Article(id=1322636257851723828, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322636234858550134, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200048, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1580572800000, receivedDateStr=2020-02-02, revisedDate=1590768000000, revisedDateStr=2020-05-30, acceptedDate=null, acceptedDateStr=null, onlineDate=1793270657265, onlineDateStr=2026-10-29, pubDate=1603123200000, pubDateStr=2020-10-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793270657265, onlineIssueDateStr=2026-10-29, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793270657265, creator=13701087609, updateTime=1793270657265, updator=13701087609, issue=Issue{id=1322636234858550134, tenantId=1146029695717560320, journalId=1263187385517883426, year='2020', volume='48', issue='10', pageStart='1505', pageEnd='1688', issueExtLink='null', onlineDate='null', pubDate='1603123200000', pubDateStr='2020-10-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793270651783, creator='13701087609', updateTime=1793277146795, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322663476976267430, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322636234858550134, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322663476976267431, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322636234858550134, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1581, endPage=1588, ext={EN=ArticleExt(id=1322636258266959925, articleId=1322636257851723828, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Performance of Transparent Cu₂S@N-doped Carbon Film as Counter Electrode for Bifacial Quantum Dot Solar Cells, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

A copper-metalloporphy in metal-organic framework material (Cu-TCPP) was synthesized via a liquid-phase epitaxy approach. Afterward, a transparent Cu₂S@N-doped carbon film was in situ fabricated using Cu-TCPP as a template, and was directly used as a counter electrode for bifacial CdS/CdSe quantum-dot sensitive solar cells (QDSSC). The morphology, construction, and performance of Cu₂S@N-doped carbon film were also investigated. During the sulfidation process, the cupric ions in Cu-TCPP thin film were transformed into Cu₂S nanoparticles, while the nitrogen-rich ligand (TCPP) was in situ carbonized, generating N-doped carbon and leading to the formation of a uniform Cu₂S@N-doped carbon film. After the sulfidation of Cu-TCPP, the original nanosheet morphology is maintained and uniform Cu₂S nanoparticles are embedded on the nanosheet surface. As a result, the transparent Cu₂S@N-doped carbon film exhibits greater power conversion efficiencies (i.e., 4.16% and 3.72%) rather than Pt (i.e., 2.39% and 1.73%) from the front and rear irradiations, respectively. Based on the analysis of the systematic electrochemical data by cyclic voltammetry test, electrochemical impedance spectroscopy and Tafel test, a transparent Cu₂S@N-doped carbon film with a low charge-transfer resistance, a fast ion diffusion rate, and an excellent catalytic ability is obtained for S_n^2-/S^2- redox reaction. As a result, the superior photovoltaic performance of bifacial CdS/CdSe QDSSC can be achieved.

, authors=Jinhua OU¹, Bonian HU¹, Huanyu ZHOU¹, Yu HAN^{2, 3}, authorsList=Jinhua OU, Bonian HU, Huanyu ZHOU, Yu HAN, authorCompany=null, correspAuthors=Yu HAN, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322636258682196022, articleId=1322636257851723828, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=透明Cu²S@氮掺杂碳纳米片用于双面量子点敏化太阳能电池对电极的性能, columnId=null, journalTitle=硅酸盐学报, columnName=, runingTitle=null, highlight=null, articleAbstract=

采用液相外延生长法制备了一种由铜和四羧基卟啉配位的金属-有机框架薄膜材料，以其为牺牲模板，原位合成了Cu₂S和氮掺杂碳的复合透明膜（Cu₂S@NCF），将其直接作双面CdS/CdSe量子点敏化太阳能电池（QDSSC）对电极，并对其进行了结构、形貌及性能研究。结果表明：Cu-（5，10，15，20-（4-羧基苯基）卟啉）（TCPP）薄膜在煅烧过程中，Cu原子在硫粉存在下转变成了Cu₂S纳米颗粒，而含氮的有机连接单元TCPP原位碳化成了氮掺杂的碳。Cu₂S@NCF保持了Cu-TCPP薄膜的纳米片形貌，且大量尺寸均一的Cu₂S小颗粒分布于纳米片上，以其作对电极所组装的CdS/CdSe QDSSC具有优异的光伏性能，从正面辐射和背面辐射分别获得了4.16%和3.72%的光电转化效率（η），高于Pt电极组装QDSSC的η（2.39%和1.73%）。通过对循环伏安曲线、电化学阻抗谱和Tafel极化曲线分析可知，Cu₂S@NCF对S_n^2-离子催化还原具有传输阻抗低、扩散速率快和催化活性高等特点，以其作对电极组装的CdS/CdSe QDSSC获得了优异的光伏性能。

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OU Jinhua (1987-), female, Ph.D., Lecturer. E-mail: oujinhua98@126.com

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欧金花（1987—），女，博士，讲师。

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