Article(id=1319236926025089917, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236892848148894, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220251, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1649088000000, receivedDateStr=2022-04-05, revisedDate=1650470400000, revisedDateStr=2022-04-21, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460193400, onlineDateStr=2026-10-20, pubDate=1668873600000, pubDateStr=2022-11-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460193400, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460193400, creator=13701087609, updateTime=1792460193400, updator=13701087609, issue=Issue{id=1319236892848148894, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='11', pageStart='2809', pageEnd='3090', issueExtLink='null', onlineDate='null', pubDate='1668873600000', pubDateStr='2022-11-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460185491, creator='13701087609', updateTime=1792460700564, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319239053275411177, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236892848148894, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319239053275411178, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236892848148894, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=3040, endPage=3060, ext={EN=ArticleExt(id=1319236926310302590, articleId=1319236926025089917, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Challenges and Solutions of Lithium-Rich Manganese-Based Cathode Materials for Lithium-Ion Batteries, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

With the rapid development of consumer electronics, electric vehicles and energy storage, it is urgent to improve the energy density of secondary energy storage devices represented by lithium-ion batteries. Cathode materials are a key issue to improve the energy density of lithium-ion batteries. Li-rich Mn-based layered oxide cathode materials (LRM) are considered as one of the most promising cathode materials for lithium-ion batteries due to their extremely high theoretical specific capacity (>350 mA·h·g^-1) and reversible specific capacity (>250 mA·h·g^-1). However, the low initial Coulombic efficiency, poor rate performance, and rapid voltage and capacity fading of LRM cathode materials seriously restrict their industrial application. This review introduced the research progress of the crystal structure and electrochemical mechanism of LRM cathode materials, and analyzed the problems of LRM. The modification strategies of LRM cathode materials were comprehensively introduced from the aspects of morphology design control, doping, coating, defect structure design, gradient composition design, layered/spinel heterostructure construction, and electrolyte additives. We provided some ideas and guidance for the future development of LRM cathodes to ultimately promote the practical application of LRM cathode materials.

, authors=Wenhua YU, Liuyang ZHAO, Yanyan WANG, Xinpeng LIU, Hongyi LI, Aimin WU, Hao HUANG, authorsList=Wenhua YU, Liuyang ZHAO, Yanyan WANG, Xinpeng LIU, Hongyi LI, Aimin WU, Hao HUANG, authorCompany=null, correspAuthors=Hao HUANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319236926599709567, articleId=1319236926025089917, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=锂离子电池富锂锰基正极材料面临的挑战及解决方案, columnId=1263922774356181565, journalTitle=硅酸盐学报, columnName=综合评述, runingTitle=null, highlight=null, articleAbstract=

随着消费类电子、电动汽车和储能等领域的迅猛发展，亟需提升以锂离子电池为代表的二次储能设备的能量密度，而正极材料是提升锂离子电池能量密度的关键。富锂锰基层状氧化物正极材料（LRM）因具有极高的理论比容量（>350 mA·h·g^-1）和可逆比容量（>250 mA·h·g^-1）被认为是最有前途的锂离子电池正极材料之一。然而，LRM正极材料的首次Coulombic效率低、倍率/性能差以及快速的电压和容量衰减等问题，严重阻碍了其产业化应用。本文介绍了LRM正极材料的晶体结构及电化学机理等方面的研究进展，分析了LRM存在的问题及起因。重点从形貌设计调控、掺杂、包覆、缺陷结构设计、梯度成分设计、层状/尖晶石异质结构构建以及电解液添加剂等方面全面介绍了LRM正极材料的改性策略，以期望为LRM正极的未来发展提供思路和指导，最终促进LRM正极材料的实际应用。

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YU Wenhua (1991-), male, Doctoral candidate. E-mail: ywhdllg@mail.dlut.edu.cn

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YU Wenhua (1991-), male, Doctoral candidate. E-mail: ywhdllg@mail.dlut.edu.cn

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于文华（1991—），女，博士研究生。

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于文华（1991—），女，博士研究生。

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