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In recent years, low dimensional organic-inorganic hybrid copper(I) halides have a great potential in the fields of photoelectric and radiation detection applications due to their high fluorescence quantum efficiency, excellent stability, and low-cost processing feasibility. We prepared a zero dimensional (0D) (TPA)CuI₂ (TPA=tetrapropylammonium, C₁₂H₂₈N⁺) single crystal scintillator by a simple solution evaporation method, and investigate its optical and scintillation properties. (TPA)CuI₂ crystal has a high thermal stability and an air stability. Under UV excitation, it exhibits an ultra-broadband white light emission with a full width at half-maximum (FWHM) of 291 nm and a photoluminescence quantum yield (PLQY) of 62%. Under X-ray excitation, it has an intense radioluminescence, a low afterglow and a decent detection limit, which can be regarded as a novel X-ray scintillator.

, authors=Wen LI, Tingting XU, Yunyun LI, Yuntao WU, authorsList=Wen LI, Tingting XU, Yunyun LI, Yuntao WU, authorCompany=null, correspAuthors=Yunyun LI, Yuntao WU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222830642877280, articleId=1319222830126977886, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=零维有机-无机杂化碘化亚铜闪烁晶体的制备及其X射线探测性能, columnId=1321890966106129285, journalTitle=硅酸盐学报, columnName=晶体结构与缺陷相关基础研究进展专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

低维有机-无机杂化铜卤化物由于拥有高荧光量子效率、高稳定性和可低成本溶液法制备等优点，近年来在光电和辐射探测等领域展现出巨大应用潜力。本工作通过溶液蒸发法成功制备了零维结构（TPA）CuI₂（TPA=四丙基铵，C₁₂H₂₈N⁺）闪烁体单晶，并对其光学和X射线闪烁探测性能进行了研究。（TPA）CuI₂晶体具有高热稳定性和空气稳定性，在紫外激发下，晶体展现出具有291 nm半高全宽的超宽带白光发射，荧光量子效率为62%；在X射线激发下表现出强辐照发光、低余辉、低检测限，是一种新型高性能X射线探测闪烁体。

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LI Wen (1996-), female, Master Candidate. E-mail: liwenLW1996@163.com

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LI Wen (1996-), female, Master Candidate. E-mail: liwenLW1996@163.com

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李雯（1996—），女，硕士研究生。

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李雯（1996—），女，硕士研究生。

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