Article(id=1322612359542190341, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612265061306700, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.2020.05.20190579, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1566403200000, receivedDateStr=2019-08-22, revisedDate=1571673600000, revisedDateStr=2019-10-22, acceptedDate=null, acceptedDateStr=null, onlineDate=1793264959463, onlineDateStr=2026-10-29, pubDate=1589904000000, pubDateStr=2020-05-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793264959463, onlineIssueDateStr=2026-10-29, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793264959463, creator=13701087609, updateTime=1793264959463, updator=13701087609, issue=Issue{id=1322612265061306700, tenantId=1146029695717560320, journalId=1263187385517883426, year='2020', volume='48', issue='5', pageStart='615', pageEnd='786', issueExtLink='null', onlineDate='null', pubDate='1589904000000', pubDateStr='2020-05-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793264936938, creator='13701087609', updateTime=1793276961694, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322662700602208333, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612265061306700, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322662700602208334, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612265061306700, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=730, endPage=738, ext={EN=ArticleExt(id=1322612360926310662, articleId=1322612359542190341, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Degradation of Dye and Ammonia by Cu/Fe-Layered Doubled Hydroxide as Heterogeneous Photoactivator of NaClO, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

Cu/Fe-layered doubled hydroxide (CuFe LDH) prepared by a coprecipitation method was used to degrade methylene blue (MB) and ammonia as a heterogeneous photoactivator of NaClO. The micro-morphology, reaction kinetics and degradation mechanism were investigated. The layered structure of the samples with Cu/Fe molar ratios from 2∶1 to 4∶1 was analyzed. The catalyst with Cu/Fe molar ratio of 3∶1 exhibits the optimum performance under given conditions (i.e., catalyst dosage of 0.5 g/L and NaClO of 0.075 mL), and the pseudo-first-order rate constant of 30 mL MB (100 mg/L) is 7.9 times greater than that without any catalyst. 30 mL ammonia (100 mg/L) at the catalyst dosage of 3 g/L and NaClO of 0.3 mL can be degraded by 99.5% within 1 min, compared to that of 66.6% without any catalyst. Based on the radical quenching experimental results, the superoxide radicals are the dominant reactive oxidants, and also involve chlorine radicals and hydroxyl radicals. The results by electrochemical impedance spectra and X-ray photoelectron spectroscopy reveal that the photoelectrons can accelerate the in-situ regeneration of reaction activity sites on the surface of catalyst and increase the separation efficiency of photo-induced charges in CuFe LDH/NaClO/light system, resulting in the improved degradation of waste water pollutants.

, authors=Guoping ZHAO¹, Yangyang WANG², Na LI¹, Shengrui SUN², Yangqiao LIU², authorsList=Guoping ZHAO, Yangyang WANG, Na LI, Shengrui SUN, Yangqiao LIU, authorCompany=null, correspAuthors=Shengrui SUN, Yangqiao LIU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322612361576427783, articleId=1322612359542190341, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=铜铁类水滑石光化学催化降解染料和氨氮应用, columnId=null, journalTitle=硅酸盐学报, columnName=, runingTitle=null, highlight=null, articleAbstract=

采用共沉淀法制备铜铁类水滑石（CuFe LDH），将其应用于染料和氨氮的光-次氯酸钠协同催化降解实验中，研究了Cu-Fe比例对CuFe LDH形貌的影响，及CuFe LDH对亚甲基蓝（MB）和氨氮的光化学催化降解效果。结果表明：比例在2∶1~4∶1时均能形成LDH结构，Cu-Fe比例为3∶1时，降解MB的动力学常数是无催化剂的7.9倍，反应1 min时氨氮的降解率为99.5%高于无催化剂的66.6%；利用自由基捕获剂证明降解过程主要由超氧自由基实现，同时存在氯自由基和少量羟基自由基；CuFe LDH在光化学催化过程中实现了表面活性位点的持续再生和电子-空穴对的高效分离。

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Zhao Guoping (1981-), male, Senior Engineer. E-mail: xajhgz@163.com

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Zhao Guoping (1981-), male, Senior Engineer. E-mail: xajhgz@163.com

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赵国萍（1981—），男，高级工程师。

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赵国萍（1981—），男，高级工程师。

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