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Article(id=1319236447522111765, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236433387303232, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220020, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1641657600000, receivedDateStr=2022-01-09, revisedDate=1642608000000, revisedDateStr=2022-01-20, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460079316, onlineDateStr=2026-10-20, pubDate=1660924800000, pubDateStr=2022-08-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460079316, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460079316, creator=13701087609, updateTime=1792460079316, updator=13701087609, issue=Issue{id=1319236433387303232, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='8', pageStart='2067', pageEnd='2350', issueExtLink='null', onlineDate='null', pubDate='1660924800000', pubDateStr='2022-08-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460075946, creator='13701087609', updateTime=1792460621958, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319238723569569958, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236433387303232, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319238723569569959, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236433387303232, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2145, endPage=2156, ext={EN=ArticleExt(id=1319236449317273880, articleId=1319236447522111765, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Preparation of High-Performance Porous Carbon Fiber Electrode from Natural Fiber and Lignin Nanoparticles, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

Carbon fiber based electrodes were prepared by a solvent exchange method with natural cellulose fibers as versatile supports of lignin nanoparticles (LNPs) to uniformly in-situ load LNPs on the surface of fibers. The morphology, specific surface area, thermal stability, phase composition, structure and electrochemical performance of carbon fiber electrodes were investigated by X-ray diffraction, scanning electron microscopy, nitrogen adsorption, thermogravimetric analysis, X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy, and electrochemical tests, respectively. The results show that the prepared carbon fiber based electrode has a maximum specific capacitance of 7.88 F/g at an initial mass ratio of LNPs to cellulose fiber of 1∶10, which is greater than that of the control biomass carbon fiber (0.60 F/g) without loading LNPs. After 10 000-cycle test (10 A/g), the capacitance retention is still 93%. Also, LNPs loaded on the surface of fibers can effectively endow composite carbon fiber electrodes with a high specific surface area and a high carbon content, which can provides a possible path for the effective utilization of lignin in energy fields.

, authors=Wei ZHANG1, Xingye AN1, Liqin LIU1, Yinying LONG1, Hao ZHANG1, Haibing CAO2, Zhengbai CHENG2, Hongbin LIU1, authorsList=Wei ZHANG, Xingye AN, Liqin LIU, Yinying LONG, Hao ZHANG, Haibing CAO, Zhengbai CHENG, Hongbin LIU, authorCompany=null, correspAuthors=Xingye AN, Hongbin LIU, authorNote=

ZHANG Wei (1996-), male, Master candidate. E-mail:

, correspAuthorsNote=
AN Xingye (1988-), male, Ph.D., Associate Professor; E-mail: Xingye An ()
LIU Hongbin (1977-), male, Ph.D., Professor. Hongbin Liu ()
, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319236450026111257, articleId=1319236447522111765, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=天然纤维/木质素纳米颗粒制备高性能多孔碳纤维电极, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

以天然纤维为载体，利用溶剂交换法将木质素纳米颗粒（LNPs）负载到纤维表面制备碳纤维电极材料，研究碳纤维材料的形貌、比表面积、热稳定性、结晶性能、表面电荷和电化学性能。结果表明：在LNPs与纤维的初始质量比为1∶10时，电极材料比电容最大，为7.88 F/g，远高于未负载LNPs的电极材料比电容值（0.60 F/g）；在经过10 000次的循环测试（10 A/g）后，电容保持率高达93%。研究表明LNPs可有效提高复合碳纤维电极材料的比表面积和碳含量，为木质素在能源领域中的高附加值利用提供了新途径。

, authors=张伟1, 安兴业1, 刘利琴1, 龙垠荧1, 张昊1, 曹海兵2, 程正柏2, 刘洪斌1, authorsList=张伟, 安兴业, 刘利琴, 龙垠荧, 张昊, 曹海兵, 程正柏, 刘洪斌, authorCompany=null, correspAuthors=安兴业, 刘洪斌, authorNote=

张伟（1996—），男，硕士研究生。

, correspAuthorsNote=
安兴业（1988—），男，博士，副教授；
刘洪斌（1977—），男，博士，研究员。
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ZHANG Wei (1996-), male, Master candidate. E-mail:

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ZHANG Wei (1996-), male, Master candidate. E-mail:

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张伟（1996—），男，硕士研究生。

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张伟（1996—），男，硕士研究生。

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天然纤维/木质素纳米颗粒制备高性能多孔碳纤维电极
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张伟 1 , 安兴业 1 , 刘利琴 1 , 龙垠荧 1 , 张昊 1 , 曹海兵 2 , 程正柏 2 , 刘洪斌 1
硅酸盐学报 | 研究论文 2022,50(8): 2145-2156
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硅酸盐学报 |研究论文 2022 , 50 (8) : 2145 -2156
天然纤维/木质素纳米颗粒制备高性能多孔碳纤维电极
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张伟1 , 安兴业1 , 刘利琴1, 龙垠荧1, 张昊1, 曹海兵2, 程正柏2, 刘洪斌1
作者信息
  • 1．天津科技大学轻工科学与工程学院，天津市制浆造纸重点实验室，天津 300457
  • 2．浙江景兴纸业股份有限公司，浙江 平湖 314214
通讯作者:
安兴业（1988—），男，博士，副教授；
刘洪斌（1977—），男，博士，研究员。
作者简介:

张伟（1996—），男，硕士研究生。

Preparation of High-Performance Porous Carbon Fiber Electrode from Natural Fiber and Lignin Nanoparticles
Wei ZHANG1 , Xingye AN1 , Liqin LIU1, Yinying LONG1, Hao ZHANG1, Haibing CAO2, Zhengbai CHENG2, Hongbin LIU1
Affiliations
  • 1.College of Light Industry Science and Engineering, Tianjin Key Laboratory of Pulp and Paper, Tianjin University of Science and Technology, Tianjin 300457, China
  • 2.Zhejiang Jing Xing Paper Joint Stock Co., Ltd., Pinghu 314214, Zhejiang, China
    • Corresponding Author:
    AN Xingye (1988-), male, Ph.D., Associate Professor; E-mail: Xingye An ()
    LIU Hongbin (1977-), male, Ph.D., Professor. Hongbin Liu ()

    ZHANG Wei (1996-), male, Master candidate. E-mail:

出版时间: 2022-08-20 doi: 10.14062/j.issn.0454-5648.20220020
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以天然纤维为载体，利用溶剂交换法将木质素纳米颗粒（LNPs）负载到纤维表面制备碳纤维电极材料，研究碳纤维材料的形貌、比表面积、热稳定性、结晶性能、表面电荷和电化学性能。结果表明：在LNPs与纤维的初始质量比为1∶10时，电极材料比电容最大，为7.88 F/g，远高于未负载LNPs的电极材料比电容值（0.60 F/g）；在经过10 000次的循环测试（10 A/g）后，电容保持率高达93%。研究表明LNPs可有效提高复合碳纤维电极材料的比表面积和碳含量，为木质素在能源领域中的高附加值利用提供了新途径。

天然纤维  /  木质素纳米颗粒  /  比表面积  /  生物质碳纤维  /  电极材料  /  电化学性能

Carbon fiber based electrodes were prepared by a solvent exchange method with natural cellulose fibers as versatile supports of lignin nanoparticles (LNPs) to uniformly in-situ load LNPs on the surface of fibers. The morphology, specific surface area, thermal stability, phase composition, structure and electrochemical performance of carbon fiber electrodes were investigated by X-ray diffraction, scanning electron microscopy, nitrogen adsorption, thermogravimetric analysis, X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy, and electrochemical tests, respectively. The results show that the prepared carbon fiber based electrode has a maximum specific capacitance of 7.88 F/g at an initial mass ratio of LNPs to cellulose fiber of 1∶10, which is greater than that of the control biomass carbon fiber (0.60 F/g) without loading LNPs. After 10 000-cycle test (10 A/g), the capacitance retention is still 93%. Also, LNPs loaded on the surface of fibers can effectively endow composite carbon fiber electrodes with a high specific surface area and a high carbon content, which can provides a possible path for the effective utilization of lignin in energy fields.

natural cellulose fiber  /  lignin nanoparticles  /  specific surface area  /  biomass based carbon fiber  /  electrode material  /  electrochemical performance
张伟, 安兴业, 刘利琴, 龙垠荧, 张昊, 曹海兵, 程正柏, 刘洪斌. 天然纤维/木质素纳米颗粒制备高性能多孔碳纤维电极. 硅酸盐学报, 2022 , 50 (8) : 2145 -2156 . DOI: 10.14062/j.issn.0454-5648.20220020
Wei ZHANG, Xingye AN, Liqin LIU, Yinying LONG, Hao ZHANG, Haibing CAO, Zhengbai CHENG, Hongbin LIU. Preparation of High-Performance Porous Carbon Fiber Electrode from Natural Fiber and Lignin Nanoparticles[J]. Journal of the Chinese Ceramic Society, 2022 , 50 (8) : 2145 -2156 . DOI: 10.14062/j.issn.0454-5648.20220020
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  • 国家重点研发计划项目(2019YFC1905904)
  • 国家自然科学基金项目(32101470)
  • 中国博士后基金项目(2021M692401)
  • 浙江景兴纸业股份有限公司校企合作项目
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doi: 10.14062/j.issn.0454-5648.20220020
  • 接收时间：2022-01-09
  • 首发时间：2026-10-20
  • 出版时间：2022-08-20
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  • 收稿日期：2022-01-09
  • 修回日期：2022-01-20
基金
国家重点研发计划项目(2019YFC1905904)
国家自然科学基金项目(32101470)
中国博士后基金项目(2021M692401)
浙江景兴纸业股份有限公司校企合作项目
作者信息
    1．天津科技大学轻工科学与工程学院，天津市制浆造纸重点实验室，天津 300457
    2．浙江景兴纸业股份有限公司，浙江 平湖 314214

通讯作者:

安兴业（1988—），男，博士，副教授；
刘洪斌（1977—），男，博士，研究员。
参考文献
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20220020
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2种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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