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Article(id=1322942447193567478, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942446610559222, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200882, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1606233600000, receivedDateStr=2020-11-25, revisedDate=1608134400000, revisedDateStr=2020-12-17, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343658492, onlineDateStr=2026-10-30, pubDate=1613750400000, pubDateStr=2021-02-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343658492, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343658492, creator=13701087609, updateTime=1793343658492, updator=13701087609, issue=Issue{id=1322942446610559222, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='2', pageStart='211', pageEnd='440', issueExtLink='null', onlineDate='null', pubDate='1613750400000', pubDateStr='2021-02-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343658354, creator='13701087609', updateTime=1793345474672, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322950064863314723, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942446610559222, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322950064863314724, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942446610559222, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=272, endPage=284, ext={EN=ArticleExt(id=1322942447394894071, articleId=1322942447193567478, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Research Progress on Structure-Performance Relationship for Novel 'Quasi-Crystalline' Thermoelectric Compounds in Sublattice Engineering, columnId=1319987100586459893, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Inerim Achievements of Key Program of National Natural Science Foundation of China, runingTitle=null, highlight=null, articleAbstract=

Thermoelectric materials as novel clean energy materials have application prospects in waste-heat recovery and solid-state refrigeration. The thermoelectric compounds evolve from simple unitary- or binary-component crystalline systems to multinary complex systems. Among them, the multinary diamond-like compounds, the compounds with distinct sublattice and chemical bond hierarchy characteristics and their derivatives exhibit a complex crystalline-amorphous hybrid behavior in an atomic scale and present some transport effects, providing a prospect for the exploration of effects of electrical-thermal transport and systems of thermoelectric materials. This review summarized recent research progress on thermoelectric materials in sublattice engineering, including the structural design of novel "quasi-crystalline" thermoelectric compounds, the optimization of thermoelectric property and the characterization of microstructures in a sublattice scale. In addition, the relationship between the crystalline-semi-crystalline sublattice structure and the thermoelectric property of the compound was also discussed.

, authors=Jiye ZHANG1, Yue LI1, Haojie HUO1, Shanshan PAN1, Lin XIE3, Kai GUO1, Jiong YANG2, Jiaqing HE3, Jun LUO1, 2, Wenqing ZHANG2, 3, authorsList=Jiye ZHANG, Yue LI, Haojie HUO, Shanshan PAN, Lin XIE, Kai GUO, Jiong YANG, Jiaqing HE, Jun LUO, Wenqing ZHANG, authorCompany=null, correspAuthors=Jiaqing HE, Jun LUO, Wenqing ZHANG, authorNote=

ZHANG Jiye (1980-), male, Professor. E-mail:

, correspAuthorsNote=
LUO Jun (1976-), male, Professor; E-mail:
HE Jiaqing (1974-), male, Professor;
ZHANG Wenqing (1966-), male, Professor.
, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322942447684301049, articleId=1322942447193567478, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=亚晶格工程与新型“半晶态”热电化合物结构-性能关系研究进展, columnId=1322942447482974456, journalTitle=硅酸盐学报, columnName=国家自然科学基金重点项目中期成果专题, runingTitle=null, highlight=null, articleAbstract=

热电材料作为新型的清洁能源材料，在固态制冷和余/废热回收等领域有着广泛的应用前景。随着研究的逐步深入，热电化合物从简单的一元和二元组分的晶态体系逐渐转向多元复杂体系。多元类金刚石化合物以及具有明显亚晶格特征和层级化学键的化合物及其衍生物，在原子尺度上表现出复杂的晶态-非晶态共存行为，并产生了新颖的输运效应，这些都为电-热输运新效应和热电材料新体系探索提供了广阔的空间。综述了近年来在亚晶格工程思路下新型“半晶态”热电化合物的结构设计、热电性能调控以及亚晶格尺度上微结构精细表征方面的研究进展，并讨论了晶态-半晶态亚晶格结构与化合物热电性能的关系。

, authors=张继业1, 李悦1, 霍豪杰1, 潘山山1, 谢琳3, 郭凯1, 杨炯2, 何佳清3, 骆军1, 2, 张文清2, 3, authorsList=张继业, 李悦, 霍豪杰, 潘山山, 谢琳, 郭凯, 杨炯, 何佳清, 骆军, 张文清, authorCompany=null, correspAuthors=何佳清, 骆军, 张文清, authorNote=

张继业（1980—），男，教授。

, correspAuthorsNote=
骆军（1976—），男，教授；
何佳清（1974—），男，教授；
张文清（1966—），男，教授。
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ZHANG Jiye (1980-), male, Professor. E-mail:

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张继业（1980—），男，教授。

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张继业（1980—），男，教授。

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亚晶格工程与新型“半晶态”热电化合物结构-性能关系研究进展
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张继业 1 , 李悦 1 , 霍豪杰 1 , 潘山山 1 , 谢琳 3 , 郭凯 1 , 杨炯 2 , 何佳清 3 , 骆军 1, 2 , 张文清 2, 3
硅酸盐学报 | 国家自然科学基金重点项目中期成果专题 2021,49(2): 272-284
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硅酸盐学报 |国家自然科学基金重点项目中期成果专题 2021 , 49 (2) : 272 -284
亚晶格工程与新型“半晶态”热电化合物结构-性能关系研究进展
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张继业1 , 李悦1, 霍豪杰1, 潘山山1, 谢琳3, 郭凯1, 杨炯2, 何佳清3 , 骆军1, 2 , 张文清2, 3
作者信息
  • 1．上海大学材料科学与工程学院，上海 200444
  • 2．上海大学材料基因组工程研究院，上海 200444
  • 3．南方科技大学物理系，深圳量子科学与工程研究院，广东 深圳 518055
通讯作者:
骆军（1976—），男，教授；
何佳清（1974—），男，教授；
张文清（1966—），男，教授。
作者简介:

张继业（1980—），男，教授。

Research Progress on Structure-Performance Relationship for Novel 'Quasi-Crystalline' Thermoelectric Compounds in Sublattice Engineering
Jiye ZHANG1 , Yue LI1, Haojie HUO1, Shanshan PAN1, Lin XIE3, Kai GUO1, Jiong YANG2, Jiaqing HE3 , Jun LUO1, 2 , Wenqing ZHANG2, 3
Affiliations
  • 1.School of Materials Science and Engineering, Shanghai University, Shanghai 200444, China
  • 2.Materials Genome Institute, Shanghai University, Shanghai 200444, China
  • 3.Department of Physics and Shenzhen Institute for Quantum Science & Technology, Southern University of Science and Technology, Shenzhen 518055, Guangdong, China
    • Corresponding Author:
    LUO Jun (1976-), male, Professor; E-mail:
    HE Jiaqing (1974-), male, Professor;
    ZHANG Wenqing (1966-), male, Professor.

    ZHANG Jiye (1980-), male, Professor. E-mail:

出版时间: 2021-02-20 doi: 10.14062/j.issn.0454-5648.20200882
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热电材料作为新型的清洁能源材料，在固态制冷和余/废热回收等领域有着广泛的应用前景。随着研究的逐步深入，热电化合物从简单的一元和二元组分的晶态体系逐渐转向多元复杂体系。多元类金刚石化合物以及具有明显亚晶格特征和层级化学键的化合物及其衍生物，在原子尺度上表现出复杂的晶态-非晶态共存行为，并产生了新颖的输运效应，这些都为电-热输运新效应和热电材料新体系探索提供了广阔的空间。综述了近年来在亚晶格工程思路下新型“半晶态”热电化合物的结构设计、热电性能调控以及亚晶格尺度上微结构精细表征方面的研究进展，并讨论了晶态-半晶态亚晶格结构与化合物热电性能的关系。

热电材料  /  亚晶格工程  /  类金刚石  /  半晶态

Thermoelectric materials as novel clean energy materials have application prospects in waste-heat recovery and solid-state refrigeration. The thermoelectric compounds evolve from simple unitary- or binary-component crystalline systems to multinary complex systems. Among them, the multinary diamond-like compounds, the compounds with distinct sublattice and chemical bond hierarchy characteristics and their derivatives exhibit a complex crystalline-amorphous hybrid behavior in an atomic scale and present some transport effects, providing a prospect for the exploration of effects of electrical-thermal transport and systems of thermoelectric materials. This review summarized recent research progress on thermoelectric materials in sublattice engineering, including the structural design of novel "quasi-crystalline" thermoelectric compounds, the optimization of thermoelectric property and the characterization of microstructures in a sublattice scale. In addition, the relationship between the crystalline-semi-crystalline sublattice structure and the thermoelectric property of the compound was also discussed.

thermoelectric materials  /  sublattice engineering  /  diamond-like  /  liquid-like
张继业, 李悦, 霍豪杰, 潘山山, 谢琳, 郭凯, 杨炯, 何佳清, 骆军, 张文清. 亚晶格工程与新型“半晶态”热电化合物结构-性能关系研究进展. 硅酸盐学报, 2021 , 49 (2) : 272 -284 . DOI: 10.14062/j.issn.0454-5648.20200882
Jiye ZHANG, Yue LI, Haojie HUO, Shanshan PAN, Lin XIE, Kai GUO, Jiong YANG, Jiaqing HE, Jun LUO, Wenqing ZHANG. Research Progress on Structure-Performance Relationship for Novel 'Quasi-Crystalline' Thermoelectric Compounds in Sublattice Engineering[J]. Journal of the Chinese Ceramic Society, 2021 , 49 (2) : 272 -284 . DOI: 10.14062/j.issn.0454-5648.20200882
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  • 国家自然科学基金重点项目(51632005)
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2021年第49卷第2期
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doi: 10.14062/j.issn.0454-5648.20200882
  • 接收时间：2020-11-25
  • 首发时间：2026-10-30
  • 出版时间：2021-02-20
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  • 收稿日期：2020-11-25
  • 修回日期：2020-12-17
基金
国家自然科学基金重点项目(51632005)
作者信息
    1．上海大学材料科学与工程学院，上海 200444
    2．上海大学材料基因组工程研究院，上海 200444
    3．南方科技大学物理系，深圳量子科学与工程研究院，广东 深圳 518055

通讯作者:

骆军（1976—），男，教授；
何佳清（1974—），男，教授；
张文清（1966—），男，教授。
参考文献
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20200882
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2种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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