Article(id=1319222248955822872, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220218, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1646582400000, receivedDateStr=2022-03-07, revisedDate=1649174400000, revisedDateStr=2022-04-06, acceptedDate=null, acceptedDateStr=null, onlineDate=1792456694114, onlineDateStr=2026-10-20, pubDate=1674144000000, pubDateStr=2023-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792456694114, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792456694114, creator=13701087609, updateTime=1792456694114, updator=13701087609, issue=Issue{id=1319222240177144549, tenantId=1146029695717560320, journalId=1263187385517883426, year='2023', volume='51', issue='1', pageStart='1', pageEnd='282', issueExtLink='null', onlineDate='null', pubDate='1674144000000', pubDateStr='2023-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792456692021, creator='13701087609', updateTime=1792456863865, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319222960989262349, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319222960989262350, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319222240177144549, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=64, endPage=72, ext={EN=ArticleExt(id=1319222249173926681, articleId=1319222248955822872, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Effect of Pyrene-Benzothiadiazole Linkage Sites on Photocatalytic Hydrogen Evolution, columnId=1321891568328487649, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Photocatalytic Materials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

The design and synthesis of organic polymers for photocatalytic hydrogen evolution have attracted recent attention. However, the corresponding work on the synthesis methods and optimal synthesis sites of organic polymers are not complete. This paper was to synthesize five organic polymer photocatalysts via a Suzuki cross-coupling polymerization reaction. The effect of linking position content on the photocatalytic H₂-evolution and photoelectrochemical performances of organic polymer semiconductors was investigated. The results show that the increase of 1,6-linkage pattern severely affects the photocatalytic hydrogen evolution effect. A 1,6-linked pyrene benzothiadiazole polymer (L16-PyBT) has a photocatalytic hydrogen evolution rate of 6.81 mmol/(h·g) under visible-light irradiation, which is greater than that of L2 (i.e., 2.80 mmol/(h·g) and L27-PyBT (i.e., 0.34 mmol/(h·g). The increased photocatalysis is since 1,6-linkage has a stronger π-π stacking, and better absorption/wettability. The evolution of this connection mode provides an important idea for the synthesis and design of organic polymers in the future.

, authors=Huan HE¹, Ruiqi GAO¹, Hongjing HE², Ningxing WANG², Weiling BI², Shuling CHEN², Rongchen SHEN¹, Xin LI¹, authorsList=Huan HE, Ruiqi GAO, Hongjing HE, Ningxing WANG, Weiling BI, Shuling CHEN, Rongchen SHEN, Xin LI, authorCompany=null, correspAuthors=Xin LI, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319222249421390618, articleId=1319222248955822872, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=芘-苯并噻二唑连接位点对光催化制氢的影响, columnId=1321891568521425634, journalTitle=硅酸盐学报, columnName=光催化材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

近来，用于光催化析氢的有机聚合物的设计和合成引起了许多关注。然而，关于有机聚合物的最佳连接位点的报道并不完整。通过Suzuki交叉偶联聚合反应合成了3种有机聚合物光催化剂。研究了连接位点的含量对有机聚合物半导体光催化剂的析氢性能及光电化学性能的影响。发现1，6-连接位点的增加大大加强了光催化析氢效果，尤其是1，6位连接的芘-苯并噻二唑基聚合物（L16-PyBT）在可见光照射下的光催化析氢速率为6.81 mmol/（h·g），远大于其他2种有机聚合物[2.80 mmol/（h·g）和0.34 mmol/（h·g）]。结果表明：1，6-连接方式具有更强的π-π堆积、更好的光吸收能力和润湿性，从而提高光催化性能。这种连接方式的演变为未来有机聚合物的合成和设计提供了重要思路。

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何欢（1999—），男，硕士研究生。

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