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Solid-state lithium batteries with solid electrolytes are expected to enhance the battery safety and energy density as one of the most promising next-generation batteries. Among various solid-state electrolytes, sulfide solid electrolyte is considered as promising candidate due to its ultra-high ionic conductivity. However, its large-scale production is restricted due to its fragility and difficulty in processing, which affects its application in solid-state batteries. Recent work indicates that the flexibility of solid electrolytes can be realized via introducing flexible polymers or supporting frameworks in solid electrolytes membranes, constituting a solution to the embrittlement challenge in large-scale and thin-film electrolyte preparations. Therefore, developing flexible solid electrolytes is one of the important strategies to promote the industrialization of solid-state batteries. This review introduced the physical/chemical properties and development of sulfide solid electrolytes, summarized the related research work on polymer self-supporting method and flexible skeleton-supporting method in the flexibility of solid electrolytes, and discussed the technical characteristics and advantages/disadvantages of wet/dry processes in the flexible sulfide solid electrolyte preparation, respectively. In addition, the future development aspects were also given to promote the practical application of solid-state lithium batteries.

, authors=Jiangkui HU^{1, 2}, Hong YUAN^{1, 2}, Chenzi ZHAO³, Yang LU³, Shuo SUN³, Jiaqi HUANG^{1, 2}, authorsList=Jiangkui HU, Hong YUAN, Chenzi ZHAO, Yang LU, Shuo SUN, Jiaqi HUANG, authorCompany=null, correspAuthors=Hong YUAN, Jiaqi HUANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319987185282040369, articleId=1319987184787112495, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=柔性硫化物固态电解质研究进展, columnId=1321891336442196302, journalTitle=硅酸盐学报, columnName=电化学储能材料专题—综合评述, runingTitle=null, highlight=null, articleAbstract=

采用固态电解质的固态锂电池有望从根本上提高电池的安全性能及能量密度，被认为是最具应用前景的下一代电池技术之一。在诸多固态电解质中，硫化物固态电解质由于超高的离子电导率被认为最具实用化前景，但固态电解质膜易碎、难以加工等问题严重阻碍了其在固态电池中的应用。近年来，大量研究成果表明在固态电解质中引入柔性聚合物或柔性支撑载体等可以实现固态电解质膜的柔性化，从而可以解决固态电解质在规模化、薄膜化制备过程中脆裂问题。因此，固态电解质柔性化是推动固态电池工业化的重要解决方案之一。首先介绍了硫化物固态电解质的理化性质及发展历程，随后，总结了聚合物自支撑方法与柔性骨架支撑策略在固态电解质柔性化方面的研究进展，并分别讨论了湿法和干法工艺在硫化物固态电解质柔性化方面的技术特点和优劣，最后对未来发展趋势进行了展望，旨在进一步推动固态锂电池迈向实用化。

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