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Article(id=1319222723071558582, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20221075, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1670774400000, receivedDateStr=2022-12-12, revisedDate=1674403200000, revisedDateStr=2023-01-23, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456807152, onlineDateStr=2026-10-20, pubDate=1687190400000, pubDateStr=2023-06-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456807152, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456807152, creator=13701087609, updateTime=1792456807152, updator=13701087609, issue=Issue{id=1319222716851405704, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='6', pageStart='1373', pageEnd='1648', issueExtLink='null', onlineDate='null', pubDate='1687190400000', pubDateStr='2023-06-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456805669, creator='13701087609', updateTime=1792456995739, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319223514108903801, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319223514108903802, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222716851405704, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1476, endPage=1483, ext={EN=ArticleExt(id=1319222725009327031, articleId=1319222723071558582, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Effect of Multi Cation Doping on Dielectric Properties for (NaLn)Cu3Ti4O12(Ln=Ce; Nd) Ceramics, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

The optimization of dielectric properties for high dielectric perovskite-like ceramics is a research hotspot. (NaLn)Cu3Ti4O12 (Ln=Ce; Nd) dielectric ceramicswere prepared by ahigh-temperature solid-state methodat different sintering temperatures. The phase characteristics, microstructure and dielectric properties of the dielectric ceramics were investigated. The results show that (NaLn)Cu3Ti4O12 (Ln=Ce; Nd) ceramics are single-phase ceramics. The dielectric constant of (NaLn)Cu3Ti4O12 ceramics increasesand the dielectric loss changeswith the increase of sintering temperature. Different doping ions caninduce the corresponding polarization mechanism, further causingdifferent dielectric properties. (Na1/3Ce2/3)Cu3Ti4O12 ceramics prepared at 1 000 ℃ havethe higher dielectric properties, i.e., ε=50 552 at 10 Hz. However, the dielectric loss of (Na1/2Nd1/2)Cu3Ti4O12 ceramics prepared at 950 ℃ is smaller, i.e., tanδ=0.09 at 10 Hz.

, authors=Longfei YUAN1, Ting ZHANG2, Dandan HAN3, Shujun CHEN2, Yu ZHANG1, authorsList=Longfei YUAN, Ting ZHANG, Dandan HAN, Shujun CHEN, Yu ZHANG, authorCompany=null, correspAuthors=null, authorNote=

YUAN Longfei (1988-), male, Ph.D., candidate, Researcher. E-mail:

, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222725483283384, articleId=1319222723071558582, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=多阳离子掺杂对(NaLn)Cu3Ti4O12(Ln=Ce；Nd)陶瓷介电性能的影响, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

高介电的类钙钛矿陶瓷材料的介电性能优化一直是该领域研究热点。本研究采用高温固相法制备了不同烧结温度的（NaLn）Cu3Ti4O12（Ln=Ce；Nd）介电陶瓷材料，探讨了介电陶瓷的物相特性、显微结构和介电性能。结果表明：（NaLn）Cu3Ti4O12（Ln=Ce；Nd）系列陶瓷均为单相陶瓷。随着烧结温度提高，（NaLn）Cu3Ti4O12的介电常数增加，介电损耗变化。不同掺杂离子会使陶瓷内部极化机制发生变化，进而影响陶瓷的介电性能。其中在1 000 ℃制备的（Na1/3Ce2/3）Cu3Ti4O12陶瓷具有最高的介电性能，ε = 50 552（10 Hz）；而950 ℃制备的（Na1/2Nd1/2）Cu3Ti4O12陶瓷的介电损耗较小，tanδ=0.09（10 Hz）。

, authors=袁龙飞1, 张婷2, 韩丹丹3, 陈书军2, 张昱1, authorsList=袁龙飞, 张婷, 韩丹丹, 陈书军, 张昱, authorCompany=null, correspAuthors=null, authorNote=

袁龙飞（1988—），男，博士研究生，研究员。

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YUAN Longfei (1988-), male, Ph.D., candidate, Researcher. E-mail:

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YUAN Longfei (1988-), male, Ph.D., candidate, Researcher. E-mail:

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袁龙飞（1988—），男，博士研究生，研究员。

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袁龙飞（1988—），男，博士研究生，研究员。

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多阳离子掺杂对(NaLn)Cu3Ti4O12(Ln=Ce；Nd)陶瓷介电性能的影响
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袁龙飞 1 , 张婷 2 , 韩丹丹 3 , 陈书军 2 , 张昱 1
硅酸盐学报 | 研究论文 2023,51(6): 1476-1483
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硅酸盐学报 |研究论文 2023 , 51 (6) : 1476 -1483
多阳离子掺杂对(NaLn)Cu3Ti4O12(Ln=Ce；Nd)陶瓷介电性能的影响
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袁龙飞1 , 张婷2, 韩丹丹3, 陈书军2, 张昱1
作者信息
  • 1．遵义师范学院物理与电子科学学院，贵州 遵义 563006
  • 2．遵义师范学院化学化工学院，贵州 遵义 563006
  • 3．吉林化工学院化学与制药工程学院，吉林 吉林 132022
作者简介:

袁龙飞（1988—），男，博士研究生，研究员。

Effect of Multi Cation Doping on Dielectric Properties for (NaLn)Cu3Ti4O12(Ln=Ce; Nd) Ceramics
Longfei YUAN1 , Ting ZHANG2, Dandan HAN3, Shujun CHEN2, Yu ZHANG1
Affiliations
  • 1.College of Physics and Electronic Science, Zunyi Normal University, Zunyi 563006, Guizhou, China
  • 2.College of Chemistry and Chemical Engineering, Zunyi Normal University, Zunyi 563006, Guizhou, China
  • 3.College of Chemistry and Pharmaceutical Engineering, Jilin institute of chemical technology, Jilin 132022, Jilin, China

    • YUAN Longfei (1988-), male, Ph.D., candidate, Researcher. E-mail:

出版时间: 2023-06-20 doi: 10.14062/j.issn.0454-5648.20221075
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高介电的类钙钛矿陶瓷材料的介电性能优化一直是该领域研究热点。本研究采用高温固相法制备了不同烧结温度的（NaLn）Cu3Ti4O12（Ln=Ce；Nd）介电陶瓷材料，探讨了介电陶瓷的物相特性、显微结构和介电性能。结果表明：（NaLn）Cu3Ti4O12（Ln=Ce；Nd）系列陶瓷均为单相陶瓷。随着烧结温度提高，（NaLn）Cu3Ti4O12的介电常数增加，介电损耗变化。不同掺杂离子会使陶瓷内部极化机制发生变化，进而影响陶瓷的介电性能。其中在1 000 ℃制备的（Na1/3Ce2/3）Cu3Ti4O12陶瓷具有最高的介电性能，ε = 50 552（10 Hz）；而950 ℃制备的（Na1/2Nd1/2）Cu3Ti4O12陶瓷的介电损耗较小，tanδ=0.09（10 Hz）。

类钙钛矿陶瓷  /  介电陶瓷  /  极化机制  /  巨介电性能

The optimization of dielectric properties for high dielectric perovskite-like ceramics is a research hotspot. (NaLn)Cu3Ti4O12 (Ln=Ce; Nd) dielectric ceramicswere prepared by ahigh-temperature solid-state methodat different sintering temperatures. The phase characteristics, microstructure and dielectric properties of the dielectric ceramics were investigated. The results show that (NaLn)Cu3Ti4O12 (Ln=Ce; Nd) ceramics are single-phase ceramics. The dielectric constant of (NaLn)Cu3Ti4O12 ceramics increasesand the dielectric loss changeswith the increase of sintering temperature. Different doping ions caninduce the corresponding polarization mechanism, further causingdifferent dielectric properties. (Na1/3Ce2/3)Cu3Ti4O12 ceramics prepared at 1 000 ℃ havethe higher dielectric properties, i.e., ε=50 552 at 10 Hz. However, the dielectric loss of (Na1/2Nd1/2)Cu3Ti4O12 ceramics prepared at 950 ℃ is smaller, i.e., tanδ=0.09 at 10 Hz.

perovskite-like ceramics  /  dielectric ceramic  /  polarization mechanism  /  giant dielectric properties
袁龙飞, 张婷, 韩丹丹, 陈书军, 张昱. 多阳离子掺杂对(NaLn)Cu3Ti4O12(Ln=Ce；Nd)陶瓷介电性能的影响. 硅酸盐学报, 2023 , 51 (6) : 1476 -1483 . DOI: 10.14062/j.issn.0454-5648.20221075
Longfei YUAN, Ting ZHANG, Dandan HAN, Shujun CHEN, Yu ZHANG. Effect of Multi Cation Doping on Dielectric Properties for (NaLn)Cu3Ti4O12(Ln=Ce; Nd) Ceramics[J]. Journal of the Chinese Ceramic Society, 2023 , 51 (6) : 1476 -1483 . DOI: 10.14062/j.issn.0454-5648.20221075
基金
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  • 贵州省省级科技计划项目资助(黔科合基础[2020]1Y207)
  • 贵州省教育厅项目(黔教合KY字[2020]098)
  • 遵义市科技局项目(黔科合平台人才[2018]5784-02号)
  • 遵义师范学院科研项目(遵师BS[2019]03)
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2023年第51卷第6期
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doi: 10.14062/j.issn.0454-5648.20221075
  • 接收时间：2022-12-12
  • 首发时间：2026-10-20
  • 出版时间：2023-06-20
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  • 收稿日期：2022-12-12
  • 修回日期：2023-01-23
基金
贵州省省级科技计划项目资助(黔科合基础[2020]1Y207)
贵州省教育厅项目(黔教合KY字[2020]098)
遵义市科技局项目(黔科合平台人才[2018]5784-02号)
遵义师范学院科研项目(遵师BS[2019]03)
作者信息
    1．遵义师范学院物理与电子科学学院，贵州 遵义 563006
    2．遵义师范学院化学化工学院，贵州 遵义 563006
    3．吉林化工学院化学与制药工程学院，吉林 吉林 132022
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20221075
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2种不同金属材料的力学参数
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Number of
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Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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