Article(id=1319222277149934577, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220688, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1661270400000, receivedDateStr=2022-08-24, revisedDate=1662048000000, revisedDateStr=2022-09-02, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456700836, onlineDateStr=2026-10-20, pubDate=1674144000000, pubDateStr=2023-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456700836, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456700836, creator=13701087609, updateTime=1792456700836, updator=13701087609, issue=Issue{id=1319222240177144549, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='1', pageStart='1', pageEnd='282', issueExtLink='null', onlineDate='null', pubDate='1674144000000', pubDateStr='2023-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456692021, creator='13701087609', updateTime=1792456863865, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319222960989262349, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319222960989262350, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=194, endPage=203, ext={EN=ArticleExt(id=1319222277556782066, articleId=1319222277149934577, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Selective Catalytic Reduction Activity of MnO_x/TiO₂ Catalyst Under Impact of Mineral Polarization, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

The low denitration activity and stability of MnO_x/TiO₂ catalyst are still challenging. In this work, a MnO_x/TiO₂ catalyst was modified via a polarization effect with tourmaline. Tourmaline with a proper fineness can improve the denitration performance of the catalytic material, obtaining the greater denitration rate above 90% in a wide temperature range and the prolonged high-efficiency denitration time. Based on the results of in-situ Fourier transform infrared spectroscopy, the reaction mechanism of the catalysts before and after modification with tourmaline follows the Langmuir-Hinshelwood mechanism, and tourmaline polarization can accelerate the adsorption rate of reaction gas and generate intermediate products liable for subsequent reaction, thus improving the denitration performance.

, authors=Yizhe HELIAN, Suping CUI, Xiaoyu MA, Yali WANG, Haiying XU, authorsList=Yizhe HELIAN, Suping CUI, Xiaoyu MA, Yali WANG, Haiying XU, authorCompany=null, correspAuthors=Suping CUI, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222277972018163, articleId=1319222277149934577, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=矿物极化效应影响下MnO_x/TiO₂催化剂SCR活性, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

MnO_x/TiO₂催化剂的低温脱硝活性和稳定性是目前具有挑战性的研究方向。采用矿物极化效应对MnO_x/TiO₂催化剂进行了改性研究。适当细度的电气石对催化材料的脱硝性能有明显的改善，在较宽的温度范围内脱硝效率保持在90%以上，并延长了较高脱硝效率的持续时间。原位漫反射红外光谱分析结果表明，改性前后的催化剂遵循Langmuir-Hinshelwood机理，电气石极化可以加快反应气体的吸附速率，生成易于参与到后续反应的中间产物，从而提高脱硝性能。

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HELIAN Yizhe (1995-), male, Ph.D. E-mail: helian@emails.bjut.edu.cn

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HELIAN Yizhe (1995-), male, Ph.D. E-mail: helian@emails.bjut.edu.cn

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赫连一哲（1995—），男，博士。

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赫连一哲（1995—），男，博士。

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