Article(id=1319726494553846783, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319726382268138030, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20250111, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1739980800000, receivedDateStr=2025-02-20, revisedDate=1743782400000, revisedDateStr=2025-04-05, acceptedDate=null, acceptedDateStr=null, onlineDate=1792576915634, onlineDateStr=2026-10-21, pubDate=1763568000000, pubDateStr=2025-11-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792576915634, onlineIssueDateStr=2026-10-21, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792576915634, creator=13701087609, updateTime=1792576915634, updator=13701087609, issue=Issue{id=1319726382268138030, tenantId=1146029695717560320, journalId=1263187385517883426, year='2025', volume='53', issue='11', pageStart='3079', pageEnd='3432', issueExtLink='null', onlineDate='null', pubDate='1763568000000', pubDateStr='2025-11-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792576888863, creator='13701087609', updateTime=1792577494231, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319728921399116056, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319726382268138030, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319728921403310361, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319726382268138030, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=3404, endPage=3419, ext={EN=ArticleExt(id=1319726494750979072, articleId=1319726494553846783, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Application and Research Progress of Nanotechnology in Air Electrode for Low-Temperature Reversible Solid Oxide Cells, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

Reversible solid oxide cells (RSOCs) are electrochemical devices that can convert energy between chemical and electrical ones, which have attracted widespread attention due to their high energy conversion efficiency, low emissions, and lack of requirement for precious metals. They can be integrated with renewable energy systems to store excess electrical energy during periods of low demand (valleys) and efficiently release it during periods of high demand (peaks), demonstrating great potential for promoting the effective utilization of renewable energy and the achievement of the dual-carbon goals. The RSOCs typically operate at 700-800 ℃. The high operating temperature not only impose stringent requirements on the stability and durability of electrode and electrolyte materials, resulting in prolonged startup or shutdown times for RSOC stacks, but also poses significant challenges to the thermal stability, thermal expansion matching, and chemical stability of sealing materials and surrounding components. These collective requirements will lead to increased system costs and reduced operational lifespan, presenting critical barriers to practical application. Therefore, reducing operating temperature has become a hot topic in RSOC development. If the operating temperature of RSOCs can be reduced to 400-600 ℃, a better reliability of power generation and electrolysis in RSOC systems can be obtained, as well as a lower cost, a promoted industrialization, which aligns with the national strategy of achieving carbon peaking and carbon neutrality as soon as possible. However, as the operating temperature of RSOCs decreases, the oxygen reduction/evolution reactions (ORR/OER) kinetics become significantly sluggish due to the slow oxygen surface exchange rate, charge transfer, and limited bulk oxygen ion diffusion. Consequently, the polarization resistance (R_p) of the air electrode increases drastically, which severely constrains the practical application of RSOCs in low-temperature regime. Therefore, enhancing the ORR/OER catalytic activity of the air electrode at low temperatures is a key factor in reducing the R_p and achieving high performance RSOCs.

Generally, air electrode materials require high electrical conductivity (electronic, ionic, and/or protonic), high intrinsic electrocatalytic activity, structural and chemical stability, and durability in high oxygen partial pressure and steam content conditions. Over years of intensive research, substantial progress has been achieved through tailoring the elemental composition and stoichiometric ratios of air electrode materials, incorporating supplementary active species, and engineering microstructures that facilitate the ORR/OER processes of air electrode. Among these methods, nanotechnology plays a significant role in enhancing the ORR/OER catalytic activity of air electrodes and improving the electrochemical performance and stability of RSOCs. This review summarizes the application and research progress of nanotechnology in RSOCs air electrode materials from two perspectives: the development of novel air electrode materials and the surface modification of air electrode materials. The development of novel air electrode materials includes the preparation of nano-powders, in situ self-assembly methods, and in situ water-induced methods. The preparation of nanoscale powders is achieved through wet chemical methods, yielding high specific surface area and narrow particle size distribution, which is the first step toward obtaining highly active air electrode materials; In situ self-assembly methods involve rational design of air electrode materials composition to produce composite air electrodes with nano-particle modifications via a one-pot process; In situ water-induced methods utilize water molecule-induced cation segregation to form catalytically active phases in air electrodes. The surface modification of air electrode materials encompasses the nano-infiltration method, atomic layer deposition (ALD), pulsed laser deposition (PLD), and the construction of new air electrode structures. The nano-infiltration method can significantly improve the electrical conductivity, electrocatalytic activity, and expand the effective three-phase reaction sites by selecting an appropriate catalyst. ALD technology offers advantages such as precise regulation of membrane thickness and composition at the atomic level, low operating temperature (<300 ℃), and excellent reproducibility. PLD technology enables high-precision stoichiometric control of nanoscale films, compatibility with complex materials, and controllable microstructures. Novel air electrode structures are engineered to facilitate gas and ion transport, thereby increasing reactive sites and reducing activation losses. Finally, several suggestions for future research directions are proposed.

, authors=Qiang XUE, Guozhu ZHENG, Yucheng WU, Guangjun ZHANG, Chenxiao WANG, Kaifeng XIE, Ting CHEN, Shaorong WANG, authorsList=Qiang XUE, Guozhu ZHENG, Yucheng WU, Guangjun ZHANG, Chenxiao WANG, Kaifeng XIE, Ting CHEN, Shaorong WANG, authorCompany=null, correspAuthors=Ting CHEN, Shaorong WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319726495002636288, articleId=1319726494553846783, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=纳米技术在低温可逆固体氧化物电池空气极中的应用及研究进展, columnId=1263922774356181565, journalTitle=硅酸盐学报, columnName=综合评述, runingTitle=null, highlight=null, articleAbstract=

可逆固体氧化物电池（RSOCs）是一种可实现化学能和电能相互转化的电化学能源装置，它与可再生能源系统耦和，在电力需求低谷（波谷）时存储多余电能，在需求高峰（波峰）时高效释放电能，具有能量转化效率高、排放少、无须贵金属等优点。然而，在低温（400~600 ℃）范围内，空气极材料缓慢的氧还原/氧析出反应活性和较差的稳定性限制了RSOCs高效稳定运行，这是低温RSOCs商业化面临的关键挑战之一。近年来，纳米技术被广泛应用于提升RSOCs空气极的性能和稳定性，推动了其在低温下的应用进程。本文主要从新型空气极材料的开发和空气极材料表面修饰这2个角度出发，综述了纳米级粉体的制备、原位自组装法、原位水诱导法、表面修饰（纳米浸渍法、原子层沉积和脉冲激光沉积和空气极新型结构的构筑等纳米技术在RSOCs空气极材料中的应用及研究进展，最后对将来的研究方向提出了若干建议。

, authors=薛强, 郑国柱, 吴宇成, 张广君, 王晨骁, 谢凯峰, 陈婷, 王绍荣, authorsList=薛强, 郑国柱, 吴宇成, 张广君, 王晨骁, 谢凯峰, 陈婷, 王绍荣, authorCompany=null, correspAuthors=陈婷, 王绍荣, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=GVw+GcvZcc/HYM+zprwd8Q==, magXml=h3P4cw17/ukLtKQZrNP57g==, pdfUrl=null, pdf=BK0KSZVnRpZ7CNBabAAEhw==, pdfFileSize=2007065, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=intHGOyGVsum9Tva9mC6hg==, mapNumber=null, fund=null)}, authors=[Author(id=1319726496852324357, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319726494553846783, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=xueqiang0815@163.com, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1319726496940404743, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319726494553846783, authorId=1319726496852324357, language=EN, stringName=Qiang XUE, firstName=Qiang, middleName=null, lastName=XUE, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=School of Chemical Engineering and Technology, China University of Mining and Technology, Xuzhou 221116, Jiangsu, China, bio={"content":"

XUE Qiang (2000-), male, Master candidate. E-mail: xueqiang0815@163.com

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XUE Qiang (2000-), male, Master candidate. E-mail: xueqiang0815@163.com

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薛强（2000—），男，硕士研究生。

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薛强（2000—），男，硕士研究生。

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