Article(id=1319222735880962074, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230010, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1673193600000, receivedDateStr=2023-01-09, revisedDate=1675353600000, revisedDateStr=2023-02-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456810207, onlineDateStr=2026-10-20, pubDate=1687190400000, pubDateStr=2023-06-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456810207, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456810207, creator=13701087609, updateTime=1792456810207, updator=13701087609, issue=Issue{id=1319222716851405704, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='6', pageStart='1373', pageEnd='1648', issueExtLink='null', onlineDate='null', pubDate='1687190400000', pubDateStr='2023-06-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456805669, creator='13701087609', updateTime=1792456995739, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319223514108903801, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319223514108903802, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1530, endPage=1540, ext={EN=ArticleExt(id=1319222736082288667, articleId=1319222735880962074, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Structure and Energy Storage Characteristics of NaNbO₃-CaZrO₃-Bi_0.5Na_0.5TiO₃ Ternary System Ceramics, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

Sodium niobate(NaNbO₃)-based lead-free ceramics have attracted much attention in the pulse power capacitors due to their non-toxicity and superior energy storage properties. However, the large recoverable energy-storage density (W_rec) and efficiency (η) cannot be achieved simultaneously, thus restricting their commercialization. This work proposed astrategy of increasing the relaxation characteristics to improve the energy storage performance via constructing a local random field. The (1-x)(0.96NaNbO₃-0.04CaZrO₃)-xBi_0.5Na_0.5TiO₃ (x=0.05, 0.10, 0.15, and 0.20) antiferroelectric energy storage ceramics were prepared by a conventional solid-state method. The effect of Bi_0.5Na_0.5TiO₃ content on the phase structure, microstructure and dielectric, ferroelectric as well as energy storage properties of 0.96NaNbO₃-0.04CaZrO₃ ceramics was investigated. The results show that the microstructure of each ceramic is homogeneous and dense. The (1-x)(0.96NaNbO₃-0.04CaZrO₃)-xBi_0.5Na_0.5TiO₃ solid solution transformsfrom antiferroelectric orthorhombic P phase (x≤0.10) to antiferroelectric orthorhombic R phase (x≥0.15), accompanied by abroadening dielectric peak moving towards the lower temperatures as Bi_0.5Na_0.5TiO₃ content increases, thus having the representative relaxation characteristics. The 0.85(0.96NaNbO₃-0.04CaZrO₃)-0.15Bi_0.5Na_0.5TiO₃ ceramic has a maximum energy storage density W_rec of 1.614 J/cm³ and a high energy storage efficiency η of 83.97% under 260 kV/cm at room temperature. Besides, the ceramic exhibits a good temperature stability at 25-150 ℃ (the variation of W_rec less than 15%) and a high energy storage efficiency, which can be used as a promising material for high-temperature pulsed power capacitors.

, authors=Zixuan WANG, Zhuo LI, Jiayong ZHANG, Jing ZHANG, Yanhui NIU, authorsList=Zixuan WANG, Zhuo LI, Jiayong ZHANG, Jing ZHANG, Yanhui NIU, authorCompany=null, correspAuthors=Zhuo LI, Yanhui NIU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222736346529820, articleId=1319222735880962074, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=NaNbO₃-CaZrO₃-Bi_0.5Na_0.5TiO₃三元系陶瓷的相结构与储能性能, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

铌酸钠（NaNbO₃）无铅陶瓷由于其无毒和出色的储能性能，在脉冲功率电容器领域吸引了越来越多的关注。然而，由于较大的有效储能密度（W_rec）和高的储能效率（η）不能同时实现，限制了其商业化。通过构建局域随机场，增加弛豫特性来提高储能性能的策略。采用传统固相法制备了（1-x）（0.96NaNbO₃-0.04CaZrO₃）-xBi_0.5Na_0.5TiO₃（x=0.05、0.10、0.15、0.20）反铁电储能陶瓷，研究了不同含量Bi_0.5Na_0.5TiO₃对0.96NaNbO₃-0.04CaZrO₃陶瓷的相结构、微观形貌、介电性能和储能特性的影响。结果表明：随着Bi_0.5Na_0.5TiO₃含量的增加，（1-x）（0.96NaNbO₃-0.04CaZrO₃）-xBi_0.5Na_0.5TiO₃固溶体由反铁电正交P相（x≤0.10）转变为反铁电正交R相（x≥0.15），同时介电峰向低温方向移动并变矮宽化，呈现出明显的弛豫特性。其中，0.85（0.96NaNbO₃-0.04CaZrO₃）-0.15Bi_0.5Na_0.5TiO₃陶瓷在室温260 kV/cm的场强下展示出最好的储能性能（储能密度W_rec=1.614 J/cm³，储能效率η=83.97%），且当温度在25~150 ℃变化时，表现出良好的温度的稳定性（W_rec变化幅度<15%），同时兼具良好的储能效率，是一种非常有前途的高温脉冲功率电容器材料。

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WANG Zixuan (1998-), female, Master candidate. E-mail: 1848736995@qq.com

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WANG Zixuan (1998-), female, Master candidate. E-mail: 1848736995@qq.com

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王子瑄（1998—），女，硕士研究生。

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王子瑄（1998—），女，硕士研究生。

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