Article(id=1319987152948154778, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210514, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1624809600000, receivedDateStr=2021-06-28, revisedDate=1628611200000, revisedDateStr=2021-08-11, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639061437, onlineDateStr=2026-10-22, pubDate=1642608000000, pubDateStr=2022-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639061437, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639061437, creator=13701087609, updateTime=1792639061437, updator=13701087609, issue=Issue{id=1319987091220574321, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='1', pageStart='1', pageEnd='276', issueExtLink='null', onlineDate='null', pubDate='1642608000000', pubDateStr='2022-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639046721, creator='13701087609', updateTime=1792639238958, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319987897588105574, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319987897588105575, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987091220574321, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=219, endPage=225, ext={EN=ArticleExt(id=1319987153183035803, articleId=1319987152948154778, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Stable High-Entropy Double Perovskite Cathode SmBa(Mn_0.2Fe_0.2Co_0.2Ni_0.2Cu_0.2)₂O_5+δ for Intermediate-Temperature Solid Oxide Fuel Cells, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

High-entropy double perovskite SmBa(Mn_0.2Fe_0.2Co_0.2Ni_0.2Cu_0.2)₂O_5+δ (HE-SBC) as a cathode material was prepared by a modified Pechini method, and the performance of HE-SBC with 10% (in mole fraction) Gd₂O₃-doped CeO₂ (GDC) (HE-SBC-GDC) was optimized. The results show that the thermal expansion of Co ions caused by the change of valence state can be reduced due to the formation of high-entropy at B-site, thereby reducing the thermal expansion coefficient of SBC. The polarization impedance (R_p) of the HE-SBC symmetrical cell with yttria-stabilized zirconia (YSZ) as an electrolyte is 1.04 Ω·cm² at 800 ℃ and the maximum power density and R_p of the anode-supported single cell are 683.53 mW/cm² and 0.46 Ω·cm², respectively. Furthermore, the catalytic activity of HE-SBC is improved by the addition of GDC[m(HE-SBC):m(GDC)=7:3] due to the enlarged three-phase interface. The polarization resistance of HE-SBC-GDC composite cathode symmetric cell is only 0.09 Ω·cm² at 800 ℃ and the maximum power density and R_p of the anode-supported single cell are 838.66 mW/cm² and 0.12 Ω·cm², respectively.

, authors=Yihan LING¹, Xu HAN¹, Yang YANG^{1, 2}, Tianqiang LIN¹, Xinxin WANG¹, Xuemei OU¹, Shaorong WANG², authorsList=Yihan LING, Xu HAN, Yang YANG, Tianqiang LIN, Xinxin WANG, Xuemei OU, Shaorong WANG, authorCompany=null, correspAuthors=null, authorNote=, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319987153413722524, articleId=1319987152948154778, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=高熵稳定双钙钛矿阴极材料SmBa(Mn_0.2Fe_0.2Co_0.2Ni_0.2Cu_0.2)₂O_5+δ的制备及性能优化, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

通过改进的自蔓延燃烧法合成制备高熵双钙钛矿SmBa（Mn_0.2Fe_0.2Co_0.2Ni_0.2Cu_0.2）₂O_5+δ（HE-SBC）阴极材料，并复合10%（摩尔分数）Gd₂O₃掺杂CeO₂（GDC）以优化性能。结果表明：通过B位高熵的方法可以显著减小Co离子由价态变化而引起的热膨胀，从而降低SmBaCo₂O_5+δ的热膨胀系数。在800 ℃，以氧化钇稳定氧化锆（YSZ）为电解质的HE-SBC对称电池的极化阻抗（R_p）为1.04Ω·cm²，阳极支撑单电池的最高功率密度和R_p分别为683.53 mW/cm²和0.46Ω·cm²。进一步通过复合GDC（HE-SBC与GDC的质量比7：3）以增加三相界面提高HE-SBC的催化活性，在800 ℃ HE-SBC-GDC复合阴极对称电池的极化阻抗仅为0.09Ω·cm²，且阳极支撑单电池的最高功率密度和R_p分别为838.66 mW/cm²和0.12Ω·cm²。

, authors=凌意瀚¹, 韩绪¹, 杨洋^{1, 2}, 林添强¹, 王鑫鑫¹, 欧雪梅¹, 王绍荣², authorsList=凌意瀚, 韩绪, 杨洋, 林添强, 王鑫鑫, 欧雪梅, 王绍荣, authorCompany=null, correspAuthors=null, authorNote=, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=0ugoiqcSn1AEkeVcNmjexw==, magXml=OxYAowgC1n0NH8veIhQ4BQ==, pdfUrl=null, pdf=3/JWrHKFhAb6PpaHRM4l8w==, pdfFileSize=1311856, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=77CxNpLHJXqRCEZOPa5CJA==, mapNumber=null, fund=null)}, authors=[Author(id=1322507154075009182, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319987152948154778, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=lyhyy@cumt.edu.cn, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1322507154158895264, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319987152948154778, authorId=1322507154075009182, language=EN, stringName=Yihan LING, firstName=Yihan, middleName=null, lastName=LING, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.School of Materials Science and Physics, China University of Mining and Technology, Xuzhou 221116, Jiangsu, China, bio={"content":"

LING Yihan (1986-), male, Ph.D., Professor. E-mail: lyhyy@cumt.edu.cn

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LING Yihan (1986-), male, Ph.D., Professor. E-mail: lyhyy@cumt.edu.cn

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凌意瀚（1986—），男，博士，研究员。

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凌意瀚（1986—），男，博士，研究员。

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