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It is of great significance for the optimization and performance improvement of aggregates to investigate the influence of aggregate chemical properties on the nucleation and growth of calcium silicate hydrate (C-S-H) and its mechanism. In this work, limestone, quartz and magnesite were used as aggregates. The interactions between different aggregates and ions in a simulated solution were determined via zeta potential measurement. Also, the nucleation and growth of C-S-H on the surface of these aggregates were analyzed by scanning electron microscopy. The hydration heat of cement pastes with the micro-aggregates was examined to investigate the effect of aggregate chemical properties on the early hydration of cement. The results show that limestone surface has a strong adsorption of Ca²⁺ (i.e., chemical adsorption), leading to a high density of C-S-H nuclei and directional growth of C-S-H, and thus greatly promoting the hydration of cement. The adsorption of Ca²⁺ on quartz surface is due to electrostatic force, which is weaker than that due to the chemical adsorption. The density of C-S-H nuclei on quartz surface is thus much lower than that on limestone surface. In the case of magnesite, its surface has a high affinity for SO₄^2- rather than Ca²⁺, reducing the nucleation density of C-S-H on the surface of magnesite, and thus slowing down the early hydration of cement.

, authors=Xiaowei OUYANG¹, Shida XU¹, Yuwei MA¹, Guang YE², authorsList=Xiaowei OUYANG, Shida XU, Yuwei MA, Guang YE, authorCompany=null, correspAuthors=null, authorNote=, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322942593402810703, articleId=1322942592790442317, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=集料化学特性对C-S-H成核和生长的影响, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

探究集料化学特性对水化硅酸钙（C-S-H）成核和生长的影响及其作用机理对集料优选和性能改善意义重大。选用石灰石、石英石和菱镁石为研究对象，通过测量3种集料的粉末颗粒在模拟溶液中的zeta电位，研究了集料表面与模拟溶液中离子间的相互作用；采用扫描电子显微镜观察了C-S-H在这些集料表面的成核和生长。采用水化热的方法，研究了集料的化学特性对水泥早期水化的影响。结果表明：石灰石表面对Ca²⁺有极强的吸附作用（化学吸附），这使得C-S-H在石灰石表面成核密度高且生长具有方向性，从而极大地促进了水泥的水化；石英石表面通过静电力作用吸附Ca²⁺，该作用弱于化学吸附作用，从而使得C-S-H在石英石表面成核密度低，且呈无序和稀疏分布；菱镁石对Ca²⁺的吸附作用最弱而对SO₄^2-具有很强的吸附作用，这使得C-S-H在菱镁石表面成核密度最低，从而减缓了水泥的早期水化。

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