Article(id=1319222254827848530, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220352, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1651248000000, receivedDateStr=2022-04-30, revisedDate=1653840000000, revisedDateStr=2022-05-30, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456695514, onlineDateStr=2026-10-20, pubDate=1674144000000, pubDateStr=2023-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456695514, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456695514, creator=13701087609, updateTime=1792456695514, updator=13701087609, issue=Issue{id=1319222240177144549, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='1', pageStart='1', pageEnd='282', issueExtLink='null', onlineDate='null', pubDate='1674144000000', pubDateStr='2023-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456692021, creator='13701087609', updateTime=1792456863865, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319222960989262349, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319222960989262350, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=14, endPage=22, ext={EN=ArticleExt(id=1319222255054340947, articleId=1319222254827848530, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Photocatalytic Properties and Reaction Mechanism of PDI/ZnIn₂S₄ S-Scheme Heterojunction, columnId=1321891568328487649, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Photocatalytic Materials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

The construction of step scheme (S-scheme) heterojunction with a great redox ability and a high charge transfer efficiency is an effective strategy to enhance the photocatalytic activity. ZnIn₂S₄ nanosheets were grown in-situ on the surface of perylenimide (PDI) rods via a solvothermal method. A PDI/ZnIn₂S₄ heterojunction exhibits an excellent photocatalytic performance due to its tight interfacial contact and matched band structures. Moreover, the 5% PDI/ZnIn₂S₄ affords high H₂/benzaldehyde production rates of 21.66 mmol/(g·h) and 1.02 mmol/(g·h), respectively, which is 2.12 and 3.00 folds of pristine ZnIn₂S₄, respectively when coupling the photocatalytic H₂ evolution and the benzyl alcohol oxidation in the reaction system. Based on the results by X-ray photoelectron spectroscopy, transient photoluminescence spectroscopy and electron paramagnetic resonance analysis, the formation of the built-in electric field at the interface of PDI/ZnIn₂S₄ and the S-scheme electron transfer path was confirmed. The enhanced photocatalytic performance and stability can be attributed to the close contact and rich active sites of PDI/ZnIn₂S₄, and the charge carrier migration and increased photoredox properties were improved by a S-scheme charge-transfer route. This organic-inorganic PDI/ZnIn₂S₄ S-scheme heterojunction photocatalyst can be used as a novel bifunctional photocatalyst in converting solar light into clean fuel and chemicals.

, authors=Hua TANG^{1, 2}, Yue LIU¹, Lele WANG¹, Qinqin LIU¹, authorsList=Hua TANG, Yue LIU, Lele WANG, Qinqin LIU, authorCompany=null, correspAuthors=Qinqin LIU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222255377302356, articleId=1319222254827848530, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=苝酰亚胺/ZnIn₂S₄ S型异质结光催化性能与反应机制, columnId=1321891568521425634, journalTitle=硅酸盐学报, columnName=光催化材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

构建较强氧化还原能力与较高电荷转移效率的阶梯型（S型）异质结光催化剂是提高光催化性能的有效策略。通过溶剂热法在棒状苝酰亚胺（PDI）表面原位生长了ZnIn₂S₄纳米片，得益于良好的界面接触与匹配的能带结构，PDI/ZnIn₂S₄异质结展现出优异的光催化性能。此外，在同步光催化产氢与苯甲醇氧化全反应体系中，5% PDI/ZnIn₂S₄光催化剂表现出较高的产氢性能[21.66 mmol/（g·h）]与苯甲醛产率[1.02 mmol/（g·h）]分别是纯ZnIn₂S₄的2.12倍和3.00倍。基于X射线光电子能谱、瞬态光致发光光谱和电子顺磁共振信号等分析，证实了PDI与ZnIn₂S₄之间内建电场的形成与S型电子转移路径。该电荷转移机制保留了复合催化剂较高的氧化还原电位，促进了界面电荷分离与转移，进而提升了光催化性能。该有机-无机S型异质结光催化剂的设计应用为新型双功能催化剂的开发提供了新思路。

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