Article(id=1320107624889176516, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1320107605469544753, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20260073, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1770048000000, receivedDateStr=2026-02-03, revisedDate=1772294400000, revisedDateStr=2026-03-01, acceptedDate=null, acceptedDateStr=null, onlineDate=1792667784187, onlineDateStr=2026-10-22, pubDate=1787241600000, pubDateStr=2026-08-21, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792667784187, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792667784187, creator=13701087609, updateTime=1792667784187, updator=13701087609, issue=Issue{id=1320107605469544753, tenantId=1146029695717560320, journalId=1263187385517883426, year='2026', volume='54', issue='9', pageStart='2949', pageEnd='3314', issueExtLink='null', onlineDate='null', pubDate='1789833600000', pubDateStr='2026-09-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792667779556, creator='13701087609', updateTime=1792737576818, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1320400356446687492, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1320107605469544753, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1320400356446687493, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1320107605469544753, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=3013, endPage=3031, ext={EN=ArticleExt(id=1320107625522516421, articleId=1320107624889176516, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Full-Process Numerical Modeling for Binder Jetting of Ceramics: Current Status, Challenges and Outlook, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

Binder Jetting (BJ) additive manufacturing emerges as a promising forming process for fabricating geometrically complex ceramic components, including thin walls, internal channels, and topology-optimized features. The process achieves forming through the selective deposition of a liquid binder onto a powder bed, typically without involving a melt pool. Consequently, it is inherently compatible with high-melting-point, brittle ceramic powders and is less constrained by melt-related instabilities. Despite these advantages, achieving robust manufacturing remains challenging. Defects and variability rarely originate from an isolated processing step. They emerge from the interaction of a series of strongly coupled steps like powder spreading, binder deposition and infiltration, drying/curing and depowdering, thermal removal of organics (debinding), and sintering. Heterogeneities introduced early in the process chain are often transmitted and amplified, ultimately manifesting as non-uniform shrinkage, warpage, cracking, residual porosity, and property scatter. In this context, full-process numerical modeling is increasingly required, serving for mechanistic interpretation and for predictive process-window design.

This review consolidates recent advances on numerical modeling of ceramic Binder Jetting (BJ) and proposes an organizing principle to enhance the coherence and utility of the literature, framing the process chain through transferable state variables that quantify process inheritance. Modeling approaches are evaluated not as isolated stage-specific problems, but according to three dimensions, i.e., 1) the specific physical quantities predicted; 2) the transferability of these quantities as consistent inputs to subsequent stages; and 3) the practicality of calibrating and validating the relevant quantities through accessible experiments. Key transferable state variables highlighted include the spatial distribution of powder-bed porosity and pore-size statistics; permeability and its directional dependence; local binder saturation and organic distribution in the green body; evolving transport coefficients and gas-generation rates during debinding; and the initial relative-density and defect fields that control densification and shape evolution during sintering. Centering on these variables enables an explicit clarification of inter-stage coupling logic and charts a path toward engineering-grade predictability.

Powder spreading modeling defines the initial mesoscale structure controlling all downstream responses. The discrete element method (DEM) is widely adopted as it enables the direct representation of particle rearrangement, contact interactions, and localized compaction under blades or rollers. The existing studies demonstrate that particle size distribution, morphology, cohesion, layer thickness, and recoater kinematics jointly regulate bed density, surface roughness and structural anisotropy. For full-process simulation, key advantage of DEM converts these attributes into downstream-ready descriptors-including porosity maps, pore-network statistics and anisotropic permeability closures.

Binder deposition and infiltration determine the saturation field and organic distribution, which simultaneously control green body strength and subsequent gas evolution. At the component level, Darcy-type infiltration models remain an effective tool for rapidly exploring printing conditions. When permeability and capillary effects are expressed through measurable parameters (e.g., viscosity, surface tension, and wetting), these models can be enhanced to incorporate drying, evaporation, and curing/solidification kinetics. When pore-scale interfacial dynamics and droplet impact dominate, higher-resolution approaches are required. Interface-capturing computational fluid dynamics (CFD) and lattice Boltzmann method (LBM) simulations have been used to resolve transient interfaces and flow pathways in complex pore geometries, while coupled DEM-CFD frameworks have been introduced to capture infiltration-induced particle rearrangement in fine powders.

Debinding is typically the most failure-prone stage since gases generated by binder decomposition must vent through a pore network while the solid skeleton remains weak and thermally stressed. Consequently, predictive modeling necessitates a coupled treatment of reaction kinetics, transport and mechanical response. Decomposition kinetics is typically constrained through thermogravimetric analysis (TGA), commonly implemented with multi-step schemes that represent complex degradation pathways. Gas transport is treated through diffusion, convection, and pressure-driven Darcy flow, with permeability and effective diffusivity evolving with porosity and temperature. Coupled heat and mass transfer in actual geometries can be solved through the finite element method (FEM) implementations, with a failure risk evaluated by relating pore pressure, strength reduction, and constrained deformation.

Sintering consolidates the debound microstructure and determines densification, grain growth, and macroscopic shape change. Continuum constitutive laws embedded within FEM remain a dominant route for component-scale prediction, providing that temperature-dependent viscosities/creep parameters are calibrated and initial relative-density fields are supplied. These models are essential for predicting anisotropic shrinkage and warpage induced by inherent heterogeneity. In the microstructural scale, the Monte Carlo Potts models and phase-field approaches reveal the mechanisms of neck growth, pore evolution, grain-boundary migration, and coarsening. Despite high computational cost, they provide a basis for reduced-order kinetics and constitutive relations applicable to engineering-scale simulations, linking fundamental mechanisms to manufacturability.

A consistent thread across all stages is that predictive capability relies on effective parameter identification and validation. Accordingly, this review recommends establishing a validation matrix aligned with transferable variables. Powder spreading should be validated via bed density, surface roughness, and anisotropy metrics; infiltration via penetration depth, saturation mapping, and spatial green strength, debinding via multi-rate TGA/DTG constraints, independent characterization of pore-network evolution, and statistical measures of cracking/distortion as well as sintering via shrinkage anisotropy, warpage, final density, and defect populations. Designing validation around variables required for downstream transfer allows uncertainty to be localized and gradually reduced, thus avoiding implicit redistribution across the chain.

Summary and Prospects

Future developments in the field are likely to follow three main trajectories. First, standardized definitions and transfer rules for transferable variables are required to reduce inconsistencies among models and to support reproducible coupled workflows. Second, the integration of uncertainty-aware calibration and sensitivity analysis into process-window design is warranted as fundamental constitutive relations and kinetic parameters are constrained by measurement limitations and condition dependence. Third, integrated workflows combining high-fidelity simulation, reduced-order modeling, and data-driven surrogates are essential for fast component-scale screening and optimization. Driven by these advances, full-process modeling can evolve from retrospective interpretation toward prospective control of process-structure-property linkages in ceramic BJ, thereby improving reliability, dimensional fidelity, and performance consistency across diverse material categories.

, authors=Wei ZHAO, Linran HUANG, Kaiqi ZOU, Jiamin WU, Qingsong WEI, authorsList=Wei ZHAO, Linran HUANG, Kaiqi ZOU, Jiamin WU, Qingsong WEI, authorCompany=null, correspAuthors=Qingsong WEI, authorNote=

ZHAO Wei (1998-), male, Doctoral candidate. E-mail:

, correspAuthorsNote=
{WEI} Qingsong (1975-), male, Ph.D., Professor. E-mail:
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高性能陶瓷在高温结构、耐蚀绝缘与精密型芯等场景中的需求持续增长。黏结剂喷射(BJ)具备室温成形与高几何自由度优势,但铺粉-喷射-脱脂-烧结的跨尺度耦合使陶瓷零件易发生难以预测的缺陷。本文面向陶瓷材料BJ成形过程,凝练全过程数值模拟进展:离散元法(DEM)量化层厚、粒径级配与刮刀/辊筒运动对孔隙率与表面粗糙度的影响;计算流体力学/流体体积法(CFD/VOF)、格子玻尔兹曼方法(LBM)及DEM-CFD耦合描述液滴冲击、毛细渗透与干燥固化过程黏结剂与粉床的作用机制;脱脂阶段汇总热重分析(TGA)驱动的多步动力学、扩散-对流-达西输运、相场网络运输与热-质-力有限元模型,建立残余黏结剂、空隙变化与裂纹风险的预测框架;烧结部分对比连续体本构、Monte Carlo与相场方法在颈部长大、致密化、晶粒演化及各向异性收缩中的适用性。文末归纳参数定义与实验验证方法,提出跨尺度耦合与数据闭环驱动的陶瓷BJ过程建模方向。

, authors=赵威, 黄琳然, 邹凯琦, 吴甲民, 魏青松, authorsList=赵威, 黄琳然, 邹凯琦, 吴甲民, 魏青松, authorCompany=null, correspAuthors=魏青松, authorNote=

赵威(1998—),男,博士研究生。

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魏青松(1975—),男,博士,教授。
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黏结剂喷射增材制造陶瓷全过程数值模拟:现状、挑战与展望
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赵威 , 黄琳然 , 邹凯琦 , 吴甲民 , 魏青松
硅酸盐学报 | 综合评述 2026,54(9): 3013-3031
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硅酸盐学报 |综合评述 2026 , 54 (9) : 3013 -3031
黏结剂喷射增材制造陶瓷全过程数值模拟:现状、挑战与展望
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赵威 , 黄琳然, 邹凯琦, 吴甲民, 魏青松
作者信息
  • 华中科技大学材料科学与工程学院,武汉 430074
通讯作者:
魏青松(1975—),男,博士,教授。
作者简介:

赵威(1998—),男,博士研究生。

Full-Process Numerical Modeling for Binder Jetting of Ceramics: Current Status, Challenges and Outlook
Wei ZHAO , Linran HUANG, Kaiqi ZOU, Jiamin WU, Qingsong WEI
Affiliations
  • School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
  • Corresponding Author:
    {WEI} Qingsong (1975-), male, Ph.D., Professor. E-mail:

    ZHAO Wei (1998-), male, Doctoral candidate. E-mail:

出版时间: 2026-08-21 doi: 10.14062/j.issn.0454-5648.20260073
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高性能陶瓷在高温结构、耐蚀绝缘与精密型芯等场景中的需求持续增长。黏结剂喷射(BJ)具备室温成形与高几何自由度优势,但铺粉-喷射-脱脂-烧结的跨尺度耦合使陶瓷零件易发生难以预测的缺陷。本文面向陶瓷材料BJ成形过程,凝练全过程数值模拟进展:离散元法(DEM)量化层厚、粒径级配与刮刀/辊筒运动对孔隙率与表面粗糙度的影响;计算流体力学/流体体积法(CFD/VOF)、格子玻尔兹曼方法(LBM)及DEM-CFD耦合描述液滴冲击、毛细渗透与干燥固化过程黏结剂与粉床的作用机制;脱脂阶段汇总热重分析(TGA)驱动的多步动力学、扩散-对流-达西输运、相场网络运输与热-质-力有限元模型,建立残余黏结剂、空隙变化与裂纹风险的预测框架;烧结部分对比连续体本构、Monte Carlo与相场方法在颈部长大、致密化、晶粒演化及各向异性收缩中的适用性。文末归纳参数定义与实验验证方法,提出跨尺度耦合与数据闭环驱动的陶瓷BJ过程建模方向。

增材制造  /  黏结剂喷射  /  多尺度模拟  /  性能预测

Binder Jetting (BJ) additive manufacturing emerges as a promising forming process for fabricating geometrically complex ceramic components, including thin walls, internal channels, and topology-optimized features. The process achieves forming through the selective deposition of a liquid binder onto a powder bed, typically without involving a melt pool. Consequently, it is inherently compatible with high-melting-point, brittle ceramic powders and is less constrained by melt-related instabilities. Despite these advantages, achieving robust manufacturing remains challenging. Defects and variability rarely originate from an isolated processing step. They emerge from the interaction of a series of strongly coupled steps like powder spreading, binder deposition and infiltration, drying/curing and depowdering, thermal removal of organics (debinding), and sintering. Heterogeneities introduced early in the process chain are often transmitted and amplified, ultimately manifesting as non-uniform shrinkage, warpage, cracking, residual porosity, and property scatter. In this context, full-process numerical modeling is increasingly required, serving for mechanistic interpretation and for predictive process-window design.

This review consolidates recent advances on numerical modeling of ceramic Binder Jetting (BJ) and proposes an organizing principle to enhance the coherence and utility of the literature, framing the process chain through transferable state variables that quantify process inheritance. Modeling approaches are evaluated not as isolated stage-specific problems, but according to three dimensions, i.e., 1) the specific physical quantities predicted; 2) the transferability of these quantities as consistent inputs to subsequent stages; and 3) the practicality of calibrating and validating the relevant quantities through accessible experiments. Key transferable state variables highlighted include the spatial distribution of powder-bed porosity and pore-size statistics; permeability and its directional dependence; local binder saturation and organic distribution in the green body; evolving transport coefficients and gas-generation rates during debinding; and the initial relative-density and defect fields that control densification and shape evolution during sintering. Centering on these variables enables an explicit clarification of inter-stage coupling logic and charts a path toward engineering-grade predictability.

Powder spreading modeling defines the initial mesoscale structure controlling all downstream responses. The discrete element method (DEM) is widely adopted as it enables the direct representation of particle rearrangement, contact interactions, and localized compaction under blades or rollers. The existing studies demonstrate that particle size distribution, morphology, cohesion, layer thickness, and recoater kinematics jointly regulate bed density, surface roughness and structural anisotropy. For full-process simulation, key advantage of DEM converts these attributes into downstream-ready descriptors-including porosity maps, pore-network statistics and anisotropic permeability closures.

Binder deposition and infiltration determine the saturation field and organic distribution, which simultaneously control green body strength and subsequent gas evolution. At the component level, Darcy-type infiltration models remain an effective tool for rapidly exploring printing conditions. When permeability and capillary effects are expressed through measurable parameters (e.g., viscosity, surface tension, and wetting), these models can be enhanced to incorporate drying, evaporation, and curing/solidification kinetics. When pore-scale interfacial dynamics and droplet impact dominate, higher-resolution approaches are required. Interface-capturing computational fluid dynamics (CFD) and lattice Boltzmann method (LBM) simulations have been used to resolve transient interfaces and flow pathways in complex pore geometries, while coupled DEM-CFD frameworks have been introduced to capture infiltration-induced particle rearrangement in fine powders.

Debinding is typically the most failure-prone stage since gases generated by binder decomposition must vent through a pore network while the solid skeleton remains weak and thermally stressed. Consequently, predictive modeling necessitates a coupled treatment of reaction kinetics, transport and mechanical response. Decomposition kinetics is typically constrained through thermogravimetric analysis (TGA), commonly implemented with multi-step schemes that represent complex degradation pathways. Gas transport is treated through diffusion, convection, and pressure-driven Darcy flow, with permeability and effective diffusivity evolving with porosity and temperature. Coupled heat and mass transfer in actual geometries can be solved through the finite element method (FEM) implementations, with a failure risk evaluated by relating pore pressure, strength reduction, and constrained deformation.

Sintering consolidates the debound microstructure and determines densification, grain growth, and macroscopic shape change. Continuum constitutive laws embedded within FEM remain a dominant route for component-scale prediction, providing that temperature-dependent viscosities/creep parameters are calibrated and initial relative-density fields are supplied. These models are essential for predicting anisotropic shrinkage and warpage induced by inherent heterogeneity. In the microstructural scale, the Monte Carlo Potts models and phase-field approaches reveal the mechanisms of neck growth, pore evolution, grain-boundary migration, and coarsening. Despite high computational cost, they provide a basis for reduced-order kinetics and constitutive relations applicable to engineering-scale simulations, linking fundamental mechanisms to manufacturability.

A consistent thread across all stages is that predictive capability relies on effective parameter identification and validation. Accordingly, this review recommends establishing a validation matrix aligned with transferable variables. Powder spreading should be validated via bed density, surface roughness, and anisotropy metrics; infiltration via penetration depth, saturation mapping, and spatial green strength, debinding via multi-rate TGA/DTG constraints, independent characterization of pore-network evolution, and statistical measures of cracking/distortion as well as sintering via shrinkage anisotropy, warpage, final density, and defect populations. Designing validation around variables required for downstream transfer allows uncertainty to be localized and gradually reduced, thus avoiding implicit redistribution across the chain.

Summary and Prospects

Future developments in the field are likely to follow three main trajectories. First, standardized definitions and transfer rules for transferable variables are required to reduce inconsistencies among models and to support reproducible coupled workflows. Second, the integration of uncertainty-aware calibration and sensitivity analysis into process-window design is warranted as fundamental constitutive relations and kinetic parameters are constrained by measurement limitations and condition dependence. Third, integrated workflows combining high-fidelity simulation, reduced-order modeling, and data-driven surrogates are essential for fast component-scale screening and optimization. Driven by these advances, full-process modeling can evolve from retrospective interpretation toward prospective control of process-structure-property linkages in ceramic BJ, thereby improving reliability, dimensional fidelity, and performance consistency across diverse material categories.

additive manufacturing  /  binder jetting  /  multiscale simulation  /  performance prediction
赵威, 黄琳然, 邹凯琦, 吴甲民, 魏青松. 黏结剂喷射增材制造陶瓷全过程数值模拟:现状、挑战与展望. 硅酸盐学报, 2026 , 54 (9) : 3013 -3031 . DOI: 10.14062/j.issn.0454-5648.20260073
Wei ZHAO, Linran HUANG, Kaiqi ZOU, Jiamin WU, Qingsong WEI. Full-Process Numerical Modeling for Binder Jetting of Ceramics: Current Status, Challenges and Outlook[J]. Journal of the Chinese Ceramic Society, 2026 , 54 (9) : 3013 -3031 . DOI: 10.14062/j.issn.0454-5648.20260073
  • 国防基础科研项目(JCKY2022213C008)
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doi: 10.14062/j.issn.0454-5648.20260073
  • 接收时间:2026-02-03
  • 首发时间:2026-10-22
  • 出版时间:2026-08-21
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  • 收稿日期:2026-02-03
  • 修回日期:2026-03-01
基金
国防基础科研项目(JCKY2022213C008)
作者信息
    华中科技大学材料科学与工程学院,武汉 430074

通讯作者:

魏青松(1975—),男,博士,教授。
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2种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
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占总种数比例
Percentage of
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属
Genus
种数
Number of
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占总种数比例
Percentage of total
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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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