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Article(id=1322943260393612146, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942627649303277, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200792, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1603209600000, receivedDateStr=2020-10-21, revisedDate=1604332800000, revisedDateStr=2020-11-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343852374, onlineDateStr=2026-10-30, pubDate=1624118400000, pubDateStr=2021-06-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343852374, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343852374, creator=13701087609, updateTime=1793343852374, updator=13701087609, issue=Issue{id=1322942627649303277, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='6', pageStart='1033', pageEnd='1246', issueExtLink='null', onlineDate='null', pubDate='1624118400000', pubDateStr='2021-06-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343701517, creator='13701087609', updateTime=1793345989266, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322952223231181603, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942627649303277, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322952223231181604, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942627649303277, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1185, endPage=1194, ext={EN=ArticleExt(id=1322943260599133044, articleId=1322943260393612146, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Adsorption of Methylene Blue by Modified Tobermorite, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

Modified tobermorillonite (AHTOB) with a specific surface area of 570 m2/g was prepared by heating and acidification of tobermorillonite (TOB). The structure and specific surface area and pore size of the modified tobermorillonite were characterized by X-ray diffraction and N2 adsorption-desorption. The adsorption properties of three adsorbents on methylene blue solution (MB) were investigated by static adsorption experiments, and the adsorption mechanism of modified TOB on MB was analyzed. The effects of adsorbents, solution pH value, initial MB concentration, adsorption time, and temperature on the adsorption behavior were investigated, and the thermodynamic and kinetic behaviors of AHTOB adsorbed on MB solution were investigated. The adsorption of MB was analyzed in 50 mL of MB at a concentration of 10 mg/L. The results show that the adsorption rates of unmodified TOB, HTOB, and AHTOB on MB are 50.00%, 53.72%, and 97.35%, respectively. At different initial concentrations of MB, the maximum adsorption capacities of TOB and HTOB are 102.36 mg/g and 113.80 mg/g, and the adsorption capacity of AHTOB on MB is 248.01 mg/g. The adsorption efficiency of AHTOB modified by heating and acidification compound is improved. The optimal conditions for adsorption are pH value of 5-7, shaking time of 30 min, and temperature of 20-25℃.

, authors=Zhizeng WANG1, Tong LI1, Qinyi ZHAO1, Dongyun WANG1, Xiaoyu CUI2, Chong CUI1, authorsList=Zhizeng WANG, Tong LI, Qinyi ZHAO, Dongyun WANG, Xiaoyu CUI, Chong CUI, authorCompany=null, correspAuthors=Chong CUI, authorNote=

WANG Zhizeng (1993-), male, Doctoral candidate. E-mail:

, correspAuthorsNote=
CUI Chong (1957-), male, Master, Professor. E-mail:
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对托贝莫来石（TOB）进行加热与酸化复合改性，成功制备出比表面积为570 m2/g的酸化改性托贝莫来石（AHTOB），并用X射线衍射、N2吸附-脱附对改性托贝莫来石进行了结构表征和表面积及孔径分析。通过静态吸附实验探讨了3种吸附剂对亚甲基蓝溶液（MB）的吸附性能，分析改性TOB对MB的吸附机制。考察了不同吸附剂及其加入量、溶液pH值、MB初始浓度、吸附时间及温度对吸附行为的影响，研究了AHTOB对MB溶液吸附的热力学和动力学行为。结果表明：对50 mL，浓度为10 mg/L的MB进行吸附，未改性TOB、热改性HTOB以及酸化改性AHTOB对MB的吸附率分别达到50、53.72%和97.35%。对于不同初始浓度的MB，TOB和HTOB的最大吸附量可达102.36 mg/g和113.80 mg/g，AHTOB的吸附量达到248.01 mg/g，经过加热与酸化复合改性的AHTOB对MB的吸附效率有了明显的提升，得到了吸附MB溶液的最佳外界条件：pH值为5~7，震荡时间为30 min，温度为20~25℃。

, authors=王志增1, 李通1, 赵秦仪1, 王冬云1, 崔晓昱2, 崔崇1, authorsList=王志增, 李通, 赵秦仪, 王冬云, 崔晓昱, 崔崇, authorCompany=null, correspAuthors=崔崇, authorNote=

王志增（1993—），男，博士研究生。

, correspAuthorsNote=
崔崇（1957—），男，硕士，教授。
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WANG Zhizeng (1993-), male, Doctoral candidate. E-mail:

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王志增（1993—），男，博士研究生。

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王志增（1993—），男，博士研究生。

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托贝莫来石改性及其对亚甲基蓝的吸附性能
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王志增 1 , 李通 1 , 赵秦仪 1 , 王冬云 1 , 崔晓昱 2 , 崔崇 1
硅酸盐学报 | 2021,49(6): 1185-1194
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硅酸盐学报 | 2021 , 49 (6) : 1185 -1194
托贝莫来石改性及其对亚甲基蓝的吸附性能
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王志增1 , 李通1, 赵秦仪1, 王冬云1, 崔晓昱2, 崔崇1
作者信息
  • 1．南京理工大学材料科学与工程学院，南京 210094
  • 2．浙江中劲环保科技有限公司，浙江 宁波 315105
通讯作者:
崔崇（1957—），男，硕士，教授。
作者简介:

王志增（1993—），男，博士研究生。

Adsorption of Methylene Blue by Modified Tobermorite
Zhizeng WANG1 , Tong LI1, Qinyi ZHAO1, Dongyun WANG1, Xiaoyu CUI2, Chong CUI1
Affiliations
  • 1.School of Materials Science & Engineering, Nanjing University of Science & Technology, Nanjing 210094, China
  • 2.Zhejiang Zhong Jin Environmental Protection Technology Co., Ltd Ningbo 315105, Zhejiang, China
    • Corresponding Author:
    CUI Chong (1957-), male, Master, Professor. E-mail:

    WANG Zhizeng (1993-), male, Doctoral candidate. E-mail:

出版时间: 2021-06-20 doi: 10.14062/j.issn.0454-5648.20200792
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对托贝莫来石（TOB）进行加热与酸化复合改性，成功制备出比表面积为570 m2/g的酸化改性托贝莫来石（AHTOB），并用X射线衍射、N2吸附-脱附对改性托贝莫来石进行了结构表征和表面积及孔径分析。通过静态吸附实验探讨了3种吸附剂对亚甲基蓝溶液（MB）的吸附性能，分析改性TOB对MB的吸附机制。考察了不同吸附剂及其加入量、溶液pH值、MB初始浓度、吸附时间及温度对吸附行为的影响，研究了AHTOB对MB溶液吸附的热力学和动力学行为。结果表明：对50 mL，浓度为10 mg/L的MB进行吸附，未改性TOB、热改性HTOB以及酸化改性AHTOB对MB的吸附率分别达到50、53.72%和97.35%。对于不同初始浓度的MB，TOB和HTOB的最大吸附量可达102.36 mg/g和113.80 mg/g，AHTOB的吸附量达到248.01 mg/g，经过加热与酸化复合改性的AHTOB对MB的吸附效率有了明显的提升，得到了吸附MB溶液的最佳外界条件：pH值为5~7，震荡时间为30 min，温度为20~25℃。

托贝莫来石  /  亚甲基蓝  /  废水  /  改性  /  吸附

Modified tobermorillonite (AHTOB) with a specific surface area of 570 m2/g was prepared by heating and acidification of tobermorillonite (TOB). The structure and specific surface area and pore size of the modified tobermorillonite were characterized by X-ray diffraction and N2 adsorption-desorption. The adsorption properties of three adsorbents on methylene blue solution (MB) were investigated by static adsorption experiments, and the adsorption mechanism of modified TOB on MB was analyzed. The effects of adsorbents, solution pH value, initial MB concentration, adsorption time, and temperature on the adsorption behavior were investigated, and the thermodynamic and kinetic behaviors of AHTOB adsorbed on MB solution were investigated. The adsorption of MB was analyzed in 50 mL of MB at a concentration of 10 mg/L. The results show that the adsorption rates of unmodified TOB, HTOB, and AHTOB on MB are 50.00%, 53.72%, and 97.35%, respectively. At different initial concentrations of MB, the maximum adsorption capacities of TOB and HTOB are 102.36 mg/g and 113.80 mg/g, and the adsorption capacity of AHTOB on MB is 248.01 mg/g. The adsorption efficiency of AHTOB modified by heating and acidification compound is improved. The optimal conditions for adsorption are pH value of 5-7, shaking time of 30 min, and temperature of 20-25℃.

tobermorite  /  methylene blue  /  waste water  /  modification  /  adsorption
王志增, 李通, 赵秦仪, 王冬云, 崔晓昱, 崔崇. 托贝莫来石改性及其对亚甲基蓝的吸附性能. 硅酸盐学报, 2021 , 49 (6) : 1185 -1194 . DOI: 10.14062/j.issn.0454-5648.20200792
Zhizeng WANG, Tong LI, Qinyi ZHAO, Dongyun WANG, Xiaoyu CUI, Chong CUI. Adsorption of Methylene Blue by Modified Tobermorite[J]. Journal of the Chinese Ceramic Society, 2021 , 49 (6) : 1185 -1194 . DOI: 10.14062/j.issn.0454-5648.20200792
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  • 国家自然科学基金面上项目(51772153)
  • 浙江清华长三角研究院宁波分院鄞州区专项(2019-12-18)
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doi: 10.14062/j.issn.0454-5648.20200792
  • 接收时间：2020-10-21
  • 首发时间：2026-10-30
  • 出版时间：2021-06-20
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  • 收稿日期：2020-10-21
  • 修回日期：2020-11-03
基金
国家自然科学基金面上项目(51772153)
浙江清华长三角研究院宁波分院鄞州区专项(2019-12-18)
作者信息
    1．南京理工大学材料科学与工程学院，南京 210094
    2．浙江中劲环保科技有限公司，浙江 宁波 315105

通讯作者:

崔崇（1957—），男，硕士，教授。
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20200792
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2种不同金属材料的力学参数
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Number of
species		 占总种数比例
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total species (%)		 属
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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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