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Article(id=1319986984798503614, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210934, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1635782400000, receivedDateStr=2021-11-02, revisedDate=1637510400000, revisedDateStr=2021-11-22, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639021347, onlineDateStr=2026-10-22, pubDate=1650384000000, pubDateStr=2022-04-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639021347, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639021347, creator=13701087609, updateTime=1792639021347, updator=13701087609, issue=Issue{id=1319986924727677753, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='4', pageStart='877', pageEnd='1200', issueExtLink='null', onlineDate='null', pubDate='1650384000000', pubDateStr='2022-04-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639007026, creator='13701087609', updateTime=1792639269665, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319988026600702366, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319988026600702367, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=975, endPage=982, ext={EN=ArticleExt(id=1319986985104687807, articleId=1319986984798503614, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Effect of Glass Network Structure on Optical Properties of CsPbI3 Perovskite Quantum Dots Glass, columnId=1321891873954837352, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on United Nations International Year of Glass—Research Articles, runingTitle=null, highlight=null, articleAbstract=

CsPbI3 quantum dots doped borosilicate glasses were prepared by a high-temperature melting-heat treatment technology with Cs2O, PbI2 and NaI as precursors. According to the results by X-ray diffraction and transmission electron microscopy, CsPbI3 quantum dots are precipitated in the glass substrate. The emission peak and absorption edge appear a red shift, the photoluminescence intensity and quantum yield firstly increase and then decrease, and the photoluminescence decay lifetime of quantum dots gradually increases with increasing the heat-treatment temperature or B2O3 concentration. Also, the two-dimensional (2D) network structure in the glass increases, and the mobility of Cs+, Pb2+ and I- ions increases with the increase of B2O3 concentration, which is beneficial for the precipitation of CsPbI3 quantum dots and the passivation of surface defect. The tunable red light emission of CsPbI3 quantum dots doped borosilicate glass could have potential applications in the visible band lasers and white light-emitting diodes (LED).

, authors=Jinhua YAN1, Jiazhi XIA1, Tao CHEN1, Tao MAN2, Zhousu XU1, Xiaofeng LIU3, Hang ZHANG1, Jianrong QIU2, authorsList=Jinhua YAN, Jiazhi XIA, Tao CHEN, Tao MAN, Zhousu XU, Xiaofeng LIU, Hang ZHANG, Jianrong QIU, authorCompany=null, correspAuthors=Zhousu XU, authorNote=

YAN Jinhua (1979-), male, Ph.D., associate Professor. E-mail:

, correspAuthorsNote=
XU Zhousu (1981-), male, Ph.D., associate Professor. E-mail:
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采用高温熔融-热处理技术，以Cs2O、PbI2和NaI为CsPbI3量子点前驱体，制备了CsPbI3量子点掺杂硼硅酸盐玻璃。X射线衍射和透射电镜观察表明，在玻璃内部析出了CsPbI3量子点。随热处理温度上升或B2O3含量的增加，发光峰和吸收边出现红移，荧光强度和量子产率先增大后减小，量子点的荧光衰减寿命逐渐增长。进一步分析表明，随着B2O3含量增大，玻璃中二维（2D）网络结构增多，Cs+、Pb2+和I-移动能力增强，有利于CsPbI3量子点析出和表面缺陷钝化。CsPbI3量子点掺杂硼硅酸盐玻璃的可调谐红光发射，在可见波段激光器和白光LED等领域具有潜在应用。

, authors=严金华1, 夏家志1, 陈涛1, 满涛2, 许周速1, 刘小峰3, 张航1, 邱建荣2, authorsList=严金华, 夏家志, 陈涛, 满涛, 许周速, 刘小峰, 张航, 邱建荣, authorCompany=null, correspAuthors=许周速, authorNote=

严金华（1979—），男，博士，副教授。

, correspAuthorsNote=
许周速（1981—），男，博士，副教授。
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YAN Jinhua (1979-), male, Ph.D., associate Professor. E-mail:

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YAN Jinhua (1979-), male, Ph.D., associate Professor. E-mail:

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严金华（1979—），男，博士，副教授。

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严金华（1979—），男，博士，副教授。

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玻璃网络结构对CsPbI3钙钛矿量子点玻璃光学性质的影响
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严金华 1 , 夏家志 1 , 陈涛 1 , 满涛 2 , 许周速 1 , 刘小峰 3 , 张航 1 , 邱建荣 2
硅酸盐学报 | “联合国国际玻璃年”特刊—研究论文 2022,50(4): 975-982
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硅酸盐学报 |“联合国国际玻璃年”特刊—研究论文 2022 , 50 (4) : 975 -982
玻璃网络结构对CsPbI3钙钛矿量子点玻璃光学性质的影响
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YAN Jinhua (1979-), male, Ph.D., associate Professor. E-mail:

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YAN Jinhua (1979-), male, Ph.D., associate Professor. E-mail:

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严金华（1979—），男，博士，副教授。

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严金华（1979—），男，博士，副教授。

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严金华1 , 夏家志1, 陈涛1, 满涛2, 许周速1 , 刘小峰3, 张航1, 邱建荣2
作者信息
  • 1．浙江工业大学光电子智能化技术研究所，杭州 310023
  • 2．浙江大学光电科学与工程学院，杭州 310027
  • 3．浙江大学材料科学与工程学院，杭州 310027
通讯作者:
许周速（1981—），男，博士，副教授。
作者简介:

严金华（1979—），男，博士，副教授。

Effect of Glass Network Structure on Optical Properties of CsPbI3 Perovskite Quantum Dots Glass
Jinhua YAN1 , Jiazhi XIA1, Tao CHEN1, Tao MAN2, Zhousu XU1 , Xiaofeng LIU3, Hang ZHANG1, Jianrong QIU2
Affiliations
  • 1.Institute of Intelligent Optoelectronic Technology, Zhejiang University of Technology, Hangzhou 310014, China
  • 2.College of Optical Science and Engineering, Zhejiang University, Hangzhou 310027, China
  • 3.School of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China
    • Corresponding Author:
    XU Zhousu (1981-), male, Ph.D., associate Professor. E-mail:

    YAN Jinhua (1979-), male, Ph.D., associate Professor. E-mail:

出版时间: 2022-04-20 doi: 10.14062/j.issn.0454-5648.20210934
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采用高温熔融-热处理技术，以Cs2O、PbI2和NaI为CsPbI3量子点前驱体，制备了CsPbI3量子点掺杂硼硅酸盐玻璃。X射线衍射和透射电镜观察表明，在玻璃内部析出了CsPbI3量子点。随热处理温度上升或B2O3含量的增加，发光峰和吸收边出现红移，荧光强度和量子产率先增大后减小，量子点的荧光衰减寿命逐渐增长。进一步分析表明，随着B2O3含量增大，玻璃中二维（2D）网络结构增多，Cs+、Pb2+和I-移动能力增强，有利于CsPbI3量子点析出和表面缺陷钝化。CsPbI3量子点掺杂硼硅酸盐玻璃的可调谐红光发射，在可见波段激光器和白光LED等领域具有潜在应用。

量子点  /  玻璃网络结构  /  硼硅酸盐玻璃  /  析晶

CsPbI3 quantum dots doped borosilicate glasses were prepared by a high-temperature melting-heat treatment technology with Cs2O, PbI2 and NaI as precursors. According to the results by X-ray diffraction and transmission electron microscopy, CsPbI3 quantum dots are precipitated in the glass substrate. The emission peak and absorption edge appear a red shift, the photoluminescence intensity and quantum yield firstly increase and then decrease, and the photoluminescence decay lifetime of quantum dots gradually increases with increasing the heat-treatment temperature or B2O3 concentration. Also, the two-dimensional (2D) network structure in the glass increases, and the mobility of Cs+, Pb2+ and I- ions increases with the increase of B2O3 concentration, which is beneficial for the precipitation of CsPbI3 quantum dots and the passivation of surface defect. The tunable red light emission of CsPbI3 quantum dots doped borosilicate glass could have potential applications in the visible band lasers and white light-emitting diodes (LED).

quantum dots  /  glass network structure  /  borosilicate glass  /  crystallization
严金华, 夏家志, 陈涛, 满涛, 许周速, 刘小峰, 张航, 邱建荣. 玻璃网络结构对CsPbI3钙钛矿量子点玻璃光学性质的影响. 硅酸盐学报, 2022 , 50 (4) : 975 -982 . DOI: 10.14062/j.issn.0454-5648.20210934
Jinhua YAN, Jiazhi XIA, Tao CHEN, Tao MAN, Zhousu XU, Xiaofeng LIU, Hang ZHANG, Jianrong QIU. Effect of Glass Network Structure on Optical Properties of CsPbI3 Perovskite Quantum Dots Glass[J]. Journal of the Chinese Ceramic Society, 2022 , 50 (4) : 975 -982 . DOI: 10.14062/j.issn.0454-5648.20210934
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  • 浙江省自然科学基金(LY21F050005; LR21E020005)
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doi: 10.14062/j.issn.0454-5648.20210934
  • 接收时间：2021-11-02
  • 首发时间：2026-10-22
  • 出版时间：2022-04-20
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  • 收稿日期：2021-11-02
  • 修回日期：2021-11-22
基金
浙江省自然科学基金(LY21F050005; LR21E020005)
作者信息
    1．浙江工业大学光电子智能化技术研究所，杭州 310023
    2．浙江大学光电科学与工程学院，杭州 310027
    3．浙江大学材料科学与工程学院，杭州 310027

通讯作者:

许周速（1981—），男，博士，副教授。
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Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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