for constructing chiral structures. Effective regulation of spin effects in organic functional crystals relies on coordinated advances in structural design, chemical-composition control, and device-structure optimization. Future studies should place a greater emphasis on the quantitative characterization of structural parameters, discriminative verification of spin-relaxation mechanisms, and statistical reliability in multicomponent and interfacial systems. It is expected to realize efficient and stable organic spintronic devices via integrating molecular design, crystal engineering, interface modulation, and device-structure optimization, supporting flexible electronics and low-power information devices as well as emerging spin-functional integration.
, authors=Shilin LI, Baowen GU, Tianyu ZHANG, Wei QIN, authorsList=Shilin LI, Baowen GU, Tianyu ZHANG, Wei QIN, authorCompany=null, correspAuthors=Wei QIN, authorNote=
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有机材料由于其弱自旋轨道耦合、较长的自旋弛豫时间以及高度可设计的分子与晶体结构，近年来在自旋电子学领域受到广泛关注。与无机体系相比，有机材料中的自旋行为对微观结构和化学环境表现出更高的敏感性，使得通过结构设计实现自旋效应调控成为可能。本文围绕有机功能晶体结构设计，从自旋动力学基础出发，系统综述了有机材料中自旋轨道耦合、交换相互作用和超精细相互作用等关键自旋弛豫机制，并概述了有机磁场效应、自旋输运以及有机磁性等典型自旋相关现象。在此基础上，重点讨论了晶体有序性、分子堆积方式及晶体参数差异等结构因素对自旋行为的调控作用，进一步总结了同位素效应、化学取代以及多组分体系中相互作用协同对自旋效应的影响。同时，本文还介绍了有机异质结界面中的自旋行为以及手性材料中手性诱导的自旋选择效应的物理机制与常用手性结构的构建策略。最后，对有机功能晶体中结构设计与自旋效应之间的内在关联进行了总结，并对未来通过精细结构工程实现高效、自旋可控有机器件的发展方向进行了展望。
, authors=李世林, 顾宝文, 张天宇, 秦伟, authorsList=李世林, 顾宝文, 张天宇, 秦伟, authorCompany=null, correspAuthors=秦伟, authorNote=
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秦伟（1984—），男，博士，教授。
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LI Shilin (1999-), male, Doctoral candidate. E-mail: lishilin0322@qq.com
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LI Shilin (1999-), male, Doctoral candidate. E-mail: lishilin0322@qq.com
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李世林（1999—），男，博士研究生。
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李世林（1999—），男，博士研究生。
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