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Article(id=1319236754960400849, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236705027207343, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220042, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1642089600000, receivedDateStr=2022-01-14, revisedDate=1643472000000, revisedDateStr=2022-01-30, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460152616, onlineDateStr=2026-10-20, pubDate=1666195200000, pubDateStr=2022-10-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460152616, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460152616, creator=13701087609, updateTime=1792460152616, updator=13701087609, issue=Issue{id=1319236705027207343, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='10', pageStart='2579', pageEnd='2808', issueExtLink='null', onlineDate='null', pubDate='1666195200000', pubDateStr='2022-10-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460140711, creator='13701087609', updateTime=1792460672919, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319238937323884737, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236705027207343, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319238937323884738, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236705027207343, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2762, endPage=2769, ext={EN=ArticleExt(id=1319236755438551506, articleId=1319236754960400849, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Preparation and Application of Colorimetric Sensor Based on Ferric Doping-Montmorillonite Nanozyme, columnId=1321898015569331178, journalTitle=Journal of the Chinese Ceramic Society, columnName=Advanced Founctional Geomaterials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

Nanozyme can quickly and sensitively detect biomarkers to prevent the outbreak of diseases. However, the low catalytic activity and poor affinity for substrates restrict the detection performance. Montmorillonite, as a typical 2:1 layered silicate clay mineral, has a good adsorption and cation exchange ability. Thus, Fe3+ can be anchored into the layers to prepare Fe doping montmorillonite nanozyme with a peroxidase-like property, enhancing the affinity for H2O2 and realizing the colorimetric detection of H2O2. The results show that the linear range and detection limit of H2O2 are 20-500 μmol/L and 5.8 μmol/L under neutral conditions, respectively. The colorimetric method for silicate clay mineral nanozyme has a good application prospect in the fields of analytical detection and disease diagnosis.

, authors=Luyuan TIAN1, 2, 3, Hao WANG1, 2, 3, Aidong TANG1, 2, 3, 4, Huaming YANG1, 2, 3, 5, 6, authorsList=Luyuan TIAN, Hao WANG, Aidong TANG, Huaming YANG, authorCompany=null, correspAuthors=Aidong TANG, Huaming YANG, authorNote=

TIAN Luyuan (1995-), male, Doctoral candidate. E-mail:

, correspAuthorsNote=
TANG Aidong (1968-), female, Ph.D., Professor; E-mail:
YANG Huaming (1968-), male, Ph.D., Professor.
, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319236755820233171, articleId=1319236754960400849, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=铁掺杂蒙脱石纳米酶的制备与应用, columnId=1321898015758074859, journalTitle=硅酸盐学报, columnName=高性能矿物功能材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

纳米酶可以快速灵敏地检测生物标记物，有效防止疾病的爆发，但是纳米酶的催化活性低、对底物亲和力差，严重地制约了其检测性能。蒙脱石是一种具有典型的2∶1型层状结构的硅酸盐黏土矿物，利用其良好的吸附能力和阳离子交换能力，将Fe3+锚定在蒙脱石的表面与层间，制备具有类过氧化物酶性质的Fe掺杂蒙脱石纳米酶，可增强对H2O2的亲和力，通过比色法可实现对H2O2的检测。结果表明：在中性条件下，H2O2的检测线性范围和检测限分别为20~500 μmol/L和5.8 μmol/L。这种蒙脱石纳米酶在分析检测和疾病诊断领域具有良好的应用前景。

, authors=田路远1, 2, 3, 汪浩1, 2, 3, 唐爱东1, 2, 3, 4, 杨华明1, 2, 3, 5, 6, authorsList=田路远, 汪浩, 唐爱东, 杨华明, authorCompany=null, correspAuthors=唐爱东, 杨华明, authorNote=

田路远（1995—），男，博士研究生。

, correspAuthorsNote=
唐爱东（1968—），女，博士，教授；
杨华明（1968—），男，博士，教授。
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铁掺杂蒙脱石纳米酶的制备与应用
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田路远 1, 2, 3 , 汪浩 1, 2, 3 , 唐爱东 1, 2, 3, 4 , 杨华明 1, 2, 3, 5, 6
硅酸盐学报 | 高性能矿物功能材料专题—研究论文 2022,50(10): 2762-2769
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硅酸盐学报 |高性能矿物功能材料专题—研究论文 2022 , 50 (10) : 2762 -2769
铁掺杂蒙脱石纳米酶的制备与应用
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3．中国非金属矿行业矿物功能材料重点实验室，中国地质大学（武汉），武汉 430074
5．中南大学资源加工与生物工程学院，长沙 410083
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田路远1, 2, 3 , 汪浩1, 2, 3, 唐爱东1, 2, 3, 4 , 杨华明1, 2, 3, 5, 6
作者信息
  • 1．中国地质大学（武汉）纳米矿物材料及应用教育部工程研究中心
  • 2．中国地质大学（武汉）材料与化学学院
  • 3．中国非金属矿行业矿物功能材料重点实验室，中国地质大学（武汉），武汉 430074
  • 4．中南大学化学化工学院，长沙 410083
  • 5．中南大学资源加工与生物工程学院，长沙 410083
  • 6．中南大学矿物材料及其应用湖南省重点实验室，长沙 410083
通讯作者:
唐爱东（1968—），女，博士，教授；
杨华明（1968—），男，博士，教授。
作者简介:

田路远（1995—），男，博士研究生。

Preparation and Application of Colorimetric Sensor Based on Ferric Doping-Montmorillonite Nanozyme
Luyuan TIAN1, 2, 3 , Hao WANG1, 2, 3, Aidong TANG1, 2, 3, 4 , Huaming YANG1, 2, 3, 5, 6
Affiliations
  • 1.Engineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan 430074, China
  • 2.Faculty of Materials Science and Chemistry, China University of Geosciences, Wuhan 430074, China
  • 3.Key Laboratory of Functional Geomaterials in China Nonmetallic Minerals Industry, China University of Geosciences, Wuhan 430074, China
  • 4.School of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China
  • 5.School of Minerals Processing and Bioengineering, Central South University, Changsha 410083, China
  • 6.Hunan Key Lab of Mineral Materials and Application, Central South University, Changsha 410083, China
    • Corresponding Author:
    TANG Aidong (1968-), female, Ph.D., Professor; E-mail:
    YANG Huaming (1968-), male, Ph.D., Professor.

    TIAN Luyuan (1995-), male, Doctoral candidate. E-mail:

出版时间: 2022-10-20 doi: 10.14062/j.issn.0454-5648.20220042
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纳米酶可以快速灵敏地检测生物标记物，有效防止疾病的爆发，但是纳米酶的催化活性低、对底物亲和力差，严重地制约了其检测性能。蒙脱石是一种具有典型的2∶1型层状结构的硅酸盐黏土矿物，利用其良好的吸附能力和阳离子交换能力，将Fe3+锚定在蒙脱石的表面与层间，制备具有类过氧化物酶性质的Fe掺杂蒙脱石纳米酶，可增强对H2O2的亲和力，通过比色法可实现对H2O2的检测。结果表明：在中性条件下，H2O2的检测线性范围和检测限分别为20~500 μmol/L和5.8 μmol/L。这种蒙脱石纳米酶在分析检测和疾病诊断领域具有良好的应用前景。

纳米酶  /  蒙脱石  /  类过氧化物酶  /  铁掺杂  /  比色法  /  分析检测

Nanozyme can quickly and sensitively detect biomarkers to prevent the outbreak of diseases. However, the low catalytic activity and poor affinity for substrates restrict the detection performance. Montmorillonite, as a typical 2:1 layered silicate clay mineral, has a good adsorption and cation exchange ability. Thus, Fe3+ can be anchored into the layers to prepare Fe doping montmorillonite nanozyme with a peroxidase-like property, enhancing the affinity for H2O2 and realizing the colorimetric detection of H2O2. The results show that the linear range and detection limit of H2O2 are 20-500 μmol/L and 5.8 μmol/L under neutral conditions, respectively. The colorimetric method for silicate clay mineral nanozyme has a good application prospect in the fields of analytical detection and disease diagnosis.

nanozyme  /  montmorillonite  /  peroxidase-like property  /  iron doping  /  colorimetric method  /  analytical detection
田路远, 汪浩, 唐爱东, 杨华明. 铁掺杂蒙脱石纳米酶的制备与应用. 硅酸盐学报, 2022 , 50 (10) : 2762 -2769 . DOI: 10.14062/j.issn.0454-5648.20220042
Luyuan TIAN, Hao WANG, Aidong TANG, Huaming YANG. Preparation and Application of Colorimetric Sensor Based on Ferric Doping-Montmorillonite Nanozyme[J]. Journal of the Chinese Ceramic Society, 2022 , 50 (10) : 2762 -2769 . DOI: 10.14062/j.issn.0454-5648.20220042
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  • 中国博士后科学基金(2020M682518)
  • 湖北省博士后创新研究计划(265053)
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doi: 10.14062/j.issn.0454-5648.20220042
  • 接收时间：2022-01-14
  • 首发时间：2026-10-20
  • 出版时间：2022-10-20
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  • 收稿日期：2022-01-14
  • 修回日期：2022-01-30
基金
中国博士后科学基金(2020M682518)
湖北省博士后创新研究计划(265053)
作者信息
    1．中国地质大学（武汉）纳米矿物材料及应用教育部工程研究中心
    2．中国地质大学（武汉）材料与化学学院
    3．中国非金属矿行业矿物功能材料重点实验室，中国地质大学（武汉），武汉 430074
    4．中南大学化学化工学院，长沙 410083
    5．中南大学资源加工与生物工程学院，长沙 410083
    6．中南大学矿物材料及其应用湖南省重点实验室，长沙 410083

通讯作者:

唐爱东（1968—），女，博士，教授；
杨华明（1968—），男，博士，教授。
参考文献
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20220042
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2种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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