Article(id=1322612257951957720, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612228126265395, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20190642, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1568908800000, receivedDateStr=2019-09-20, revisedDate=1574524800000, revisedDateStr=2019-11-24, acceptedDate=null, acceptedDateStr=null, onlineDate=1793264935242, onlineDateStr=2026-10-29, pubDate=1587312000000, pubDateStr=2020-04-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793264935242, onlineIssueDateStr=2026-10-29, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793264935242, creator=13701087609, updateTime=1793264935242, updator=13701087609, issue=Issue{id=1322612228126265395, tenantId=1146029695717560320, journalId=1263187385517883426, year='2020', volume='48', issue='4', pageStart='463', pageEnd='614', issueExtLink='null', onlineDate='null', pubDate='1587312000000', pubDateStr='2020-04-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793264928132, creator='13701087609', updateTime=1793276729826, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322661728073138752, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612228126265395, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322661728073138753, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612228126265395, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=483, endPage=490, ext={EN=ArticleExt(id=1322612259747119833, articleId=1322612257951957720, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Improvement of Electron Transport in Dye-Sensitized Solar Cells Based on TiO₂/MWCNTs Composite Films as a Photoanode and SnO₂/MWCNTs as a Pt-free Counter Electrode, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

In order to improve the electron transport rate of TiO₂ photoanode, multi-walled carbon nanotubes (MWCNTs) were loaded in TiO₂. TiO₂/MWCNTs composite sols were formed by a sol-gel hydrothermal method, and the uniform TiO₂/MWCNTs composite films were formed by an electro-hydrodynamic method. The films were optimized with TiCl₄. The samples were characterized by scanning electron microscopy, transmission electron microscopy, X-ray diffractometer and ultraviolet-visible absorption spectroscopy. The photoelectric properties of dye-sensitized solar cells (DSSCs) based on TiO₂/MWCNTs composite photoanodes and SnO₂/MWCNTs counter electrode were analyzed by electrochemical impedance spectroscopy and current density-voltage curve measurement. The results show that the addition of MWCNTs considerably accelerates the transport of electrons in the films and decreases the recombination of electrons with oxidized dye and I₃^-; The DSSC with a CNT-0.12 (0.12%, in mass) composite photoanode shows the optimal performance (i.e., V_oc=0.70 V, J_sc=13.0 mA/cm², η_FF=0.64, η=5.80%), and the power conversion efficiency is 30.6% greater than that of DSSC with a pure TiO₂ photoanode (i.e., η=4.44%).

, authors=Qinglong LIU, Xiaoyu WANG, Liping ZHAO, Liguo JIN, authorsList=Qinglong LIU, Xiaoyu WANG, Liping ZHAO, Liguo JIN, authorCompany=null, correspAuthors=Liguo JIN, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322612260908942042, articleId=1322612257951957720, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=基于TiO₂/多壁碳纳米管复合光阳极和SnO₂/多壁碳纳米管非铂对电极的染料敏化太阳能电池电子传输的改善, columnId=null, journalTitle=硅酸盐学报, columnName=, runingTitle=null, highlight=null, articleAbstract=

为了提高TiO₂光阳极的电子传输速率，在TiO₂中负载了多壁碳纳米管（MWCNTs）。采用溶胶-凝胶水热法制备了TiO₂/MWCNTs复合溶胶，利用电流体动力学方法制备了均匀的TiO₂/MWCNTs复合薄膜，并用TiCl₄对薄膜进行了优化。用扫描电子显微镜、透射电子显微镜、X射线衍射仪和紫外可见吸收光谱仪对样品进行了表征分析。利用电化学阻抗谱和电流密度-电压曲线分析了基于TiO₂/MWCNTs复合光阳极和SnO₂/MWCNTs对电极的染料敏化太阳能电池（DSSC）的光电性能。结果表明，MWCNTs的加入极大地加速了电子在薄膜中的传输，减少了电子与氧化态染料和I₃^-的复合；基于CNT-0.12（质量分数0.12%）复合光阳极的DSSC性能最佳（V_OC=0.70 V，J_SC=13.0 mA/cm²，η_FF=0.64，η=5.80%），与基于纯TiO₂光阳极的DSSC（η=4.44 %）相比，能量转换效率提高了30.6%。

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LIU Qinglong (1995-), male, Master candidate. E-mail: 774882853@qq.com

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LIU Qinglong (1995-), male, Master candidate. E-mail: 774882853@qq.com

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刘青龙（1995—），男，硕士研究生。

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刘青龙（1995—），男，硕士研究生。

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