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Ultra-broadband near-infrared (NIR) luminescence of bismuth ions in glass is widely used, but the stability problem of Bi NIR centers limits its practical application. Therefore, in this work, the original local excess charge model that can effectively regulate the Bi NIR luminescence behavior was expanded and supplemented in bismuth doped yttrium aluminum-silicate glass. The statistical excess charge field around Bi was built up via either introduction of glass modifier (Y³⁺) or substitution of silicon by different glass former ions with a valence state lower than +4 (Al³⁺) in yttrium aluminumsilicate glass. As a result, the behavior of Bi NIR centers (i.e., the valence states of Bi, the intensities and peak positions of absorption and NIR emission) was determined. Also, the distribution characteristics of Bi NIR centers were proposed. Bi⁰ NIR centers are preferentially located in the multimember rings of silicon, while Bi⁺ NIR centers are situated at the interstices of silicon network. This work could solve a problem to stabilize Bi NIR centers in yttrium aluminumsilicate glass, even other alkali metals and alkali metals (Li/Na/K, Mg/Ca/Sr/Ba, etc.) aluminumsilicate glass, thus establishing the experimental and theoretical supports for the design of Bi-doped laser glasses and fabrication of fibers in future. This work also verified the effectiveness and universality of the local excess charge model, providing a strategy for stabilizing the valance state of other multivalent luminescent ions (i.e. Eu, Ce, Cu, Ag, Sn) and their distribution in glass network structure.

, authors=Xiaoman LI¹, Hai GUO², authorsList=Xiaoman LI, Hai GUO, authorCompany=null, correspAuthors=Hai GUO, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319986958634435111, articleId=1319986958131118629, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=铝硅酸盐玻璃中基于局域过剩电荷模型的Bi近红外发光调控, columnId=1321891874147775337, journalTitle=硅酸盐学报, columnName=“联合国国际玻璃年”特刊—研究论文, runingTitle=null, highlight=null, articleAbstract=

玻璃中铋离子的超宽带近红外（NIR）发光应用前景广泛，但Bi近红外中心的稳定性问题限制了其实际应用。为此，本工作以铋掺杂钇铝硅酸盐玻璃为研究对象，对可有效调控铋近红外发光行为的局域过剩电荷模型进行了补充与拓展，通过调控玻璃网络中引入的网络修饰体（Y³⁺）和低于四价的可取代Si⁴⁺的网络形成体（Al³⁺），在铋离子周围建成了局域过剩负电荷场，从而有效调控了铋离子在钇铝硅酸盐玻璃中的近红外发光行为（包括其价态、吸收和发光强度与峰位）；同时提出了Bi近红外中心的分布规律：Bi⁰主要分布在Si-O-Si/Si-O-Al网络结构多元环中，而Bi⁺主要分布在Si网络框架结构的缝隙沟道内。一方面，解决了钇铝硅酸盐玻璃，甚至其他碱金属、碱土金属（锂/钠/钾、镁/钙/锶/钡等）铝硅酸盐玻璃中铋近红外中心的稳定性问题，为铋激光玻璃的设计和后期光纤制备奠定了实验与理论基础；另一方面，也证实了局域过剩电荷模型的有效性和普适性，为其他多价态发光离子（例如Eu、Ce、Cu、Ag、Sn等）的价态稳定化和网络分布可调化提供了新思路、新方法。

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LI Xiaoman (1990-), female, Ph.D., Associate Professor. E-mail: lxmwyk668@qfnu.edu.cn

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LI Xiaoman (1990-), female, Ph.D., Associate Professor. E-mail: lxmwyk668@qfnu.edu.cn

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李晓曼（1990—），女，博士，副教授。

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李晓曼（1990—），女，博士，副教授。

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