Article(id=1322636213857669828, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322636193100050547, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20190077, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1581782400000, receivedDateStr=2020-02-16, revisedDate=1584720000000, revisedDateStr=2020-03-21, acceptedDate=null, acceptedDateStr=null, onlineDate=1793270646775, onlineDateStr=2026-10-29, pubDate=1600531200000, pubDateStr=2020-09-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793270646775, onlineIssueDateStr=2026-10-29, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793270646775, creator=13701087609, updateTime=1793270646775, updator=13701087609, issue=Issue{id=1322636193100050547, tenantId=1146029695717560320, journalId=1263187385517883426, year='2020', volume='48', issue='9', pageStart='1353', pageEnd='1510', issueExtLink='null', onlineDate='null', pubDate='1594569600000', pubDateStr='2020-07-13', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793270641826, creator='13701087609', updateTime=1793270641826, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext=null, issueFiles=null, downloadFileDto=null}, startPage=1474, endPage=1481, ext={EN=ArticleExt(id=1322636214025441989, articleId=1322636213857669828, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Effect of Zr⁴⁺ Substitution on Structure and Luminescence Properties of Ba(Mg_1/3Nb_2/3)O₃:Eu³⁺ Phosphors, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

(Ba_0.97Eu_0.03)(Mg_(1-x)/3Nb_2(1-x)/3Zr_x)O₃ phosphors were prepared via a solid-state route. The crystal structure and luminescent properties were investigated. A phase structure transformation from hexagonal to cubic occurs as Zr⁴⁺ content (x) increases to 0.05, thus weakening the luminescence properties. When x>0.05, the crystal structure is cubic. The introduction of Zr⁴+into the phosphor increases the tilting of BO₆ octahedron, which makes the energy level split and broadens the bonding energy range of B—O bond, thus enhancing the absorption of near ultraviolet (NUV) light and increasing the intensity of charge transfer band (CTB). The CTB intensity increases the sensitization effect of the host on Eu³⁺ and improves the luminescent properties in NUV and blue light regions. The chromaticity coordinate of the phosphor shifts from (0.658, 0.342) to (0.642, 0.358) due to Zr⁴⁺ substitution, indicating its potential application in the excitation of NUV (395 nm) LED chips.

, authors=Jie SHEN¹, Lina HU¹, Yuanyuan CHENG¹, Jing ZHOU¹, Wen CHEN¹, Wei ZHANG², Hui CAI², authorsList=Jie SHEN, Lina HU, Yuanyuan CHENG, Jing ZHOU, Wen CHEN, Wei ZHANG, Hui CAI, authorCompany=null, correspAuthors=Jing ZHOU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322636214230962886, articleId=1322636213857669828, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=Zr⁴⁺取代对Ba（Mg_1/3Nb_2/3）O₃：Eu³⁺荧光粉结构和荧光特性的影响, columnId=null, journalTitle=硅酸盐学报, columnName=, runingTitle=null, highlight=null, articleAbstract=

采用固相法制备了不同Zr⁴⁺取代量的（Ba_0.97Eu_0.03）（Mg_（1-x）/3Nb_2（1-x）/3Zr_x）O₃荧光粉，研究了Zr⁴⁺取代量对荧光粉的晶体结构以及荧光特性的影响规律。随着Zr⁴⁺取代量的增加，当x=0.05时，体系发生了从六方相到立方相的转变，发光行为有所减弱；当x>0.05时，体系为立方相，Zr⁴⁺的引入使BO₆八面体扭转程度增强，能级简并消除，B—O成键范围变大，基质对近紫外光区域的光吸收增强，来源于基质的电荷迁移带强度增加，增强了对Eu³⁺的敏化作用，使稀土Eu³⁺在近紫外与蓝光区域的激发与发射均得到增强。Zr⁴⁺取代后，荧光粉的色坐标由从（0.658，0.342）移动到（0.642，0.358），是一种适用于近紫外（395 nm） LED芯片激发的红色荧光粉。

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SHEN Jie (1981-), male, Ph.D., Professor. E-mail: shenjie@whut.edu.cn

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SHEN Jie (1981-), male, Ph.D., Professor. E-mail: shenjie@whut.edu.cn

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沈杰（1981—），男，博士，教授。

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沈杰（1981—），男，博士，教授。

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