Article(id=1322942777931202914, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200203, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1585497600000, receivedDateStr=2020-03-30, revisedDate=1590681600000, revisedDateStr=2020-05-29, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343737346, onlineDateStr=2026-10-30, pubDate=1611072000000, pubDateStr=2021-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343737346, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343737346, creator=13701087609, updateTime=1793343737346, updator=13701087609, issue=Issue{id=1322942385474384734, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='1', pageStart='1', pageEnd='210', issueExtLink='null', onlineDate='null', pubDate='1611072000000', pubDateStr='2021-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343643777, creator='13701087609', updateTime=1793345438198, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322949911880282449, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322949911880282450, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=202, endPage=210, ext={EN=ArticleExt(id=1322942780015772005, articleId=1322942777931202914, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=AgBr/ZnO Composite Photocatalyst ant Its Photocatalytic Performance, columnId=1319726165087077079, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Article, runingTitle=null, highlight=null, articleAbstract=

AgBr/ZnO composite photocatalyst was prepared by a simple one-step hydrothermal method. The composites were characterized by scanning electron microscopy, transmission electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy, ultraviolet-visible spectroscopy and photoluminescence spectroscopy. The effect of AgBr/ZnO system synthesis on the photocatalytic properties of the materials was analyzed. The photocatalytic activity of the composite catalyst was investigated with rhodamine B solution as a target pollutant. The results show that an optimum AgBr/ZnO-2 composite with a molar ratio of AgBr to ZnO of 1∶5 has a degradation rate of rhodamine B of 98.98% for 60 min under visible light irradiation. Compared to ZnO, the photocatalytic activity is improved and the degradation rate constant is increased by 11.08 times. Compared to commercial TiO2(P25), the degradation rate constant is increased by 10.14 times. That is mainly since AgBr/ZnO has a lower electron-hole recombination ratio than ZnO, and the optical absorption band edge of the composite catalyst is red-shifted, thereby enhancing the absorption of visible light.

, authors=Chong TAN1, Yuanyuan LI1, Hao LIU1, Junsheng LI2, Zhi XIA2, Jinlong ZUO2, Lin YAO3, authorsList=Chong TAN, Yuanyuan LI, Hao LIU, Junsheng LI, Zhi XIA, Jinlong ZUO, Lin YAO, authorCompany=null, correspAuthors=Junsheng LI, authorNote=

TAN Chong (1980-), male, Ph.D., Research Assistant. E-mail:

, correspAuthorsNote=
LI Junsheng (1970-), male, Master, Associate Professor. E-mail:
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通过一步水热法制备了AgBr/ZnO复合光催化剂,并采用扫描电子显微镜、透射电子显微镜、X射线衍射仪、X射线光电子能谱仪、紫外-可见光漫反射光谱仪和光致发光光谱仪对样品进行表征,分析了AgBr/ZnO体系的合成对材料光催化性能的影响。以罗丹明B溶液为目标污染物,研究复合催化剂的光催化活性。结果表明:在制备的复合样品中,AgBr与ZnO摩尔比为1∶5时(AgBr/ZnO-2)光催化活性最好,在可见光照射下,60 min对罗丹明B的降解率可达98.98%,相比于ZnO光催化活性明显提升,降解速率常数提升了11.08倍;与商用TiO2(P25)相比,降解速率常数提升了10.14倍,这主要归因于AgBr/ZnO拥有比ZnO更低的电子空穴复合概率,且复合催化剂的光学吸收带边发生红移,从而增强了对可见光的吸收。

, authors=谭冲1, 李媛媛1, 刘昊1, 李俊生2, 夏至2, 左金龙2, 姚琳3, authorsList=谭冲, 李媛媛, 刘昊, 李俊生, 夏至, 左金龙, 姚琳, authorCompany=null, correspAuthors=李俊生, authorNote=

谭冲(1980—),男,博士,助理研究员。

, correspAuthorsNote=
李俊生(1970—),男,硕士,副教授。
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AgBr/ZnO复合材料光催化剂及其光催化性能
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谭冲 1 , 李媛媛 1 , 刘昊 1 , 李俊生 2 , 夏至 2 , 左金龙 2 , 姚琳 3
硅酸盐学报 | 研究论文 2021,49(1): 202-210
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硅酸盐学报 |研究论文 2021 , 49 (1) : 202 -210
AgBr/ZnO复合材料光催化剂及其光催化性能
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谭冲(1980—),男,博士,助理研究员。

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谭冲1 , 李媛媛1, 刘昊1, 李俊生2 , 夏至2, 左金龙2, 姚琳3
作者信息
  • 1.哈尔滨商业大学药学院(药物工程技术研究中心),哈尔滨 150076
  • 2.哈尔滨商业大学食品工程学院,哈尔滨 150076
  • 3.哈尔滨师范大学生命科学与技术学院,哈尔滨 150025
通讯作者:
李俊生(1970—),男,硕士,副教授。
作者简介:

谭冲(1980—),男,博士,助理研究员。

AgBr/ZnO Composite Photocatalyst ant Its Photocatalytic Performance
Chong TAN1 , Yuanyuan LI1, Hao LIU1, Junsheng LI2 , Zhi XIA2, Jinlong ZUO2, Lin YAO3
Affiliations
  • 1.School of Pharmacy (Pharmaceutical Engineering Technology Research Center), Harbin University of Commerce, Harbin 150076, China
  • 2.School of Food Science and Engineering, Harbin University of Commerce, Harbin 150076, China
  • 3.College of Life Science and Technology, Harbin Normal University, Harbin 150025, China
  • Corresponding Author:
    LI Junsheng (1970-), male, Master, Associate Professor. E-mail:

    TAN Chong (1980-), male, Ph.D., Research Assistant. E-mail:

出版时间: 2021-01-20 doi: 10.14062/j.issn.0454-5648.20200203
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通过一步水热法制备了AgBr/ZnO复合光催化剂,并采用扫描电子显微镜、透射电子显微镜、X射线衍射仪、X射线光电子能谱仪、紫外-可见光漫反射光谱仪和光致发光光谱仪对样品进行表征,分析了AgBr/ZnO体系的合成对材料光催化性能的影响。以罗丹明B溶液为目标污染物,研究复合催化剂的光催化活性。结果表明:在制备的复合样品中,AgBr与ZnO摩尔比为1∶5时(AgBr/ZnO-2)光催化活性最好,在可见光照射下,60 min对罗丹明B的降解率可达98.98%,相比于ZnO光催化活性明显提升,降解速率常数提升了11.08倍;与商用TiO2(P25)相比,降解速率常数提升了10.14倍,这主要归因于AgBr/ZnO拥有比ZnO更低的电子空穴复合概率,且复合催化剂的光学吸收带边发生红移,从而增强了对可见光的吸收。

溴化银  /  氧化锌  /  光催化  /  复合光催化剂  /  罗丹明B

AgBr/ZnO composite photocatalyst was prepared by a simple one-step hydrothermal method. The composites were characterized by scanning electron microscopy, transmission electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy, ultraviolet-visible spectroscopy and photoluminescence spectroscopy. The effect of AgBr/ZnO system synthesis on the photocatalytic properties of the materials was analyzed. The photocatalytic activity of the composite catalyst was investigated with rhodamine B solution as a target pollutant. The results show that an optimum AgBr/ZnO-2 composite with a molar ratio of AgBr to ZnO of 1∶5 has a degradation rate of rhodamine B of 98.98% for 60 min under visible light irradiation. Compared to ZnO, the photocatalytic activity is improved and the degradation rate constant is increased by 11.08 times. Compared to commercial TiO2(P25), the degradation rate constant is increased by 10.14 times. That is mainly since AgBr/ZnO has a lower electron-hole recombination ratio than ZnO, and the optical absorption band edge of the composite catalyst is red-shifted, thereby enhancing the absorption of visible light.

silver bromide  /  zinc oxide  /  photocatalysis  /  composite photocatalyst  /  rhodamine B
谭冲, 李媛媛, 刘昊, 李俊生, 夏至, 左金龙, 姚琳. AgBr/ZnO复合材料光催化剂及其光催化性能. 硅酸盐学报, 2021 , 49 (1) : 202 -210 . DOI: 10.14062/j.issn.0454-5648.20200203
Chong TAN, Yuanyuan LI, Hao LIU, Junsheng LI, Zhi XIA, Jinlong ZUO, Lin YAO. AgBr/ZnO Composite Photocatalyst ant Its Photocatalytic Performance[J]. Journal of the Chinese Ceramic Society, 2021 , 49 (1) : 202 -210 . DOI: 10.14062/j.issn.0454-5648.20200203
  • 黑龙江省自然科学基金(QC2018021)
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2021年第49卷第1期
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doi: 10.14062/j.issn.0454-5648.20200203
  • 接收时间:2020-03-30
  • 首发时间:2026-10-30
  • 出版时间:2021-01-20
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  • 收稿日期:2020-03-30
  • 修回日期:2020-05-29
基金
黑龙江省自然科学基金(QC2018021)
作者信息
    1.哈尔滨商业大学药学院(药物工程技术研究中心),哈尔滨 150076
    2.哈尔滨商业大学食品工程学院,哈尔滨 150076
    3.哈尔滨师范大学生命科学与技术学院,哈尔滨 150025

通讯作者:

李俊生(1970—),男,硕士,副教授。
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20200203
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2种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
species
占总种数比例
Percentage of
total species (%)
属
Genus
种数
Number of
species
占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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