Article(id=1322942667830735865, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942634976752425, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210035, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1610380800000, receivedDateStr=2021-01-12, revisedDate=1612281600000, revisedDateStr=2021-02-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343711097, onlineDateStr=2026-10-30, pubDate=1626710400000, pubDateStr=2021-07-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343711097, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343711097, creator=13701087609, updateTime=1793343711097, updator=13701087609, issue=Issue{id=1322942634976752425, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='7', pageStart='1249', pageEnd='1518', issueExtLink='null', onlineDate='null', pubDate='1626710400000', pubDateStr='2021-07-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343703264, creator='13701087609', updateTime=1793345819416, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322951510828659213, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942634976752425, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322951510828659214, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942634976752425, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1403, endPage=1411, ext={EN=ArticleExt(id=1322942668032062458, articleId=1322942667830735865, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Monoclinic Pyrrhotite Derived from Pyrite through Thermal Decomposition to Activate PDS for the Degradation of Oxytetracycline, columnId=1322942641213682516, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Mineral Material, runingTitle=null, highlight=null, articleAbstract=

Monoclinic pyrrhotite (M-Pyr) was derived from pyrite through thermal decomposition in nitrogen atmosphere with controlled temperature and time, which was used to activate sodium persulfate (PDS) for the degradation of oxytetracycline (OTC). The effects of initial concentration of OTC, initial solution pH value, contents of PDS and M-Pyr on OTC degradation were studied. The contents of PDS and M-Pyr had a positive effect on the OTC removal rate, while the effect of the initial OTC concentration was negative. Specifically, 99% of OTC was degraded in the M-Pyr/PDS system with pH=6-7, ρ (M-Pyr) =0.1 g/L and c(PDS)=1.0 mmol/L. The removal rate of OTC was 86.5% after recycling for two times, where the relatively poor recyclability might be attributed to the corrosion of M-Pyr and the formation of intermediate product to occupy the active sites. Sulfate radical and hydroxyl radical were the main active species in the M-Pyr/PDS system.

, authors=Meng LIU, Hanlin WANG, Haibo LIU, Tianhu CHEN, Xuehua ZOU, Fuwei SUN, Ziyang CHU, Peixun ZHAI, Dong CHEN, authorsList=Meng LIU, Hanlin WANG, Haibo LIU, Tianhu CHEN, Xuehua ZOU, Fuwei SUN, Ziyang CHU, Peixun ZHAI, Dong CHEN, authorCompany=null, correspAuthors=Haibo LIU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322942668266943483, articleId=1322942667830735865, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=热分解黄铁矿制备单斜磁黄铁矿活化PDS降解土霉素, columnId=1322942641389843286, journalTitle=硅酸盐学报, columnName=矿物材料专题, runingTitle=null, highlight=null, articleAbstract=

通过控制氮气气氛下黄铁矿热分解的温度和时间，制备单斜磁黄铁矿（M-Pyr），用于活化过二硫酸钠（PDS）降解土霉素（OTC）。考察了OTC初始浓度、溶液初始pH值、PDS和M-Pyr剂量对降解效果的影响。结果表明：M-Pyr/PDS体系对OTC的去除率与PDS和M-Pyr的量成正相关，与OTC初始浓度成负相关，当pH=6或7，ρ（M-Pyr）=0.1 g/L，c（PDS）=1 mmol/L时，初始浓度为20 mg/L的OTC降解率可达99%以上。M-Pyr在重复2次使用后，对OTC的去除率为86.5%，其循环使用效果不佳的原因是M-Pyr溶蚀以及中间产物占据活性位点。通过淬灭实验可知，在M-Pyr/PDS体系中硫酸根自由基和羟基自由基是主要的活性物种。黄铁矿热分解产生的M-Pyr可有效活化PDS降解土霉素。

, authors=刘梦, 王汉林, 刘海波, 陈天虎, 邹雪华, 孙付炜, 储梓杨, 翟沛勋, 陈冬, authorsList=刘梦, 王汉林, 刘海波, 陈天虎, 邹雪华, 孙付炜, 储梓杨, 翟沛勋, 陈冬, authorCompany=null, correspAuthors=刘海波, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=LOvP9E6cDcsz12O5SMiD7g==, magXml=vVf/+Gr/WZyC7S1cC5x91A==, pdfUrl=null, pdf=1xc37DAs5WEOtq1o+1ADlQ==, pdfFileSize=2699787, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=/nYrOypVx+r2cnCmxRiscQ==, mapNumber=null, fund=null)}, authors=[Author(id=1322942668531184640, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1322942667830735865, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=1051138322@qq.com, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1322942668615069697, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1322942667830735865, authorId=1322942668531184640, language=EN, stringName=Meng LIU, firstName=Meng, middleName=null, lastName=LIU, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=Key Laboratory of Nano-minerals and Pollution Control of Anhui Higher Education Institutes, School of Resources & Environmental Engineering, Hefei University of Technology, Hefei 230009, China, bio={"content":"

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LIU Meng(1996-), female, Master candidate. E-mail: 1051138322@qq.com

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刘梦（1996—），女，硕士研究生。

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刘梦（1996—），女，硕士研究生。

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