Article(id=1319987134564520185, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210615, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1627833600000, receivedDateStr=2021-08-02, revisedDate=1633536000000, revisedDateStr=2021-10-07, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639057054, onlineDateStr=2026-10-22, pubDate=1642608000000, pubDateStr=2022-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639057054, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639057054, creator=13701087609, updateTime=1792639057054, updator=13701087609, issue=Issue{id=1319987091220574321, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='1', pageStart='1', pageEnd='276', issueExtLink='null', onlineDate='null', pubDate='1642608000000', pubDateStr='2022-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639046721, creator='13701087609', updateTime=1792639238958, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319987897588105574, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319987897588105575, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2, endPage=8, ext={EN=ArticleExt(id=1319987134803595514, articleId=1319987134564520185, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Synthesis and Sodium Storage Performance of Highly Stable Vanadium Sulfide Microsphere Anodes, columnId=1321891465115062324, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Electrochemical Energy Storage Materials—Research Articles, runingTitle=null, highlight=null, articleAbstract=

VS₄ has an one-dimensional chain structure with the chain spacing of 0.583 nm, which is greater than Na⁺ ion radius of 0.102 nm. Moreover, its theoretical sodium storage capacity is 1 196 mA·h/g, making it one of the most promising anode materials for sodium storage. However, the volume of the electrode material expands and contracts dramatically during repeated cycling, resulting in collapse of the structure, poor cycling stability and capacity decay, and severely affecting the practical application of VS₄. In this paper, VS₄ microspheres (approximately 1 μm in diameter) with a high stability were constructed for the unique three-dimensional microsphere structure to alleviate the volume expansion, improve the cycling stability and the electrochemical reaction kinetics. This microsphere structured material as an anode material for sodium ion batteries exhibits a superior rate performance (i.e., 372 mA·h/g@2.0 A/g and 297 mA·h/g@5.0 A/g) and a long-cycle life (i.e., stable cycling for 100 times at 5.0 A/g).

, authors=Siling CHENG, Wei LUO, Kunxiong ZHENG, Xianhong RUI, authorsList=Siling CHENG, Wei LUO, Kunxiong ZHENG, Xianhong RUI, authorCompany=null, correspAuthors=Xianhong RUI, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319987135030087931, articleId=1319987134564520185, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=高稳定性微球结构硫化钒负极材料的合成与储钠性能, columnId=1321891465291223093, journalTitle=硅酸盐学报, columnName=电化学储能材料专题—研究论文, runingTitle=null, highlight=null, articleAbstract=

VS₄是极具发展前景的储钠负极材料之一，它具有一维链状结构，链间距远大于钠离子半径（0.583 nm vs. 0.102 nm），且理论储钠容量高达1 196 mA·h/g。然而，在反复的充放电循环过程中，该电极材料体积会发生剧烈地膨胀收缩，最终导致结构崩塌，电池循环稳定性差、容量衰减等问题，严重限制了VS₄的实际应用。为此，提出构筑高稳定性微球结构VS₄（直径约1 μm）。独特的三维微球结构，可以缓解体积膨胀，提高循环稳定性，改善电化学反应动力学。当用作钠离子电池负极材料时，电池表现出优异的倍率性能（372 mA·h/g@2.0 A/g和297 mA·h/g@5.0 A/g）和长循环稳定性（5.0 A/g下稳定循环100圈）。

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CHENG Siling (1996-), male, Master candidate. E-mail: Siling_Cheng0619@163.com

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CHENG Siling (1996-), male, Master candidate. E-mail: Siling_Cheng0619@163.com

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程肆灵（1996—），男，硕士研究生。

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程肆灵（1996—），男，硕士研究生。

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