Article(id=1322943328169370044, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942634976752425, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200664, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1598889600000, receivedDateStr=2020-09-01, revisedDate=1603296000000, revisedDateStr=2020-10-22, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343868534, onlineDateStr=2026-10-30, pubDate=1626710400000, pubDateStr=2021-07-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343868534, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343868534, creator=13701087609, updateTime=1793343868534, updator=13701087609, issue=Issue{id=1322942634976752425, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='7', pageStart='1249', pageEnd='1518', issueExtLink='null', onlineDate='null', pubDate='1626710400000', pubDateStr='2021-07-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343703264, creator='13701087609', updateTime=1793345819416, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322951510828659213, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942634976752425, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322951510828659214, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942634976752425, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1466, endPage=1484, ext={EN=ArticleExt(id=1322943328584606141, articleId=1322943328169370044, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Interface Optimization in Solid-State Lithium Batteries, columnId=1319726165087077079, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Article, runingTitle=null, highlight=null, articleAbstract=

All-solid-state lithium batteries become popular due to their high energy density, high safety, and wide electrochemical window. However, there are also some problems in the practical applications, such as the rigid contact between solid electrolyte and electrode material, side reactions occurring readily in contact with electrolyte because of active lithium metal causing the interface to be unstable, sulfide solid electrolyte being unstable to air and high production costs. This review summarized some research work on the interface between electrode material and oxide solid electrolyte, sulfide solid electrolyte, and polymer solid electrolyte, analyzed the interface problems, and discussed the interface optimization strategies to solve the interface problems of all solid-state lithium batteries in the future.

, authors=Xiaowei XU, Shuhao WANG, Yinghe Zhao, Huiqiao LI, authorsList=Xiaowei XU, Shuhao WANG, Yinghe Zhao, Huiqiao LI, authorCompany=null, correspAuthors=Yinghe Zhao, Huiqiao LI, authorNote=

XU Xiaowei(1996-), male, Master candidate; E-mail:

WANG Shuhao (1996-), male, Doctoral candidate

, correspAuthorsNote=
ZHAO Yinghe (1989-), male, Ph.D., Associate Professor; E-mail:
LI Huiqiao (1980-), female, Ph.D., Professor.
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全固态锂电池由于高安全性、高能量密度、宽电化学窗口受到研究者的关注,但是在实际应用中也存在一些问题,如固态电解质和电极材料之间为刚性接触,界面电阻大;锂金属较为活泼,与电解质接触易发生副反应导致界面不稳定;硫化物固态电解质对空气不稳定,生产成本高等。综述了电极材料与氧化物固态电解质、硫化物固态电解质、聚合物固态电解质的界面问题,对界面优化策略进行介绍和讨论,为以后解决全固态锂电池界面问题提供参考。

, authors=许晓伟, 王书豪, 赵英鹤, 李会巧, authorsList=许晓伟, 王书豪, 赵英鹤, 李会巧, authorCompany=null, correspAuthors=赵英鹤, 李会巧, authorNote=

许晓伟(1996—),男,硕士研究生;

王书豪(1996—),男,博士研究生。

, correspAuthorsNote=
赵英鹤(1989—),男,博士,副教授;
李会巧(1980—),女,博士,教授。
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王书豪(1996—),男,博士研究生。

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固态锂电池中的界面优化
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许晓伟 , 王书豪 , 赵英鹤 , 李会巧
硅酸盐学报 | 综合评述 2021,49(7): 1466-1484
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硅酸盐学报 |综合评述 2021 , 49 (7) : 1466 -1484
固态锂电池中的界面优化
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许晓伟 , 王书豪 , 赵英鹤 , 李会巧
作者信息
  • 华中科技大学材料科学与工程学院,材料成形与模具技术国家重点实验室,武汉 430074
通讯作者:
赵英鹤(1989—),男,博士,副教授;
李会巧(1980—),女,博士,教授。
作者简介:

许晓伟(1996—),男,硕士研究生;

王书豪(1996—),男,博士研究生。

Interface Optimization in Solid-State Lithium Batteries
Xiaowei XU , Shuhao WANG , Yinghe Zhao , Huiqiao LI
Affiliations
  • State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
  • Corresponding Author:
    ZHAO Yinghe (1989-), male, Ph.D., Associate Professor; E-mail:
    LI Huiqiao (1980-), female, Ph.D., Professor.

    XU Xiaowei(1996-), male, Master candidate; E-mail:

    WANG Shuhao (1996-), male, Doctoral candidate

出版时间: 2021-07-20 doi: 10.14062/j.issn.0454-5648.20200664
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全固态锂电池由于高安全性、高能量密度、宽电化学窗口受到研究者的关注,但是在实际应用中也存在一些问题,如固态电解质和电极材料之间为刚性接触,界面电阻大;锂金属较为活泼,与电解质接触易发生副反应导致界面不稳定;硫化物固态电解质对空气不稳定,生产成本高等。综述了电极材料与氧化物固态电解质、硫化物固态电解质、聚合物固态电解质的界面问题,对界面优化策略进行介绍和讨论,为以后解决全固态锂电池界面问题提供参考。

氧化物固态电解质  /  硫化物固态电解质  /  聚合物固态电解质  /  界面优化

All-solid-state lithium batteries become popular due to their high energy density, high safety, and wide electrochemical window. However, there are also some problems in the practical applications, such as the rigid contact between solid electrolyte and electrode material, side reactions occurring readily in contact with electrolyte because of active lithium metal causing the interface to be unstable, sulfide solid electrolyte being unstable to air and high production costs. This review summarized some research work on the interface between electrode material and oxide solid electrolyte, sulfide solid electrolyte, and polymer solid electrolyte, analyzed the interface problems, and discussed the interface optimization strategies to solve the interface problems of all solid-state lithium batteries in the future.

oxide solid electrolyte  /  sulfide solid electrolyte  /  polymer solid electrolyte  /  interface optimization
许晓伟, 王书豪, 赵英鹤, 李会巧. 固态锂电池中的界面优化. 硅酸盐学报, 2021 , 49 (7) : 1466 -1484 . DOI: 10.14062/j.issn.0454-5648.20200664
Xiaowei XU, Shuhao WANG, Yinghe Zhao, Huiqiao LI. Interface Optimization in Solid-State Lithium Batteries[J]. Journal of the Chinese Ceramic Society, 2021 , 49 (7) : 1466 -1484 . DOI: 10.14062/j.issn.0454-5648.20200664
  • 国家自然科学基金面上项目(52072138)
  • 国家研究重点与计划专项(2018YFE0206900)
  • 2019湖北省创新群体(2019CFA002)
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2021年第49卷第7期
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doi: 10.14062/j.issn.0454-5648.20200664
  • 接收时间:2020-09-01
  • 首发时间:2026-10-30
  • 出版时间:2021-07-20
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  • 收稿日期:2020-09-01
  • 修回日期:2020-10-22
基金
国家自然科学基金面上项目(52072138)
国家研究重点与计划专项(2018YFE0206900)
2019湖北省创新群体(2019CFA002)
作者信息
    华中科技大学材料科学与工程学院,材料成形与模具技术国家重点实验室,武汉 430074

通讯作者:

赵英鹤(1989—),男,博士,副教授;
李会巧(1980—),女,博士,教授。
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20200664
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2种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
species
占总种数比例
Percentage of
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属
Genus
种数
Number of
species
占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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