Article(id=1319987158836953400, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210620, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1627488000000, receivedDateStr=2021-07-29, revisedDate=1629993600000, revisedDateStr=2021-08-27, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639062842, onlineDateStr=2026-10-22, pubDate=1642608000000, pubDateStr=2022-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639062842, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639062842, creator=13701087609, updateTime=1792639062842, updator=13701087609, issue=Issue{id=1319987091220574321, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='1', pageStart='1', pageEnd='276', issueExtLink='null', onlineDate='null', pubDate='1642608000000', pubDateStr='2022-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639046721, creator='13701087609', updateTime=1792639238958, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319987897588105574, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319987897588105575, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=26, endPage=36, ext={EN=ArticleExt(id=1319987159038279993, articleId=1319987158836953400, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=BiCl₃-Regulated and ZIF8-Derived Hierarchical Porous Carbon as Anode for High-Performance Soudium-Ion Batteries, columnId=1321891465115062324, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Electrochemical Energy Storage Materials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

To improve the rate capability of hard carbon (HC), the corresponding hierarchical porous morphology was designed and the metal organic framework (ZIF-8) was selected as a precursor, and the hierarchical pore structure was adjusted via the addition of BiCl₃. The results show that the synthesized hierarchical structure of HC electrodes can effectively improve the diffusion of Na ions. The synthesized hierarchical porous hard carbon can achieve a high reversible capacity of 225 mA·h/g and 177 mA·h/g at different currents of 2 A/g and 5 A/g, respectively, based on the optimized micro- and macro-pores. Furthermore, a relationship between the hierarchical porous structure (with micro- and macro-pores) and the sodium storage process was discussed. It is indicated that the micro-pores prefer to facilitate the sodium-ion diffusion in a plateau region, while the meso-pores prefer to provide more defect sites to enhance the adsorption of sodium ions, consequently improving the sodium storage capacity.

, authors=Yi WAN^{1, 2}, Pengfei YAO^{1, 2}, Huamin ZHANG¹, Qiong ZHENG¹, Xianfeng LI¹, authorsList=Yi WAN, Pengfei YAO, Huamin ZHANG, Qiong ZHENG, Xianfeng LI, authorCompany=null, correspAuthors=Qiong ZHENG, Xianfeng LI, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319987160846025018, articleId=1319987158836953400, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=基于BiCl₃调控、ZIF-8转化的分级多孔硬碳结构设计及在钠离子电池中的应用, columnId=1321891465291223093, journalTitle=硅酸盐学报, columnName=电化学储能材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

从微观多孔结构设计的角度出发，以ZIF-8为碳化前驱体，采用BiCl₃对硬碳微孔、介孔结构进行调控，实现了分级多孔硬碳结构的可控设计与调控优化，有效提高了Na⁺的扩散能力，提高了钠离子动力学。结果表明：该分级多孔碳表现出优异的倍率性能，在2 A/g和5A/g时，可逆比容量分别为225 mA·h/g和177 mA·h/g。通过分级多孔硬碳微孔和介孔结构对储钠过程影响机制的研究发现，微孔结构有利于平台区Na⁺的扩散；介孔结构主要通过增大比表面提供更多的缺陷位点，促进Na⁺的吸附，提升斜线区储钠容量。

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WAN Yi (1996-), male, Master candidate. E-mail: wanyi@dicp.ac.cn

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WAN Yi (1996-), male, Master candidate. E-mail: wanyi@dicp.ac.cn

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万意（1996—），男，硕士研究生。

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万意（1996—），男，硕士研究生。

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