Article(id=1322622785529168396, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322622757339250965, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.2020.07.20190727, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1572969600000, receivedDateStr=2019-11-06, revisedDate=1577116800000, revisedDateStr=2019-12-24, acceptedDate=null, acceptedDateStr=null, onlineDate=1793267445212, onlineDateStr=2026-10-29, pubDate=1595174400000, pubDateStr=2020-07-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793267445212, onlineIssueDateStr=2026-10-29, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793267445212, creator=13701087609, updateTime=1793267445212, updator=13701087609, issue=Issue{id=1322622757339250965, tenantId=1146029695717560320, journalId=1263187385517883426, year='2020', volume='48', issue='7', pageStart='939', pageEnd='1144', issueExtLink='null', onlineDate='null', pubDate='1595174400000', pubDateStr='2020-07-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793267438492, creator='13701087609', updateTime=1793277091258, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322663244053992200, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322622757339250965, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322663244053992201, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322622757339250965, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1128, endPage=1133, ext={EN=ArticleExt(id=1322622785747272205, articleId=1322622785529168396, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Effect of Template Composition on Structure and Methanol to Olefins Catalytic Performance of SAPO-34 Molecular Sieve, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

The flake structure SAPO-34 was firstly synthesized via a hydrothermal method with co-template triethylamine and tetraethylammonium bromide as crystal seeds, and then the layered SAPO-34 molecular sieves with different thicknesses were synthesized via changing the template composition. The prepared samples were characterized by X-ray diffraction, scanning electronic microscopy and NH₃-temperature programmed desorption. The methanol to olefins catalytic performance of the SAPO-34 was evaluated by a fixed-bed reactor. The results show that the crystallization time of SAPO-34 shortens by to 36 h and the SAPO-34 cannot be produced without template. The template has an influence on the thickness of layered SAPO-34. The lamellar SAPO-34 has better light olefins selectivity than the flake and cubic ones, but its catalytic stability is slightly inferior to that of the flake one.

, authors=Yujia WANG^{1, 2}, Lu LI¹, Yingzhi BAI¹, Min WEI¹, Haiyan WANG^{1, 2}, authorsList=Yujia WANG, Lu LI, Yingzhi BAI, Min WEI, Haiyan WANG, authorCompany=null, correspAuthors=null, authorNote=, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322622786040873486, articleId=1322622785529168396, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=模板剂组成对SAPO-34分子筛结构和甲醇制烯烃性能的影响, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

添加双模板剂三乙胺和四乙基溴化铵，利用水热法合成片状SAPO-34作为晶种，改变模板剂组成合成不同厚度的层状SAPO-34分子筛。采用X射线衍射、扫描电子显微镜、氨气程序升温脱附等手段对合成的分子筛进行表征，在固定床反应器上评价SAPO-34的甲醇制烯烃催化性能。实验结果表明：添加晶种使SAPO-34分子筛的晶化时间缩短了36 h，无模板剂导向作用无法合成SAPO-34，利用模板剂组成可以调变层状SAPO-34分子筛的厚度；板层状SAPO-34比片层状和立方体状分子筛的低碳烯烃选择性略高，但其稳定性较片层的SAPO-34稍差。

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^2.China University of Petroleum (East China), Qingdao 266555, Shandong, China, bio={"content":"

WANG Yujia (1988-), female, Master. E-mail: fsyzww@126.com

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WANG Yujia (1988-), female, Master. E-mail: fsyzww@126.com

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王钰佳（1988—），女，硕士，实验师。

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王钰佳（1988—），女，硕士，实验师。

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